journal article·2025-11Open access

Study on micro failure mechanism of flip-chip bump interface by in-situ transmission electron microscope

Yiming Zhou, Ming Sheng, Hai Li, Sijing Chen, Tian Liu, Qiuyue Xu, Yuan Yuan, Zongguang Yu, Liyi Li, Li Zhong

Abstract

The mechanical reliability of microbumps is critical for advanced flip-chip packaging. Conventional macroscopic tests, such as bump pull and shear tests, provide overall joint reliability but cannot directly probe interfacial behavior at the nanoscale. In this work, quantitative in-situ transmission electron microscopy (TEM) mechanical tests are conducted to evaluate the intrinsic bonding and fracture behavior of heterogeneous microbump interfaces. Using microbump specimens with electroplated Ni under-bump metallization (UBM), the tensile strength of the Cu/Ni interface (∼1775 MPa) is found to be significantly higher than that of the Ni/SnAg interface (∼335 MPa). The Cu/Ni interface fails within the Cu layer, where nanotwins effectively hinder microcrack propagation. In contrast, the Ni/SnAg interface shows distinct fracture mechanisms: under tension, void growth and coalescence at the IMC/SnAg boundary lead to interface cracking, while under shear, cracks propagate along IMC grain boundaries. These findings highlight the effectiveness of the proposed in-situ TEM approach for quantitatively assessing interfacial reliability and provide guidance for minimizing void formation and strengthening IMC grain boundaries in practical microbump applications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Electronic Packaging and Soldering Technologies · 3D IC and TSV technologies · Copper Interconnects and Reliability

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (38)

Show source-provided references
1. High-performance, power-efficient three-dimensional system-in-package designs with universal chiplet interconnect express10.1038/s41928-024-01126-y ↗
2. A review on the fabrication and reliability of three-dimensional integration technologies for microelectronic packaging: through-Si-via and solder bumping process10.3390/met11101664 ↗
3. A true process-heterogeneous stacked embedded DRAM structure based on wafer-level hybrid bonding10.3390/electronics12051077 ↗
4. Research progress of hybrid bonding technology for three-dimensional integration10.1016/j.microrel.2024.115372 ↗
5. Fabrication of 30 μm Sn microbumps by electroplating and investigation of IMC characteristics on shear strength10.3390/electronics12010144 ↗
6. Research on the reliability of advanced packaging under multi-field coupling: a review10.3390/mi15040422 ↗
7. Effects of limited Cu supply on soldering reactions between SnAgCu and Ni10.1007/BF02692562 ↗
8. Brittle fracture induced by phase transformation of ni-cu-sn intermetallic compounds in Sn-3Ag-0.5 Cu/Ni solder joints under extreme temperature environment10.1016/j.jallcom.2018.10.394 ↗
9. Effect of tin grain orientation on electromigration-induced dissolution of Ni metallization in SnAg solder joints10.3390/ma15207115 ↗
10. Effects of shear test temperatures and conditions on mechanical properties of Sn–Ag flip-chip solder bumps10.1007/s10854-022-07991-7 ↗
11. Modern trends in microelectronics packaging reliability testing10.3390/mi15030398 ↗
12. Critical review of size effects on microstructure and mechanical properties of solder joints for electronic packaging10.3390/app9020227 ↗
13. Sample dimensions influence strength and crystal plasticity10.1126/science.1098993 ↗
14. A further step towards an understanding of size-dependent crystal plasticity: in situ tension experiments of miniaturized single-crystal copper samples10.1016/j.actamat.2007.10.015 ↗
15. Source truncation and exhaustion: insights from quantitative in situ TEM tensile testing10.1021/nl201890s ↗
16. Nanocrystalline copper for direct copper-to-copper bonding with improved cross-interface formation at low thermal budget10.1038/s41467-024-51510-7 ↗
17. Thermal instability of nanocrystalline Cu enables Cu-Cu direct bonding in interconnects at low temperature10.1016/j.scriptamat.2022.114900 ↗
18. Modified single cantilever adhesion test for EMC/PSR interface in thin semiconductor packages10.1016/j.microrel.2016.05.015 ↗
19. Deformation mechanisms in nanotwinned metal nanopillars10.1038/nnano.2012.116 ↗
20. Unraveling the effect of Sn crystallographic orientation on electromigration-induced intermetallic compounds formations in Cu/Ni/SnAg/Ni/Cu microbumps10.1016/j.jallcom.2025.179631 ↗
21. Effect of Ag addition on the mechanical properties of Cu/Ni/Sn/Ni/Cu microbump with a sub-10 micron bump thickness10.1007/s10854-024-13559-4 ↗
22. Thermal conductivity and nanocrystalline structure of platinum deposited by focused ion beam10.1088/0957-4484/26/8/085704 ↗
23. An investigation of slip transmission during uniaxial tensile deformation of a coarse-grained copper via EBSD characterization and crystal plasticity modelling10.1016/j.commatsci.2023.112245 ↗
24. Dislocation density distribution at slip band-grain boundary intersections10.1016/j.actamat.2019.10.031 ↗
25. Evolution and microstructural characteristics of deformation bands in fatigued copper single crystals10.1016/S1359-6454(01)00219-1 ↗
26. Nanotwinned and hierarchical nanotwinned metals: a review of experimental, computational and theoretical efforts10.1038/s41524-018-0062-2 ↗
27. Micro void growth in NiSnP layer between (Cu, Ni) 6Sn5 intermetallic compound and Ni3P by higher reflow temperature and multiple reflow10.1007/s10854-010-0072-4 ↗
28. Fracture reliability concern of (Au, Ni) Sn4 phase in 3D integrated circuit microbumps using Ni/Au surface finishing10.1016/j.scriptamat.2016.02.025 ↗
29. Tu · 2014
30. Effect of 0.5 wt% Cu in Sn− 3.5% Ag solder on the interfacial reaction with Au/Ni metallization10.1021/cm034692c ↗
31. Kirkendall void formation in eutectic SnPb solder joints on bare Cu and its effect on joint reliability10.1063/1.1839637 ↗
32. Preventing Void Growth between Ni 3 Sn 4 and solder10.1007/s11664-022-09853-8 ↗
33. Adhesive strength and tensile fracture of Ni particle enhanced Sn–Ag composite solder joints10.1016/j.msea.2005.12.021 ↗
34. TEM investigation of interfacial microstructure and fracture mode of the Sn-Ag-Cu/Ni joint system10.1016/j.msea.2017.08.116 ↗
35. Tu · 2021
36. A comparative study of microstructure and mechanical properties among Cu/Sn/Cu, Ni/Sn/Ni and Cu/Sn/Ni solder joints10.1108/09540911111099695 ↗
37. Ductile fracture by void growth to coalescence10.1016/S0065-2156(10)44003-X ↗
38. Effect of Cu content on the mechanical reliability of Ni/Sn–3.5 Ag system10.1557/jmr.2007.0085 ↗