Alkynyl BODIPY-Core Bridged Perylene Diimide Star-Shaped Nonfullerene Acceptors for Efficient Polymer Solar Cells

Xuanlai Zong; Hemraj Dahiya; Yuting Song; Xu Liang; Sarvesh Kumar Pandey; Haijun Xu; Ganesh D. Sharma

doi:10.1021/acsaem.2c03200

journal article·2022-12-26

Alkynyl BODIPY-Core Bridged Perylene Diimide Star-Shaped Nonfullerene Acceptors for Efficient Polymer Solar Cells

Xuanlai Zong, Hemraj Dahiya, Yuting Song, Xu Liang, Sarvesh Kumar Pandey, Haijun Xu, Ganesh D. Sharma

ACS Applied Energy Materials· Volume 5· Issue 12

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Source abstract

Abstract

Two new star-shaped perylene diimide (PDI)-based small-molecule acceptors denoted as BDP-3PDI and BDP-4PDI with BODIPY derivatives as the core and PDI units as peripheral groups were designed and successfully synthesized, and their photophysical and electrochemical properties were studied. When paired with a compatible D–A polymer donor P(BTT-DPP), the polymer solar cells based on the bulk heterojunction active layer attained power conversion efficiencies (PCEs) of about 10.97 and 13.94% for BDP-3PDI and BDP-4PDI, respectively. The higher value of PCE for BDP-4PDI is mainly owing to the enhanced values of the fill factor and short circuit current as compared to BDP-3PDI and related to the more balanced charge transport and blocked charge recombination owing to the appropriate phase separation in the P(BTT-DPP):BDP-4PDI active layer as compared to P(BTT-DPP):BDP-3PDI.

Source: openalex_inverted_index · Quality: baseline

Research context

Polymers

OpenAlex topics: Organic Electronics and Photovoltaics · Conducting polymers and applications · Perovskite Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Jiangsu Co-innovation Center of Efficient Processing and Utilization of Forest Resources, College of Chemical Engineering, Nanjing Forestry University, Nanjing 210037, P. R. China

Department of Physics, The LNM Information Technology, Jamdoli, Jaipur, Rajasthan 302031, India

School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, P. R. China

Department of Inorganic and Physical Chemistry, Indian Institute of Science, Bengaluru, Karnataka 560012, India

Department of Electronics and Communication Engineering, The LNM Information Technology, Jamdoli, Jaipur, Rajasthan 302031, India

Funding

University Grants Commission · School of Chemistry and Chemical Engineering, Henan Normal University

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