journal article·2015-04

High-temperature wetting and interfacial interaction between liquid Al and TiB2 ceramic

L. Xi, I. Kaban, R. Nowak, B. Korpała, G. Bruzda, N. Sobczak, N. Mattern, J. Eckert

Journal of Materials Science· Volume 50· Issue 7
Publisher page

Abstract

The wetting behaviour and interfacial interactions between liquid Al and TiB2 ceramic have been studied by the sessile drop technique in the temperature range from 700 to 1400 °C. At about 800 °C, liquid Al starts to wet TiB2 and at about 1000 °C it completely spreads over the ceramic. Al3Ti and Al2O3 are found to be the main phases precipitating at the interface. Starting from 1000 °C, liquid Al either fill pores or penetrates along the grain boundaries of the TiB2 ceramic. Scanning electron microscopy analysis of the interfaces evidences that the TiB2 grains remain intact after the aluminium melt/ceramic interaction even at 1400 °C.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Aluminum Alloys Composites Properties · Advanced ceramic materials synthesis · Aluminum Alloy Microstructure Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (35)

Show source-provided references
1. Basu B, Balani K (2011) Advanced structural ceramics. Wiley, Hoboken10.1002/9781118037300 ↗
2. Justin JF, Jankowiak A (2011) Ultra high temperature ceramics: densification, properties and thermal stability. AerospaceLab 3:AL03-08
3. Witusiewicz VT, Bondar AA, Hecht U, Rex S, Velikanova TYa (2008) The Al–B–Nb–Ti system. Re-assessment of the constituent binary systems B-Nb and B-Ti on the basis of new experimental data. J Alloys Compd 448:185–19410.1016/j.jallcom.2006.10.034 ↗
4. Smith AV, Chung DDL (1996) Titanium diboride particle-reinforced aluminium with high wear resistance. J Mater Sci 31:5961–5973. doi: 10.1007/BF0115214610.1007/BF01152146 ↗
5. Bayraktar E, Ayari F, Katundi D, Chevalier J-P, Bonnet F (2011) Damage analysis of the ceramic reinforced steel matrix composites sheets: experimental and numerical study. J Achiev Mater Manufact Eng 49:53–61
6. Gupta N, Prasad VVB, Madhu V, Basu B (2012) Ballistic studies on TiB2-Ti functionally graded armor ceramics. Defence Sci J 62:382–38910.14429/dsj.62.2666 ↗
7. Jones GP, Pearson J (1976) Factors affecting the grain-refinement of aluminum using titanium and boron additives. Metall Trans B 7:223–23410.1007/BF02654921 ↗
8. Greer AL, Bunn AM, Tronche A, Evans PV, Bristow DJ (2000) Modelling of inoculation of metallic melts: application to grain refinement of aluminium by Al-Ti-B. Acta Mater 48:2823–283510.1016/S1359-6454(00)00094-X ↗
9. Kaban I, Köhler M, Ratke L, Hoyer W, Mattern N, Eckert J, Greer AL (2011) Interfacial tension, wetting and nucleation in Al-Bi and Al-Pb monotectic alloys. Acta Mater 59:6880–688910.1016/j.actamat.2011.07.031 ↗
10. Rhee SK (1970) Wetting of ceramics by liquid aluminum. J Am Ceram Soc 53:386–38910.1111/j.1151-2916.1970.tb12138.x ↗
11. Samsonov GV, Panasyuk AD, Borovikova MS (1973) Contact reaction between refractory compounds and liquid metals. Acad Sci Ukra SSR 12:403–407
12. Weirauch DA Jr, Krafick WJ, Ackart G, Ownby PD (2005) The wettability of titanium diboride by molten aluminium drops. J Mater Sci 40:2301–2306. doi: 10.1007/s10853-005-1949-010.1007/s10853-005-1949-0 ↗
13. Dorward RC (1982) Aluminum penetration and fracture of titanium diboride. J Am Ceram Soc 65:C-610.1111/j.1151-2916.1982.tb09927.x ↗
14. Zdaniewski WA (1985) Role of microstructure and intergranular phases in stress corrosion of TiB2 exposed to liquid aluminum. J Am Ceram Soc 68:C-309–C-31210.1111/j.1151-2916.1985.tb16154.x ↗
15. Nord-Varhaug K (1996) TEM investigation of impurity phases and the penetration of liquid aluminum in hot isostatically pressed TiB2 compacts. J Am Ceram Soc 79:1147–115410.1111/j.1151-2916.1996.tb08566.x ↗
16. Heidari H, Alamdari H, Dubéa D, Schulz R (2012) Interaction of molten aluminum with porous TiB2-based ceramics containing Ti-Fe additives. J Eur Ceram Soc 32:937–94510.1016/j.jeurceramsoc.2011.10.053 ↗
17. Forsthoefel K, Sneddon LG (2004) Precursor routes to Group 4 metal borides, and metal boride/carbide and metal boride/nitride composites. J Mater Sci 39:6043–6049. doi: 10.1023/B:JMSC.0000041700.54302.0d10.1023/B:JMSC.0000041700.54302.0d ↗
18. Köhler M (2008) Aufbau und Erprobung eines Messplatzes zur Untersuchung der Oberflächenspannung flüssiger Metalllegierungen nach der Methode des liegenden Tropfens. Diploma thesis, Chemnitz University of Technology, Chemnitz, Germany
19. Sobczak N, Nowak R, Radziwill W, Budzioch J, Glenz A (2008) Experimental complex for investigations of high temperature capillarity phenomena. Mater Sci Eng A 495:43–4910.1016/j.msea.2007.11.094 ↗
20. Liggieri L, Passerone A (1989) An automatic technique for measuring the surface tension of liquid metals. High Temp Technol 7:82–8610.1080/02619180.1989.11753417 ↗
21. Cichy H, Fromm E (1991) Oxidation kinetics of metal films at 300 K studied by the piezoelectric quartz crystal microbalance technique. Thin Solid Films 195:147–15810.1016/0040-6090(91)90267-2 ↗
22. Martin M, Fromm E (1993) Kinetics of aluminium film oxidation measured by a modified quartz crystal microbalance. Thin Solid Films 236:199–20310.1016/0040-6090(93)90669-G ↗
23. Devyatkin SV, Kaptay G (2000) Chemical and electrochemical behavior of titanium diboride in cryolite-alumina melt and in molten aluminum. J Solid State Chem 154:107–10910.1006/jssc.2000.8819 ↗
24. Coudurier L, Adorian J, Pique D, Eustathopoulos N (1984) Etude de la mouillabilité par l’aluminium liquide de l’alumine et de l’alumine recouverte d’une couche de métal ou de composé réfractaire. Rev Int Hautes Tempér Réfract 21:81–93
25. Hehn W, Fromm E (1988) Anfangsstadium der Oxidation von Alumini- umschmelzen bei Drücken unterhalb von 10−6 bar. Aluminium 64:180–185
26. Sobczak N, Astana R, Radziwill W, Nowak R, Kudyba A (2007) The role of aluminum oxidation in the wetting-bonding relationship of Al/oxide couples. Arch Metal Mater 52:55–65
27. Koh YH, Lee SY, Kim HE (2001) Oxidation behavior of TiB2 at elevated temperatures. J Am Ceram Soc 84:239–24110.1111/j.1151-2916.2001.tb00641.x ↗
28. Avraham S, Kaplan WD (2005) Reactive wetting of rutile by liquid aluminium. J Mater Sci 40:1093–1100. doi: 10.1007/s10853-005-6922-410.1007/s10853-005-6922-4 ↗
29. Sobczak N, Stobierski L, Radziwill W, Ksiazek M, Warmuzek M (2004) Wettability and interfacial reactions in Al/TiO2. Surf Interface Anal 36:1067–107010.1002/sia.1838 ↗
30. Feng CF, Froyen L (2000) Formation of Al3Ti and Al2O3 from an Al-TiO2 system for preparing in situ aluminum matrix composites. Compos A 31A:385–39010.1016/S1359-835X(99)00041-X ↗
31. Gheorghe I, Rack HJ (2002) Reactive infiltration of 25 vol pct TiO2/Al composites. Metall Mater Trans A 33:2155–216210.1007/s11661-002-0047-z ↗
32. Dake LS, Lad RJ (1993) Electronic and chemical interactions at aluminum/TiO2(110) interfaces. Surf Sci 289:297–30610.1016/0039-6028(93)90662-4 ↗
33. Gotman I, Koczak MJ (1994) Fabrication of Al matrix in situ composites via self-propagating synthesis. Mater Sci Eng A 187:189–19910.1016/0921-5093(94)90347-6 ↗
34. Frage N, Frumin N, Levin L, Polak M, Dariel MP (1998) High-temperature phase equilibria in the Al-rich corner of the Al-Ti-C system. Metal Mater Trans A 29:1341–134510.1007/s11661-998-0260-5 ↗
35. Froumin N, Frage N, Polak M, Dariel MP (1997) Wettability and phase formation in TiCx/Al system. Scripta Mater 37:1263–126710.1016/S1359-6462(97)00235-2 ↗