journal article·2025-11Open access

Strongly enhanced mechanical and electromagnetic shielding properties of short carbon fiber reinforced epoxy composites by a comprehensive “absorption-transfer” interface

Jie Hu, Yihong Zhao, Nan Chen, Xuezhong Gong, Yao Wang, Jun Li, Ihor Rusetskyi, Mykhailo Danilov, Olga Grigoryeva, Alexander Fainleib, Petro Stryzhak, Jianguo Tang

Abstract

The development of short carbon fiber-reinforced polymers (SCFRPs) with high comprehensive performance is a crucial key for modern applications. However, weak interfacial adhesion between short carbon fibers (SCFs) and the epoxy matrix (EP) significantly limits stress transfer and load-bearing efficiency, resulting in suboptimal mechanical performance. In this work, a synergistic interface structure (absorption-transfer interface) has been generated by combining a cut carbon nanotube (CCNTs) and self-polymerized dopamine (PDA) to efficiently absorb and transfer external loads as well as enhance electromagnetic waves loss. The incorporation of CCNTs-PDA into the silane-modified SCFs-EP (SCFs-Si-EP) results in remarkable enhancements in flexural strengths, which increase by 208%, compared with those of SCFs-Si-EP. The dominant failure mechanism changes from fiber pull-out to delamination failure after introduction of the CCNTs-PDA interface. Moreover, the SCFs-Si-EP composites exhibit an EMI shielding effectiveness of 47.3 dB with incorporation of CCNTs and 2 wt% PDA (SCFs-CP-EP-2). This enhancement is attributed to the conductive networks and scattering centers provided by the CCNTs-PDA interface layer, which facilitates interfacial polarization and optimizes impedance matching, thereby leading to efficient electromagnetic wave attenuation. As a result, the SCFs-CP-EP-2 shows excellent mechanical properties and admirable electromagnetic shielding performance.
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Research context

OpenAlex topics: Electromagnetic wave absorption materials · Smart Materials for Construction · Fiber-reinforced polymer composites

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