Slurry‐Coated Sulfur/Sulfide Cathode with Li Metal Anode for All‐Solid‐State Lithium‐Sulfur Pouch Cells
Source abstract
Abstract
Abstract All‐solid‐state lithium‐sulfur batteries are strongly considered as the most promising next‐generation electrochemical energy storage systems due to their high safety and energy density. However, in view of practical application, it is difficult to obtain large‐scale solid‐state sulfur cathode continuously. Herein we achieve the large‐scale fabrication of solid sulfur cathode by a facile slurry‐coating process through the screening of various solvents and binder contents. The composite cathodes in all‐solid‐state lithium‐sulfur pouch cells exhibit a high specific capacity of 1169 mAh g−1 and excellent cycling stability. Furthermore, a practical lithium‐sulfur pouch cell with an areal discharge capacity of up to 2.3 mAh cm−2 is also demonstrated. This work makes a leap towards the practical application of all‐solid‐state lithium‐sulfur batteries.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Advanced Battery Materials and Technologies · Advancements in Battery Materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering Tsinghua University Beijing 100084 China
Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing 100081 China
School of Chemical Engineering and Light Industry Guangdong University of Technology Guangzhou 510006 China
Shenzhen Key Laboratory of Functional Polymer College of Chemistry and Chemical Engineering Shenzhen University Shenzhen 518000 China
Funding
National Basic Research Program of China · National Natural Science Foundation of China · China Postdoctoral Science Foundation
References (90)
Show source-provided references
1.
2. 10.1038/s41560-018-0108-110.1038/s41560-018-0108-1 ↗
3. 10.1016/j.chempr.2017.01.00310.1016/j.chempr.2017.01.003 ↗
4. 10.1021/acs.chemrev.7b0011510.1021/acs.chemrev.7b00115 ↗
5. 10.1039/C8EE01373J10.1039/C8EE01373J ↗
6. 10.1002/inf2.1200010.1002/inf2.12000 ↗
7. 10.1016/j.etran.2019.10003310.1016/j.etran.2019.100033 ↗
8.
9. 10.1039/C5CS00410A10.1039/C5CS00410A ↗
10. 10.1002/adma.20140511510.1002/adma.201405115 ↗
11. 10.1002/aenm.20170026010.1002/aenm.201700260 ↗
12. 10.1016/j.jechem.2019.02.00210.1016/j.jechem.2019.02.002 ↗
13. 10.1002/batt.20180002410.1002/batt.201800024 ↗
14. 10.1002/advs.20180050210.1002/advs.201800502 ↗
15. 10.1002/adfm.20190190710.1002/adfm.201901907 ↗
16.
17. 10.1002/adma.20170521910.1002/adma.201705219 ↗
18. 10.1002/aenm.20160163010.1002/aenm.201601630 ↗
19. 10.1002/inf2.1205610.1002/inf2.12056 ↗
20. 10.1038/ncomms1120310.1038/ncomms11203 ↗
21. 10.1002/aenm.20180276810.1002/aenm.201802768 ↗
22. 10.31635/ccschem.019.2018001610.31635/ccschem.019.20180016 ↗
23. 10.1002/batt.20180001310.1002/batt.201800013 ↗
24. 10.1038/s41467-018-06877-910.1038/s41467-018-06877-9 ↗
25.
26. 10.1002/adfm.20170753310.1002/adfm.201707533 ↗
27. 10.1016/j.ensm.2017.09.00710.1016/j.ensm.2017.09.007 ↗
28. 10.1002/chem.20170456810.1002/chem.201704568 ↗
29. 10.1016/j.joule.2018.07.00910.1016/j.joule.2018.07.009 ↗
30. 10.1002/smll.20190395210.1002/smll.201903952 ↗
31. 10.1016/j.chempr.2018.11.01310.1016/j.chempr.2018.11.013 ↗
32. 10.1016/j.ensm.2018.03.01510.1016/j.ensm.2018.03.015 ↗
33. 10.1016/j.jechem.2018.12.01310.1016/j.jechem.2018.12.013 ↗
34. 10.1002/batt.20190011910.1002/batt.201900119 ↗
35. 10.1002/anie.20171084110.1002/anie.201710841 ↗
36. 10.1002/ange.20171084110.1002/ange.201710841 ↗
37.
38. 10.1039/C7EE01004D10.1039/C7EE01004D ↗
39. 10.1016/j.ensm.2018.11.00910.1016/j.ensm.2018.11.009 ↗
40.
41. 10.1007/s11426-017-9164-210.1007/s11426-017-9164-2 ↗
42. 10.1038/natrevmats.2016.10310.1038/natrevmats.2016.103 ↗
43. 10.1021/acsenergylett.7b0017510.1021/acsenergylett.7b00175 ↗
44. 10.1016/j.jechem.2018.11.01610.1016/j.jechem.2018.11.016 ↗
45. 10.1016/j.eng.2018.10.00810.1016/j.eng.2018.10.008 ↗
46.
47. 10.1002/aenm.20180003510.1002/aenm.201800035 ↗
48. 10.1016/j.jechem.2018.12.01710.1016/j.jechem.2018.12.017 ↗
49. 10.1002/anie.20180406810.1002/anie.201804068 ↗
50. 10.1002/ange.20180406810.1002/ange.201804068 ↗
51. 10.1002/anie.20190173910.1002/anie.201901739 ↗
52. 10.1002/ange.20190173910.1002/ange.201901739 ↗
53. 10.1007/s41918-019-00029-310.1007/s41918-019-00029-3 ↗
54.
55. 10.1038/nmat306610.1038/nmat3066 ↗
56. 10.1021/acsami.9b0372610.1021/acsami.9b03726 ↗
57. 10.1002/aenm.20160292310.1002/aenm.201602923 ↗
58.
59. 10.1038/nenergy.2016.3010.1038/nenergy.2016.30 ↗
60. 10.1002/adma.20190113110.1002/adma.201901131 ↗
61.
62. 10.1002/anie.20070390010.1002/anie.200703900 ↗
63. 10.1002/ange.20070390010.1002/ange.200703900 ↗
64. 10.1021/acs.nanolett.6b0175410.1021/acs.nanolett.6b01754 ↗
65. 10.1021/acsenergylett.8b0199710.1021/acsenergylett.8b01997 ↗
66.
67. 10.1002/admi.20180204610.1002/admi.201802046 ↗
68. 10.1016/j.ensm.2018.02.02010.1016/j.ensm.2018.02.020 ↗
69. 10.1016/j.ensm.2019.04.04410.1016/j.ensm.2019.04.044 ↗
70.
71. 10.1002/aenm.20190325310.1002/aenm.201903253 ↗
72. 10.1002/adfm.20190618910.1002/adfm.201906189 ↗
73. 10.1016/j.jechem.2019.03.00610.1016/j.jechem.2019.03.006 ↗
74.
75. 10.1039/C8TA08420C10.1039/C8TA08420C ↗
76. 10.1002/ente.20190007710.1002/ente.201900077 ↗
77.
78. 10.1016/j.ensm.2018.11.01110.1016/j.ensm.2018.11.011 ↗
79. 10.1149/2.0951712jes10.1149/2.0951712jes ↗
80. 10.1039/C9CS00635D10.1039/C9CS00635D ↗
81. 10.1007/s41918-018-0010-310.1007/s41918-018-0010-3 ↗
82. 10.1002/adfm.20160422910.1002/adfm.201604229 ↗
83.
84. 10.1016/j.nanoen.2019.01.00410.1016/j.nanoen.2019.01.004 ↗
85. 10.1021/acsami.7b1617610.1021/acsami.7b16176 ↗
86. 10.1016/S0167-2738(02)00889-510.1016/S0167-2738(02)00889-5 ↗
87. 10.1016/S0378-7753(03)00293-310.1016/S0378-7753(03)00293-3 ↗
88. 10.1002/anie.20171289510.1002/anie.201712895 ↗
89. 10.1002/ange.20171289510.1002/ange.201712895 ↗
90. 10.1016/j.ensm.2019.09.03710.1016/j.ensm.2019.09.037 ↗