Investigation on the Adhesion Force between Tetrabutylammonium Bromide Hydrate Particles Using Atomic Force Microscopy
Source abstract
Abstract
This work investigates the adhesion force between tetrabutylammonium bromide (TBAB) hydrate particles dispersed in decane at different temperatures and TBAB concentrations using an atomic force microscopy. The thickness of the quasi-liquid layer (QLL) on the surface of the hydrate particles is calculated based on an adhesion force model. The results of force measurements indicate that the adhesion force between the hydrate particles increases with increasing temperature when TBAB concentration is 30 wt %. The increment of adhesion force between particles could be due to the increase in the QLL thickness on the particle surfaces. Furthermore, the force results also reveal that the adhesion force between hydrate particles(ice) at 253 K decreases when TBAB concentration increases from 0 to 30 wt %. The calculation indicates that QLL on the surface of formed hydrate particles becomes thinner at higher TBAB concentrations, which could be due to the conversion rate of water to hydrate within particles. The thickness of QLL is directly influenced by the temperature and TBAB concentration, which contributes to the adhesion force between hydrate particles.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Methane Hydrates and Related Phenomena · CO2 Sequestration and Geologic Interactions · Surface Modification and Superhydrophobicity
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Beijing Key Laboratory of Urban Oil and Gas Distribution Technology, MOE Key Laboratory of Petroleum Engineering, State Key Laboratory of Natural Gas Hydrates, China University of Petroleum, Beijing. No. 18 Fuxue Road, Changping District, 102249 Beijing, P. R. China
School of Petrochemical Engineering, Lanzhou University of Technology. No. 287, Langongping Road, Qilihe District, Lanzhou, Gansu 730050, P. R. China
Funding
Science and Technology Program of Gansu Province · National Natural Science Foundation of China
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