journal article·2023-08-22Open access

Monolayer Capping Provides Close to Optimal Resistance to Laser Dewetting of Au Films

Christopher P. Murray, Daniyar Mamyraimov, Mugahid Ali, Clive Downing, Ian M. Povey, David McCloskey, David D. O’Regan, John F. Donegan

Abstract

High Resolution Image Download MS PowerPoint Slide Next-generation heat-assisted magnetic recording (HAMR) relies on fast, localized heating of the magnetic medium during the write process. Au plasmonic near-field transducers are an attractive solution to this challenge, but increased thermal stability of Au films is required to improve long-term reliability. This work compares the effect of nanoscale Al, AlO x, and Ta capping films on Au thin films with Ti or Ta adhesion layers for use in HAMR and other high-temperature plasmonic applications. Thermal stability is investigated using a bespoke laser dewetting system, and SEM and AFM are extensively used to interrogate the resulting dewet areas. The most effective capping layers are found to be 0.5–1 nm of Al or AlO x, which can eliminate dewetting under certain conditions. Even one monolayer of AlO x is shown to be highly effective in reducing dewetting. In the case of thicker capping layers of Ta and AlO x, the Au film can easily dewet underneath, leaving an intact capping layer. It is concluded that thinner capping layers are most effective against dewetting as the Au cannot dewet without breaking them and pulling them apart during the dewetting process. A simple model based on energetics considerations is developed, which explains how thinner capping layers can more effectively protect the metal from pore or fissure creation. The model provides some convenient guidelines for choosing both the substrate and capping layer, for a given metal, to maximize the resistance to laser-induced damage.
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Research context

OpenAlex topics: Fluid Dynamics and Thin Films · Optical Coatings and Gratings · Semiconductor materials and devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Physics, CRANN and AMBER, Trinity College Dublin, The University of Dublin, Dublin 2, Ireland

Tyndall National Institute, Lee Maltings, Prospect Row, Cork T12 R5CP, Ireland

Funding

Science Foundation Ireland · ASRC

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