Inhibiting Cracks in Latte Droplets

Latte is a mixture of coffee and milk and a model of complex fluids containing biomolecules, usually leaving complex deposit patterns after droplet evaporation. Despite the universality and applicability of biofluids, their evaporation and deposition dynamics are not fully understood and controllable because of the complexity of their components. Here we investigate latte droplet evaporation and deposition dynamics, primarily the crack development and inhibition in droplet deposit patterns. With regard to a mixture of milk and coffee, we find that the surfactant-like nature of milk and intermolecular interactions between coffee particles and milk bioparticles are responsible for achieving uniform crack-free deposits. This finding improves our understanding of pattern formation from evaporating droplets with complex biofluids, offering a clue to applications of bioinks with both printability and biocompatibility.