Continuous Anode Slurry Production in Twin-Screw Extruders: Effects of the Process Setup on the Dispersion
Source abstract
Abstract
Screw design in the extrusion process has an important effect on the distribution of material through the extruder, resulting in partially filled sections in the processing zone. Accordingly, the local accumulation of material in the extruder leads to variations in material strain conditions and also influences the local residence time of the material in a given screw section. This work evaluates particle dispersion in anode slurry considering three different screw arrangements. The particle size distribution is considered as a quality parameter representing the microstructure of the battery slurry components and their distribution. Numerical simulation of the material flow behavior through a laboratory extruder was performed to investigate the filling ratios and resulting shear rates for different screw designs and process conditions. The importance of process parameters and a suitable screw configuration to achieve specific particle sizes in battery slurry is discussed.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Recycling and Waste Management Techniques · Aluminum Alloy Microstructure Properties · Molten salt chemistry and electrochemical processes
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Institute of Mechanical Process Engineering and Mechanics, Karlsruhe Institute of Technology, Straße am Forum 8, 76131 Karlsruhe, Germany
Funding
Ministry of Education and Research (Bundesministerium für Bildung und Forschung [BMBF])
References (25)
Show source-provided references
1. From Materials to Cell: State-of-the-Art and Prospective Technologies for Lithium-Ion Battery Electrode Processing10.1021/acs.chemrev.1c00565 ↗
2. Mixing methods for solid state electrodes: Techniques, fundamentals, recent advances, and perspectives10.1016/j.cej.2023.142469 ↗
3. Effects of the Mixing Sequence on Making Lithium Ion Battery Electrodes10.1149/1945-7111/ab95c6 ↗
4. Effect of the Slurry Mixing Process on the Structural Properties of the Anode and the Resulting Fast-Charging Performance of the Lithium-Ion Battery Cell10.1149/1945-7111/ac4cdb ↗
5. Influence of the Mixing and Dispersing Process on the Slurry Properties and the Microstructure and Performance of Ultrathick Cathodes for Lithium–Ion Batteries10.1002/ente.202200484 ↗
6. Digitalization Platform for Sustainable Battery Cell Production: Coupling of Process, Production, and Product Models10.1002/ente.202200801 ↗
7. Impact of Formulation and Slurry Properties on Lithium–ion Electrode Manufacturing10.1002/batt.202300396 ↗
8. Influence of the mixing speed in the rheology of NMC622-based Li-ion battery electrode slurries10.1016/j.powera.2024.100141 ↗
9. Continuous Processing of Cathode Slurry by Extrusion for Lithium–Ion Batteries10.1002/ente.202100250 ↗
10. Semi–Dry Extrusion–Based Processing for Graphite Anodes: Morphological Insights and Electrochemical Performance10.1002/ente.202300341 ↗
11. Kohlgrüber, K. (2019). Co-Rotating Twin-Screw Extruders Fundamentals, Hanser Publications. [1st ed.].10.3139/9781569907481.fm ↗
12. Mechanistic modeling of modular co-rotating twin-screw extruders10.1016/j.ijpharm.2014.08.005 ↗
13. Analysis of flow and mixing in screw elements of corotating twin–screw extruders via SPH10.1002/aic.15607 ↗
14. A composite model for an intermeshing counter–rotating twin–screw extruder and its experimental verification10.1002/pen.24175 ↗
15. Mesoscopic Model of Extrusion during Solvent–Free Lithium–ion Battery Electrode Manufacturing10.1002/batt.202300441 ↗
16. Investigating local residence time and thermomechanical stress profile in twin-screw extrusion of plant proteins by using the moving particle semi-implicit simulation method10.1016/j.jfoodeng.2023.111665 ↗
17. Numerical Investigation of the Local Shear Rate in a Twin–Screw Extruder for the Continuous Processing of Li–Ion Battery Electrode Slurries10.1002/ente.202201517 ↗
18. Modeling of Carbon Black Fragmentation During High–Intensity Dry Mixing Using the Population Balance Equation and the Discrete Element Method10.1002/ente.202200867 ↗
19. Winck, J., Gottschalk, T., and Thommes, M. (2023). Predicting Residence Time and Melt Temperature in Pharmaceutical Hot Melt Extrusion. Pharmaceutics, 15.10.3390/pharmaceutics15051417 ↗
20. Water-Soluble Binders for Lithium-Ion Battery Graphite Electrodes: Slurry Rheology, Coating Adhesion, and Electrochemical Performance10.1002/ente.201700200 ↗
21. Direct recycling of carbon black and graphite from an aqueous anode slurry of lithium-ion batteries by centrifugal fractionation10.1016/j.nxener.2023.100082 ↗
22. DualSPHysics: From fluid dynamics to multiphysics problems10.1007/s40571-021-00404-2 ↗
23. The Carbon Black Dispersion Index DI CB: A Novel Approach Describing the Dispersion Progress of Carbon Black Containing Battery Slurries10.1002/ente.202201299 ↗
24. Vergnes, B. (2021). Average Shear Rates in the Screw Elements of a Corotating Twin-Screw Extruder. Polymers, 13.10.3390/polym13020304 ↗
25. Population balance modelling to describe the particle aggregation process: A review10.1016/j.powtec.2017.12.033 ↗