journal article·2023-07

Fe2O3/BiVO4 heterogeneous photo-Fenton catalyst with excellent dye degradation performance prepared by ultrasonic-assisted calcination

Jingjing Li, Junhua You, Zhiwei Wang, Yao Zhao, Jingsheng Xu, Mingyi Duan, Hangzhou Zhang

Journal of Materials Science· Volume 58· Issue 25
Publisher page

Abstract

A series of Fe2O3/BiVO4 composite photo-Fenton catalysts were prepared by a simple ultrasonic-assisted calcination method. By changing the calcination temperature, FB-2 with tetragonal structure BiVO4 has excellent photo-Fenton performance. The crystal structure and chemical composition of the composite catalyst were studied by a series of characterizations. Under 5 W LED illumination, 97% rhodamine B dye (Rh B) was degraded within 40 min in FB-2 sample, which was attributed to the high efficiency of photogenic electron–hole pair separation. The subsequent capture experiment and Tafel test proved that h+, e−, ·OH were the main active substances in the degradation process and the flow direction of electrons in the reaction process. The composite catalyst has good cyclic stability and efficient photo-Fenton catalytic degradation performance, and has good reference value for the degradation of water dyes.
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Research context

OpenAlex topics: Advanced Photocatalysis Techniques · TiO2 Photocatalysis and Solar Cells · Advanced oxidation water treatment

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (35)

Show source-provided references
1. Hitam CNC, Jalil AA (2020) A review on exploration of Fe2O3 photocatalyst towards degradation of dyes and organic contaminants. J Environ Manag 258:110050. https://doi.org/10.1016/j.jenvman.2019.11005010.1016/j.jenvman.2019.110050 ↗
2. Xu M, Yang J, Sun C, Liu L, Cui Y, Liang B (2020) Performance enhancement strategies of bi-based photocatalysts: a review on recent progress. Chem Eng J. https://doi.org/10.1016/j.cej.2020.12440210.1016/j.cej.2020.124402 ↗
3. Li J, You J, Wang Z et al (2022) Application of α-Fe2O3-based heterogeneous photo-Fenton catalyst in wastewater treatment: a review of recent advances. J Environ Chem Eng. https://doi.org/10.1016/j.jece.2022.10832910.1016/j.jece.2022.108329 ↗
4. Tokunaga S, Kato H, Kudo A (2001) Selective preparation of monoclinic and tetragonal BiVO4 with scheelite structure and their photocatalytic properties. Chem Mater 13:4624–4628. https://doi.org/10.1021/cm010339010.1021/cm0103390 ↗
5. Wen Y, Zhao Y, Guo M, Xu Y (2019) Synergetic effect of Fe2O3 and BiVO4 as photocatalyst nanocomposites for improved photo-Fenton catalytic activity. J Mater Sci 54:8236–8246. https://doi.org/10.1007/s10853-019-03511-x10.1007/s10853-019-03511-x ↗
6. Wang W, Zhao W, Zhang H, Dou X, Shi H (2021) 2D/2D step-scheme α-Fe2O3/Bi2WO6 photocatalyst with efficient charge transfer for enhanced photo-Fenton catalytic activity. Chin J Catal 42:97–106. https://doi.org/10.1016/s1872-2067(20)63602-610.1016/s1872-2067(20)63602-6 ↗
7. Wang W, Zhao W, Huang H, Chen R, Shi H (2021) A 2D/2D S-scheme photo-Fenton catalyst based on ultrathin Bi2MoO6 and Fe2O3 hexagonal nanosheets for efficient tetracycline degradation. Catal Sci Technol 11:2948–2956. https://doi.org/10.1039/d1cy00051a10.1039/d1cy00051a ↗
8. Jiang J, Gao J, Li T et al (2019) Visible-light-driven photo-Fenton reaction with α-Fe2O3/BiOI at near neutral pH: boosted photogenerated charge separation, optimum operating parameters and mechanism insight. J Colloid Interface Sci 554:531–543. https://doi.org/10.1016/j.jcis.2019.07.03810.1016/j.jcis.2019.07.038 ↗
9. Zhou L, Wang W, Liu S, Zhang L, Xu H, Zhu W (2006) A sonochemical route to visible-light-driven high-activity BiVO4 photocatalyst. J Mol Catal A Chem 252:120–124. https://doi.org/10.1016/j.molcata.2006.01.05210.1016/j.molcata.2006.01.052 ↗
10. Hao C, Feng F, Wang X et al (2015) The preparation of Fe2O3 nanoparticles by liquid phase-based ultrasonic-assisted method and its application as enzyme-free sensor for the detection of H2O2. RSC Adv 5:21161–21169. https://doi.org/10.1039/c4ra17226d10.1039/c4ra17226d ↗
11. Liu S, Tang H, Zhou H, Dai G, Wang W (2017) Photocatalytic perfermance of sandwich-like BiVO4 sheets by microwave assisted synthesis. Appl Surf Sci 391:542–547. https://doi.org/10.1016/j.apsusc.2016.06.18410.1016/j.apsusc.2016.06.184 ↗
12. Ji K, Dai H, Deng J et al (2015) 3DOM BiVO4 supported silver bromide and noble metals: high-performance photocatalysts for the visible-light-driven degradation of 4-chlorophenol. Appl Catal B 168–169:274–282. https://doi.org/10.1016/j.apcatb.2014.12.04510.1016/j.apcatb.2014.12.045 ↗
13. Guo R, Yan A, Xu J et al (2020) Effects of morphology on the visible-light-driven photocatalytic and bactericidal properties of BiVO4/CdS heterojunctions: a discussion on photocatalysis mechanism. J Alloys Compd. https://doi.org/10.1016/j.jallcom.2019.15324610.1016/j.jallcom.2019.153246 ↗
14. Ma C, Lee J, Kim Y, Cheol Seo W, Jung H, Yang W (2021) Rational design of α-Fe2O3 nanocubes supported BiVO4 Z-scheme photocatalyst for photocatalytic degradation of antibiotic under visible light. J Colloid Interface Sci 581:514–522. https://doi.org/10.1016/j.jcis.2020.07.12710.1016/j.jcis.2020.07.127 ↗
15. Yamashita T, Hayes P (2008) Analysis of XPS spectra of Fe2+ and Fe3+ ions in oxide materials. Appl Surf Sci 254:2441–2449. https://doi.org/10.1016/j.apsusc.2007.09.06310.1016/j.apsusc.2007.09.063 ↗
16. Gao X, Ma C, Liu Y, Xing L, Yan Y (2019) Self-induced Fenton reaction constructed by Fe (III) grafted BiVO4 nanosheets with improved photocatalytic performance and mechanism insight. Appl Surf Sci 467–468:673–683. https://doi.org/10.1016/j.apsusc.2018.10.17210.1016/j.apsusc.2018.10.172 ↗
17. Xie T, Zhang Y, Yao W, Liu Y, Wang H, Wu Z (2019) Synthesis of Bi-deficient monolayered Bi2WO6 nanosheets with enhanced photocatalytic activity under visible light irradiation. Catal Sci Technol 9:1178–1188. https://doi.org/10.1039/c8cy02344a10.1039/c8cy02344a ↗
18. Liu N, Ouyang D, Cai Y, Li Y (2020) Heterostructured Fe2O3/BiVO4 nano-photocatalyst for the reduction of nitroarenes into amines. Ceram Int 46:24534–24543. https://doi.org/10.1016/j.ceramint.2020.06.24010.1016/j.ceramint.2020.06.240 ↗
19. Liu Y, Ge HY, Zhang XZ, Huang SF, Cheng X (2013) Surface chemical modification and characterization of nano Fe2O3. Appl Mech Mater 345:180–183. https://doi.org/10.4028/www.scientific.net/AMM.345.18010.4028/www.scientific.net/AMM.345.180 ↗
20. Gotić M, Musić S, Ivanda M, Šoufek M, Popović S (2005) Synthesis and characterisation of bismuth (III) vanadate. J Mol Struct 744–747:535–570. https://doi.org/10.1016/j.molstruc.2004.10.07510.1016/j.molstruc.2004.10.075 ↗
21. Xi J, Xia H, Ning X et al (2019) Carbon-intercalated 0D/2D hybrid of hematite quantum dots/graphitic carbon nitride nanosheets as superior catalyst for advanced oxidation. Small 15:e1902744. https://doi.org/10.1002/smll.20190274410.1002/smll.201902744 ↗
22. Xu T, Zhu R, Zhu G et al (2017) Mechanisms for the enhanced photo-Fenton activity of ferrihydrite modified with BiVO4 at neutral pH. Appl Catal B 212:50–58. https://doi.org/10.1016/j.apcatb.2017.04.06410.1016/j.apcatb.2017.04.064 ↗
23. Zhou L, Wang L, Zhang J, Lei J, Liu Y (2016) Well‐dispersed Fe2O3 nanoparticles on g‐C3N4for efficient and stable photo‐fenton photocatalysis under visible‐light irradiation. Eur J Inorg Chem 2016:5387–5392. https://doi.org/10.1002/ejic.20160095910.1002/ejic.201600959 ↗
24. Sahar S, Zeb A, Liu Y, Ullah N, Xu A (2017) Enhanced Fenton, photo-Fenton and peroxidase-like activity and stability over Fe3O4/g-C3N4 nanocomposites. Chin J Catal 38:2110–2119. https://doi.org/10.1016/s1872-2067(17)62957-710.1016/s1872-2067(17)62957-7 ↗
25. Zhao Y, Tao C, Xiao G et al (2016) Controlled synthesis and photocatalysis of sea urchin-like Fe3O4@TiO2@Ag nanocomposites. Nanoscale 8:5313–5326. https://doi.org/10.1039/c5nr08624h10.1039/c5nr08624h ↗
26. Wei B, Wang C, He Y, Ran G, Song Q (2021) A novel FeS2@g-C3N4 composite with enhanced photo-Fenton catalytic activity for pollutant degradation. Compos Commun. https://doi.org/10.1016/j.coco.2021.10065210.1016/j.coco.2021.100652 ↗
27. Wang T, Liu X, Men Q et al (2019) Photocatalytic removal using g-C3N4 quantum dots/Bi2Ti2O7 composites. Spectrochim Acta A Mol Biomol Spectrosc 213:19–27. https://doi.org/10.1016/j.saa.2019.01.05110.1016/j.saa.2019.01.051 ↗
28. Zhang M, Zhang Y, Tang L et al (2019) Ultrathin Bi2WO6 nanosheets loaded g-C3N4 quantum dots: a direct Z-scheme photocatalyst with enhanced photocatalytic activity towards degradation of organic pollutants under wide spectrum light irradiation. J Colloid Interface Sci 539:654–664. https://doi.org/10.1016/j.jcis.2018.12.11210.1016/j.jcis.2018.12.112 ↗
29. Liu L, Hu P, Cui W, Li X, Zhang Z (2017) Increased photocatalytic hydrogen evolution and stability over nano-sheet g-C3N4 hybridized CdS core@shell structure. Int J Hydrog Energy 42:17435–17445. https://doi.org/10.1016/j.ijhydene.2017.02.17110.1016/j.ijhydene.2017.02.171 ↗
30. Bornoz P, Prevot MS, Yu X, Guijarro N, Sivula K (2015) Direct light-driven water oxidation by a ladder-type conjugated polymer photoanode. J Am Chem Soc 137:15338–15341. https://doi.org/10.1021/jacs.5b0572410.1021/jacs.5b05724 ↗
31. Chakraborty A, Sarangapany S, Mishra U, Mohanty K (2021) Green synthesized magnetically separable iron oxide nanoparticles for efficient heterogeneous photo-Fenton degradation of dye pollutants. J Clust Sci 33:675. https://doi.org/10.1007/s10876-021-02010-x10.1007/s10876-021-02010-x ↗
32. Xu H, Wu L, Jin L, Wu K (2017) Synthesis of Fe2O3/TiO2 monoliths for the enhanced degradation of industrial dye and pesticide via photo-Fenton catalysis. J Mater Sci Technol 33:30–38. https://doi.org/10.1016/j.jmst.2016.04.00810.1016/j.jmst.2016.04.008 ↗
33. Singh J, Sharma S, Aanchal, Basu S (2019) Synthesis of Fe2O3/TiO2 monoliths for the enhanced degradation of industrial dye and pesticide via photo-Fenton catalysis. J Photochem Photobiol A Chem 376:32–42. https://doi.org/10.1016/j.jphotochem.2019.03.00410.1016/j.jphotochem.2019.03.004 ↗
34. Liu X, Xu J, Ni Z, Wang R, You J, Guo R (2019) Adsorption and visible-light-driven photocatalytic properties of Ag3PO4/WO3 composites: a discussion of the mechanism. Chem Eng J 356:22–33. https://doi.org/10.1016/j.cej.2018.09.00110.1016/j.cej.2018.09.001 ↗
35. Zhang K, Liu Y, Deng J et al (2017) Fe2O3/3DOM BiVO4: high-performance photocatalysts for the visible light-driven degradation of 4-nitrophenol. Appl Catal B 202:569–579. https://doi.org/10.1016/j.apcatb.2016.09.06910.1016/j.apcatb.2016.09.069 ↗