journal article·2024-07-08Open access

Surface Treatment of Garnet-Type Solid Electrolyte for Suppressing Dendritic Growth

Tsuyoshi Ohnishi, Isao Sakaguchi, Kazunori Takada

ACS Applied Energy Materials· Volume 7· Issue 13

Abstract

High Resolution Image Download MS PowerPoint Slide Garnet-type solid electrolytes are regarded as promising electrolytes for oxide-based solid-state batteries due to their stability against lithium metal. However, lithium metal anodes on garnet-type solid electrolytes often exhibit dendritic growth, leading to internal short-circuit. This study reveals that immersion of the solid electrolytes in an aqueous solution of LiOH is a very simple and effective way to suppress dendritic growth. It removes the contamination layer formed on the electrolyte surface by exposure to ambient air, and it makes the interface to the lithium metal anode conductive and the current density homogeneous.
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Research context

OpenAlex topics: Advanced Battery Materials and Technologies · Perovskite Materials and Applications · Advancements in Battery Materials

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Affiliations

Research Center for Energy and Environmental Science, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan

Research Center for Electronic and Optical Materials, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan

Funding

Ministry of Education, Culture, Sports, Science and Technology · Japan Science and Technology Agency · Advanced Low Carbon Technology Research and Development Program

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