journal article·2025-09-22

Enhancing Photocatalytic Performance by One-Step Vapor Deposition of SnSe/SnSe2 Composites

Han Tang, Xu Li, Siwei Luo, Siming Luo, Zuoming He, Xiongqing Wu, Hui Qiao, Yun Fang, Yundan Liu, Xiang Qi, Jianxin Zhong

ACS Applied Energy Materials· Volume 8· Issue 18
Publisher page

Abstract

Two-dimensional materials and their van der Waals heterostructures offer significant advantages in photoelectrochemical (PEC) photodetectors and water splitting due to their unique physical and chemical properties. In this study, SnSe, SnSe 2, and SnSe/SnSe 2 composites were successfully synthesized on FTO glass and carbon cloth substrates using a one-step vapor deposition method. Experimental results demonstrate that the SnSe/SnSe 2 composite exhibits a high photocurrent density (29.83 μA/cm 2 ) and superior stability compared to individual SnSe and SnSe 2 . Moreover, benefiting from its efficient light absorption and synergistic charge transfer, the SnSe/SnSe 2 composite shows excellent photocatalytic performance, achieving a total hydrogen production of 57.4 μmol/cm 2 within 2 h─7.5 times and 5.1 times higher than that of SnSe and SnSe 2, respectively. These findings highlight the significant advantages of composite materials in photocatalysis and water splitting applications. Furthermore, this work presents a simple one-step strategy for the preparation of SnSe/SnSe 2 on various substrates, providing a solid foundation for future research and practical applications in this field.
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Research context

OpenAlex topics: Advanced Photocatalysis Techniques · Chalcogenide Semiconductor Thin Films · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Hunan Key Laboratory for Micro-Nano Energy Materials and Devices, Laboratory for Quantum Engineering and Micro-Nano Energy Technology, and School of Physics and Optoelectronics

Xiangtan University

College of Railway Transportation

Hunan University of Technology

Institute for Quantum Science and Technology

Shanghai University

Funding

National Key Research and Development Program of China · Scientific Research Foundation of Hunan Provincial Education Department · Program for Changjiang Scholars and Innovative Research Team in University · Science Fund for Distinguished Young Scholars of Hunan Province · National Natural Science Foundation of China

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