journal article·2019-07-22

Soluble Telluride-Based Molecular Precursor for Solution-Processed High-Performance Thermoelectrics

Seungki Jo, Sun Hwa Park, Hosun Shin, Inseon Oh, Seung Hwae Heo, Hyeong Woo Ban, Hyewon Jeong, Fredrick Kim, Seungjun Choo, Da Hwi Gu, Seongheon Baek, Soyoung Cho, Jin Sang Kim, Bong-Seo Kim, Ji Eun Lee, Seungwoo Song, Jung-Woo Yoo, Jae Yong Song, Jae Sung Son

ACS Applied Energy Materials· Volume 2· Issue 7
Publisher page

Abstract

The recent interest in wearable electronics suggests flexible thermoelectrics as candidates for the power supply. Herein, we report a solution process to fabricate flexible Sb2Te3 thermoelectric thin films using molecular Sb2Te3 precursors, synthesized by the reduction of Sb2Te3 powder in ethylenediamine and ethanedithiol with superhydride. The fabricated flexible Sb2Te3 thin films exhibit a power factor of ∼8.5 μW cm–1 K−2 at 423 K, maintaining the properties during 1000 bending cycles. FePt nanoparticles are homogeneously embedded in the Sb2Te3 thin film, reducing the thermal conductivity. The current study offers considerable potential for manufacturing high-performance flexible thin film devices.
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Research context

OpenAlex topics: Advanced Thermoelectric Materials and Devices · Thermal Radiation and Cooling Technologies · Thermal properties of materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Materials Science and Engineering, Ulsan National Institute of Science and Technology (UNIST), Ulsan 44919, Republic of Korea

Center for Convergence Property Measurement, Korea Research Institute of Standards and Science (KRISS), Daejeon 34113, Republic of Korea

Center for Electronic Materials, Korea Institute of Science and Technology (KIST), Seoul 02792, Republic of Korea

Energy Conversion Research Center, Korea Electrotechnology Research Institute (KERI), Changwon 51543, Republic of Korea

Funding

National Research Foundation of Korea · Korea Research Institute of Standards and Science · Ministry of Science, ICT and Future Planning · R&D Convergence Program of National Research Council of Science and Technology of Republic of Korea

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