Simultaneously ultra-low dielectric loss and rapid discharge time in Ta2O5 doped niobate-based glass–ceramics
Source abstract
Abstract
SrO–Na2O–Nb2O5–SiO2 (SNNS) glass–ceramics with Ta2O5 dopants were prepared by a method of conventional melt-quenching and crystallization. The effects of different contents of Ta2O5 dopants on the microstructures, dielectric properties, energy storage densities and discharge properties of SNNS glass–ceramics were exhaustively investigated. Results showed that the doping of Ta5+ cations can significantly improve the dielectric constant of SNNS glass–ceramics, attributing to the increase in NaNbO3 precipitation. In addition, an optimal amount of Ta2O5 doping can effectively reduce the grain agglomeration of the glass–ceramics and improve their electric breakdown strength. A maximum theoretical energy storage density reached 15.22 J cm–3 over SNNS glass–ceramics with 2 mol% of Ta2O5 dopants; in particular, approximately 0.41% of ultra-low dielectric loss was obtained in this composition. Besides, a tremendous instantaneous power density of 125 MW cm–3 was achieved at 400 kV cm–1 electric field in the single-layer capacitor based on those SNNS glass–ceramics, as well as a rapid discharge time of 10 ns. All these outcomes demonstrate the doped SNNS glass–ceramics have a giant potential for pulse power applications.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Ferroelectric and Piezoelectric Materials · Semiconductor materials and devices · Dielectric materials and actuators
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (44)
Show source-provided references
1. Li F, Jiang T, Zhai J, Shen B, Zeng H (2018) Exploring novel bismuth-based materials for energy storage applications. J Mater Chem C 6:7976–7981. https://doi.org/10.1039/c8tc02801j10.1039/c8tc02801j ↗
2. Huang YH, Wu YJ, Qiu WJ, Li J, Chen XM (2015) Enhanced energy storage density of Ba0.4Sr0.6TiO3–MgO composite prepared by spark plasma sintering. J Eur Ceram Soc 35(5):1469–1476. https://doi.org/10.1016/j.jeurceramsoc.2014.11.02210.1016/j.jeurceramsoc.2014.11.022 ↗
3. Pan Z, Yao L, Zhai J, Yao X, Chen H (2018) Interfacial coupling effect in organic/inorganic nanocomposites with high energy density. Adv Mater 30:1705662. https://doi.org/10.1002/adma.20170566210.1002/adma.201705662 ↗
4. Li Z, Fredin LA, Tewari P et al (2010) In situ catalytic encapsulation of core-shell nanoparticles having variable shell thickness: dielectric and energy storage properties of high-permittivity metal oxide nanocomposites. Chem Mater 22:5154–5164. https://doi.org/10.1021/cm100949310.1021/cm1009493 ↗
5. Liu SH, Shen B, Hao HS, Zhai JW (2019) Glass-ceramic dielectric materials with high energy density and ultra-fast discharge speed for high power energy storage applications. J Mater Chem C 7:15118–15135. https://doi.org/10.1039/c9tc05253d10.1039/c9tc05253d ↗
6. Gorzkowski EP, Pan MJ, Bender B, Wu CCM (2007) Glass-ceramics of barium strontium titanate for high energy density capacitors. J Electroceram 18:269–276. https://doi.org/10.1007/s10832-007-9127-110.1007/s10832-007-9127-1 ↗
7. Xiao S, Xiu S, Xue S, Shen B, Zhai J (2016) Optimization of the dielectric properties and energy storage density in (K2O, SrO)–Nb2O5–B2O3–Al2O3–SiO2 glass–ceramics. J Mater Sci 51:5880–5888. https://doi.org/10.1007/s10853-016-9889-410.1007/s10853-016-9889-4 ↗
8. Yadav AK, Gautam C (2014) Dielectric behavior of perovskite glass ceramics. J Mater Sci Mater Electron 25:5165–5187. https://doi.org/10.1007/s10854-014-2311-610.1007/s10854-014-2311-6 ↗
9. Xiu S, Xiao S, Xue S, Shen B, Zhai J (2016) Crystallization kinetics behaviour and dielectric properties of strontium barium niobate-based glass–ceramics. J Mater Sci Mater Electron 27:5324–5330. https://doi.org/10.1007/s10854-016-4431-710.1007/s10854-016-4431-7 ↗
10. Wang S, Tian J, Jiang T, Zhai J, Shen B (2018) Effect of phase structures on dielectric properties and energy storage performances in Na2O-BaO-PbO-Nb2O5-SiO2-Al2O3 glass-ceramics. Ceram Int 44:23109–23115. https://doi.org/10.1016/j.ceramint.2018.09.11810.1016/j.ceramint.2018.09.118 ↗
11. Li C, Zhang Q, Tang Q, Zhou H, Tan F, Du J (2016) Dielectric and energy storage properties of BaO-SrO-Na2O-Nb2O5-SiO2 glass-ceramics with different crystallization times. J Electron Mater 45:3025–3029. https://doi.org/10.1007/s11664-015-4298-z10.1007/s11664-015-4298-z ↗
12. Song J, Chen G (2013) Dielectric behavior and energy storage properties in BaO–SrO–Nb2O5–B2O3 system glass–ceramics with Gd2O3 addition. J Mater Sci Mater Electron 25:349–354. https://doi.org/10.1007/s10854-013-1593-410.1007/s10854-013-1593-4 ↗
13. Zhou Y, Zhang Q, Luo J, Tang Q, Du J (2011) Structural and dielectric characterization of Gd2O3-added BaO–Na2O–Nb2O5–SiO2 glass–ceramic composites. Struct Mater 65:296–299. https://doi.org/10.1016/j.scriptamat.2011.04.02710.1016/j.scriptamat.2011.04.027 ↗
14. Liu TY, Chen GH, Song J, Yuan CL (2013) Crystallization kinetics and dielectric characterization of CeO2-added BaO–SrO–Nb2O5–B2O3–SiO2 glass-ceramics. Ceram Int 39:5553–5559. https://doi.org/10.1016/j.ceramint.2012.12.06910.1016/j.ceramint.2012.12.069 ↗
15. Tian J, Wang S, Jiang T, Chen K, Zhai J, Shen B (2019) Ultrahigh energy storage density and excellent charge-discharge properties of Bi2O3-Nb2O5-SiO2-Al2O3 glass ceramic with CeO2 doping. J Electron Mater 48:6183–6188. https://doi.org/10.1007/s11664-019-07432-y10.1007/s11664-019-07432-y ↗
16. Zhao Z, Liang X, Zhang T, Hu K, Li S, Zhang Y (2020) Effects of cerium doping on dielectric properties and defect mechanism of barium strontium titanate glass-ceramics. J Eur Ceram Soc 40:712–719. https://doi.org/10.1016/j.jeurceramsoc.2019.10.02310.1016/j.jeurceramsoc.2019.10.023 ↗
17. Jiang T, Chen K, Shen B, Zhai J (2019) Enhanced energy-storage density in sodium-barium-niobate based glass-ceramics realized by doping CaF2 nucleating agent. J Mater Sci Mater Electron 30:15277–15284. https://doi.org/10.1007/s10854-019-01900-110.1007/s10854-019-01900-1 ↗
18. Zheng J, Chen GH, Yuan CL et al (2016) Dielectriccharacterization and energy-storage performance of lead-free niobateglass–ceramics added with La2O3. Ceram Int 42:1827–1832. https://doi.org/10.1016/j.ceramint.2015.09.14610.1016/j.ceramint.2015.09.146 ↗
19. Chakrabarti A, Molla AR (2020) Zirconia assisted crystallization of ferroelectric BaBi2Nb2O9 based glass-ceramics: kinetics, optical and dielectrical properties. J Alloys Compd 844:156181. https://doi.org/10.1016/j.jallcom.2020.15618110.1016/j.jallcom.2020.156181 ↗
20. Chakrabarti A, Tarafder A, Molla AR (2018) Synthesis of Eu3+-doped BaBi2Ta2O9 based glass-ceramic nanocomposites: optical and dielectric properties. J Am Ceram Soc 101:231–243. https://doi.org/10.1111/jace.1521710.1111/jace.15217 ↗
21. Reddy ASS, Brik MG, Kumar JS et al (2016) Structural and electrical properties of zinc tantalum borate glass ceramic. Ceram Int 42:17269–17282. https://doi.org/10.1016/j.ceramint.2016.08.02210.1016/j.ceramint.2016.08.022 ↗
22. Xiao S, Xiu S, Xue S, Shen B, Zhai J (2015) Crystallization behavior and dielectric properties of K2O–SrO–Nb2O5–B2O3–Al2O3–SiO2 glass-ceramic for energy storage. J Alloys Compd 648:745–750. https://doi.org/10.1016/j.jallcom.2015.07.04710.1016/j.jallcom.2015.07.047 ↗
23. Othman AA, Tahon K, Osman MA (2002) Glass transition and crystallization kinetic studies in Mg0.10As0.34Se0.56 chalcogenide glass by using non-isothermal techniques. Phys B 31:356–365. https://doi.org/10.1016/S0921-4526(01)01029-810.1016/S0921-4526(01)01029-8 ↗
24. Zhao L, Liu Q, Gao J, Zhang SJ, Li JF (2017) Lead-free antiferroelectric silver niobate tantalate with high energy storage performance. Adv Mater 29:7. https://doi.org/10.1002/adma.20170182410.1002/adma.201701824 ↗
25. Khan HU, Alam K, Mateenullah M, Blaschke T, Haq BS (2015) Synthesis and characterization of solid solution Ag(NbxTa1−x)O3 (x = 0, 0.25, 0.5, 0.75, 1.0). J Eur Ceram Soc 35:2775–2789. https://doi.org/10.1016/j.jeurceramsoc.2015.04.00710.1016/j.jeurceramsoc.2015.04.007 ↗
26. Yang Z, Gu R, Wei L, Ren H (2010) Phase formation, microstructure and dielectric properties of Sr0.53Ba0.47Nb2-xTaxO6 ceramics. J Alloys Compd 504:211–216. https://doi.org/10.1016/j.jallcom.2010.05.09310.1016/j.jallcom.2010.05.093 ↗
27. Rangarajan B, Jones B, Shrout T, Lanagan M (2007) Barium/lead-rich high permittivity glass-ceramics for capacitor applications. J Am Ceram Soc 90:784–788. https://doi.org/10.1111/j.1551-2916.2006.01470.x10.1111/j.1551-2916.2006.01470.x ↗
28. Kolodiaznyi T, Sakurai H, Isobe M et al (2015) Superconductivity and crystal structural origins of the metal-insulator transition in Ba6−xSrxNb10O30 tetragonal tungsten bronzes. Phys Rev B 92:214508. https://doi.org/10.1103/PhysRevB.92.21450810.1103/PhysRevB.92.214508 ↗
29. Bian JJ, Otonicar M, Spreitzer M, Vengust D, Suvorov D (2019) Structural evolution, dielectric and energy storage properties of Na(Nb1−xTax)O3 ceramics prepared by spark plasma sintering. J Eur Ceram Soc 39:2339–2347. https://doi.org/10.1016/j.jeurceramsoc.2019.02.00710.1016/j.jeurceramsoc.2019.02.007 ↗
30. Xu L, Wu S, Zhu K et al (2021) Enhanced piezoelectricity and reduced leakage current of a novel (1–x)Bi0.5Na0.5TiO3–x(Sr0.7Bi0.2□0.1)TiO3 thin film. Inorg Chem Front 8:700–710. https://doi.org/10.1039/d0qi01169j10.1039/d0qi01169j ↗
31. Sharma S, Sharma H, Kumar S, Thakur S, Kotnala RK, Negi NS (2020) Analysis of sintering temperature effects on structural, dielectric, ferroelectric, and piezoelectric properties of BaZr0.2Ti0.8O3 ceramics prepared by sol–gel method. J Mater Sci Mater Electron 31:19168–19179. https://doi.org/10.1007/s10854-020-04453-w10.1007/s10854-020-04453-w ↗
32. Song X, Zhang Y, Chen Y, Yang D, Shen Z (2016) SiO2/Al2O3 ratio dependence of microstructures and dielectric properties in barium strontium titanate glass ceramics. Ceram Int 42:18453–18458. https://doi.org/10.1016/j.ceramint.2016.08.18010.1016/j.ceramint.2016.08.180 ↗
33. Young A, Hilmas G, Zhang SC, Schwartz RW (2007) Effect of liquid-phase sintering on the breakdown strength of barium titanate. J Am Ceram Soc 90:1504–1510. https://doi.org/10.1111/j.1551-2916.2007.01637.x10.1111/j.1551-2916.2007.01637.x ↗
34. Chu BJ, Zhou X, Neese B, Zhang QM, Bauer F (2006) Relaxor ferroelectric poly (vinylidene fluoride-trifluoroethylene-chlorofluoroethylene) terpolymer for high energy density storage capacitors. IEEE Trans Dielectr Electr Insul 13:1162–1169. https://doi.org/10.1109/TDEI.2006.24784510.1109/TDEI.2006.247845 ↗
35. Young AL, Hilmas GE, Zhang SC, Schwartz RW (2007) Mechanical vs. electrical failure mechanisms in high voltage, high energy density multilayer ceramic capacitors. J Mater Sci 42:5613–5619. https://doi.org/10.1007/s10853-006-1116-210.1007/s10853-006-1116-2 ↗
36. Adak MK, Mukherjee A, Chowdhury A, Khatun J, Ghorai UK, Dhak D (2018) Electrical and energy storage properties of nickel substituted barium bismuth niobate nano-ceramics prepared by chemical route. J Mater Sci Mater Electron 29:15847–15858. https://doi.org/10.1007/s10854-018-9671-210.1007/s10854-018-9671-2 ↗
37. Rafiq MA, Maaz K, Karim S, Oh Cho S, Hasan MM (2012) Temperature induced delocalization of charge carriers and metallic phase in Co0.6Sn0.4Fe2O4 nanoparticles. J Appl Phys 112:063718. https://doi.org/10.1063/1.475455910.1063/1.4754559 ↗
38. Wang H, Liu J, Zhai J, Pan Z, Shen B (2017) Effects of Sr substitution for Ba on dielectric and energy-storage properties of SrO-BaO-K2O-Nb2O5-SiO2 glass-ceramics. J Eur Ceram Soc 37:3917–3925. https://doi.org/10.1016/j.jeurceramsoc.2017.04.04910.1016/j.jeurceramsoc.2017.04.049 ↗
39. Wang S, Tian J, Liu J, Yang K, Shen B, Zhai J (2018) Ultrahigh energy storage density and instantaneous discharge power density in BaO–PbO–Na2O–Nb2O5–SiO2–Al2O3 glass-ceramics. J Mater Chem C 6:12608–12614. https://doi.org/10.1039/c8tc04096f10.1039/c8tc04096f ↗
40. Xu R, Zhu Q, Xu Z, Feng Y, Wei X (2019) PLZST antiferroelectric ceramics with promising energy storage and discharge performance for high power applications. J Am Ceram Soc 103:1831–1838. https://doi.org/10.1111/jace.1687810.1111/jace.16878 ↗
41. Yang K, Liu J, Shen B, Zhai J, Wang S, Tian J (2018) Effects of TiO2 addition on dielectric and energy storage properties of BaO-K2O-Nb2O5-SiO2 glass ceramics. Ceram Int 44:6181–6185. https://doi.org/10.1016/j.ceramint.2018.01.00210.1016/j.ceramint.2018.01.002 ↗
42. Zhang H, Chen X, Cao F, Wang G, Dong X (2010) Charge-discharge properties of an antiferroelectric ceramics capacitor under different electric fields. J Am Ceram Soc 93:4015–4017. https://doi.org/10.1111/j.1551-2916.2010.04226.x10.1111/j.1551-2916.2010.04226.x ↗
43. Chen GH, Zheng J, Yuan CL et al (2016) Enhanced energy storage properties of P2O5 modified niobate-based B2O3 system glass ceramic composites. Mater Lett 176:46–48. https://doi.org/10.1016/j.matlet.2016.04.09610.1016/j.matlet.2016.04.096 ↗
44. Xu C, Liu Z, Chen X et al (2017) Pulse discharge properties of PLZST antiferroelectric ceramics compared with ferroelectric and linear dielectrics. AIP Adv. https://doi.org/10.1063/1.500580810.1063/1.5005808 ↗