DataVXACS Applied Energy MaterialsPaper
journal article·2020-12-28

Cathode-Supported-Electrolyte Configuration for High-Performance All-Solid-State Lithium–Sulfur Batteries

Liu Wang, Xuesong Yin, Chengbin Jin, Chen Lai, Gan Qu, Guangyuan Wesley Zheng

ACS Applied Energy Materials· Volume 3· Issue 12
Publisher page
Source abstract

Abstract

The sluggish conversion reaction of sulfur and poor interfacial contact restrict electrochemical performance and practical application of all-solid-state Li–S batteries. Herein, we present a rational design of cell structure with a cathode-supported-electrolyte configuration to attain high-performance all-solid-state Li–S batteries. A mechanically robust sulfur cathode was constructed, and a slurry-based polymer electrolyte layer was subsequently cast on the cathode to form an intimate interfacial contact. The resulting battery shows a high specific capacity and good cycle performance. As a proof-of-concept, full cells with variable configurations, excellent flexibility, and safety features are demonstrated.
Source: openalex_inverted_index · Quality: baseline

Research context

Energy storagePolymers

OpenAlex topics: Advanced Battery Materials and Technologies · Advancements in Battery Materials · Advanced Battery Technologies Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemical and Biomolecular Engineering, National University of Singapore, 117585, Singapore

Institute of Materials Research and Engineering, A*STAR (Agency for Science, Technology and Research), 138634, Singapore

College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China

School of Chemical Engineering and Technology, Xi’an Jiaotong University, Xi’an 710049, China

College of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, China

Funding

Ministry of Education - Singapore

References (30)

Show source-provided references
1. 10.1002/anie.20130476210.1002/anie.201304762 ↗
2. 10.1002/adma.20140511510.1002/adma.201405115 ↗
3. 10.1038/nenergy.2016.13210.1038/nenergy.2016.132 ↗
4. 10.1039/C9CS00635D10.1039/C9CS00635D ↗
5. 10.1038/natrevmats.2016.10310.1038/natrevmats.2016.103 ↗
6. 10.1038/nenergy.2016.3010.1038/nenergy.2016.30 ↗
7. 10.1038/nmat306610.1038/nmat3066 ↗
8. 10.1038/2881810.1038/28818 ↗
9. 10.1038/s41565-019-0465-310.1038/s41565-019-0465-3 ↗
10. 10.1002/adfm.20190104710.1002/adfm.201901047 ↗
11. 10.1002/adfm.20170757010.1002/adfm.201707570 ↗
12. 10.1002/adfm.20170753310.1002/adfm.201707533 ↗
13. 10.1021/acs.chemmater.9b0028210.1021/acs.chemmater.9b00282 ↗
14. 10.1039/C8EE00907D10.1039/C8EE00907D ↗
15. 10.1002/aenm.20160292310.1002/aenm.201602923 ↗
16. 10.1021/acs.nanolett.6b0175410.1021/acs.nanolett.6b01754 ↗
17. 10.1021/acs.nanolett.8b0501910.1021/acs.nanolett.8b05019 ↗
18. 10.1038/s41560-019-0349-710.1038/s41560-019-0349-7 ↗
19. 10.1149/1945-7111/ab76a410.1149/1945-7111/ab76a4 ↗
20. 10.1002/aenm.20180292710.1002/aenm.201802927 ↗
21. 10.1039/C7EE01004D10.1039/C7EE01004D ↗
22. 10.1021/acs.nanolett.9b0088210.1021/acs.nanolett.9b00882 ↗
23. 10.1039/C5TA03471J10.1039/C5TA03471J ↗
24. 10.1039/C8EE02617C10.1039/C8EE02617C ↗
25. 10.1002/aenm.20190184110.1002/aenm.201901841 ↗
26. 10.1016/0032-3861(95)96855-310.1016/0032-3861(95)96855-3 ↗
27. 10.1039/D0EE00342E10.1039/D0EE00342E ↗
28. 10.1002/advs.20200130310.1002/advs.202001303 ↗
29. 10.1002/aenm.20190076310.1002/aenm.201900763 ↗
30. 10.1002/adfm.20200181210.1002/adfm.202001812 ↗