journal article·2024-07-28

Oxygen doping and interface engineering in O-MoS2&rGO heterostructure for efficient piezocatalytic dye degradation

Zhichao Lu, Yuanjuan Bai, Shuaijie Zhang, Yaxuan Li, Mingxuan Liu, Ling Fang, Li Liu, Kun Du, Gonggang Liu, Laiqiang Xu, Yuanyuan Liao, Shanshan Chang, Jinbo Hu

Journal of Materials Research· Volume 39· Issue 14
Publisher page

Abstract

To further apply MoS2as a promising non-noble catalyst for addressing environmental issues, its catalytic ability must be improved. As a result of the hetero-atom doping effect and varied structure phase of MoS2, we demonstrated excellent piezocatalysis for the degradation of methylene blue (MB) dye under stirring/ultrasonic catalyzed by MoS2. Compared with pristine MoS2and O-doping MoS2(O-MoS2), O-MoS2& reduced graphene oxide (O-MoS2&rGO) exhibits enhanced piezocatalytic activity. When the initial concentration of MB solution is ≤ 15 mg L−1, both stirring and ultrasonication can make the optimal O-MoS2&rGO composite to degrade the dye completely within 20 min. The experimental results have led to the proposal of a mechanism that elucidates the enhancement effect of rGO and O doping on the piezocatalytic performance of MoS2. This study highlights the significance of constructing heterostructure interfaces and the impact of hetero-atom doping on the promotion of piezocatalysis efficiency.Graphical abstractBoosting the catalytic ability of MoS2is vital to its further application as a class of promising non-noble catalysts to address environmental issues. Benefiting from the O-doping-induced electronic effect and interfacial coupling and synergistic effect between MoS2and reduced graphene oxide (rGO), the as-prepared O-MoS2&rGO heterogeneous catalyst exhibits enhanced degradation efficiency for methylene blue (MB) dye.
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Research context

OpenAlex topics: Advanced Photocatalysis Techniques · Gas Sensing Nanomaterials and Sensors · Advanced Memory and Neural Computing

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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