journal article·2021-03-14

Thermally stable dielectric properties of 0.5Na0.5Bi0.5TiO3–0.4SrTiO3–0.1BiFeO3 ceramics at high temperature

Xi Wu, Hongbo Liu, Jianguo Chen

Journal of Materials Research· Volume 36· Issue 5
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Abstract

Na0.5Bi0.5TiO3‐based ceramics have been paid great attention as Pb‐free piezoelectric and electrical energy storage materials. Here, adding 10 mol% BiFeO3 in Na0.5Bi0.5TiO3–SrTiO3 binary system, 0.5Na0.5Bi0.5TiO3–0.4SrTiO3–0.1BiFeO3 ceramics were prepared by a conventional solid‐state reaction method. Dielectric measurements reflected a near‐plateau dielectric response at high temperature, e.g., the mid‐dielectric permittivity of 2052 with the variation within ±10% from 57 to 371 °C and within ±15% from 54 to 371 °C for the ceramic sintered at 1100 °C. At a moderate electric field of 70 kV/cm, a capacitor made by the ceramic has an electrical energy storage density of 0.95 J/cm3, while the polarization has yet saturated at the moderate electric field. These results suggest that 0.5Na0.5Bi0.5TiO3–0.4SrTiO3–0.1BiFeO3 ceramic is a promising novel material with thermally stable dielectric permittivity and high electrical energy storage property for applications in high‐temperature electronics.
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Research context

OpenAlex topics: Ferroelectric and Piezoelectric Materials · Multiferroics and related materials · Dielectric properties of ceramics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (45)

Show source-provided references
1. H. Liu and B. Dkhil: Effect of resistivity ratio on energy storage and dielectric relaxation properties of 0‐3 dielectric composites. J. Mater. Sci. 52, 6074 (2017).10.1007/s10853-017-0846-7 ↗
2. J. Watson and G. Castro: A review of high‐temperature electronics technology and applications. J. Mater. Sci.: Mater. Electron. 26, 9226 (2015).
3. J. Bultitude, J. McConnell, and C. Shearer: High temperature capacitors and transient liquid phase interconnects for Pb‐solder replacement. J. Mater. Sci.: Mater. Electron. 26, 9236 (2015).
4. A. Zeb and S.J. Milne: High temperature dielectric ceramics: a review of temperature‐stable high‐permittivity perovskites. J. Mater. Sci.: Mater. Electron. 26, 9243 (2015).
5. J. Hao, W. Li, J. Zhai, and H. Chen: Progress in high‐strain perovskite piezoelectric ceramics. Mater. Sci. Eng., R 135, 1 (2019).10.1016/j.mser.2018.08.001 ↗
6. G. Liu, Z. Wang, L. Zhang, W. Shi, J. Jing, Y. Chen, H. Liu, and Y. Yan: Phase segregation and dielectric, ferroelectric, and piezoelectric properties of MgO‐doped NBT‐BT lead‐free ferroelecric ceramics. Mater. Res. Express 5, 036305 (2018).10.1088/2053-1591/aab33b ↗
7. L. Yang, X. Kong, F. Li, H. Hao, Z. Cheng, H. Liu, J.‐F. Li, and S. Zhang: Perovskite lead‐free dielectrics for energy storage applications. Prog. Mater. Sci. 102, 72 (2019).10.1016/j.pmatsci.2018.12.005 ↗
8. P. Chen, L. Zhang, J. Cai, Z. Wang, W. Shi, J. Jing, F. Wei, G. Liu, Y. Yan, H. Liu, and L. Jin: Effect of Dy2O3 content on the dielectric, ferroelectric, and energy storage properties of lead‐free 0.5Na0.5Bi0.5TiO3‐0.5SrTiO3 bulk ceramics. J. Mater. Sci.: Mater. Electron. 30, 13556 (2019).
9. R. Dittmer, E.‐M. Anton, W. Jo, H. Simons, J.E. Daniels, M. Hoffman, J. Pokorny, I.M. Reaney, and J. Rödel: A high‐temperature‐capacitor dielectric based on K0.5Na0.5NbO3‐modified Bi1/2Na1/2TiO3‐Bi1/2K1/2TiO3. J. Am. Ceram. Soc. 95, 3519 (2012).10.1111/j.1551-2916.2012.05321.x ↗
10. A. Zeb, S. ullah Jan, F. Bamiduro, D.A. Hall, and S.J. Milne: Temperature‐stable dielectric ceramics based on Na0.5Bi0.5TiO3. J. Eur. Ceram. Soc. 38, 1548 (2018).10.1016/j.jeurceramsoc.2017.12.032 ↗
11. F. Han, J. Deng, X. Liu, T. Yan, S. Ren, X. Ma, S. Liu, B. Peng, and L. Liu: High‐temperature dielectric and relaxation behavior of Yb‐doped Bi0.5Na0.5TiO3 ceramics. Ceram. Int. 43, 5564 (2017).10.1016/j.ceramint.2017.01.086 ↗
12. J. Shi, H. Fan, X. Liu, Y. Ma, and Q. Li: Bi deficiencies induced high permittivity in lead‐free BNBT‐BST high‐temperature dielectrics. J. Alloys Compd. 627, 463 (2015).10.1016/j.jallcom.2014.12.022 ↗
13. D. Rout, K.‐S. Moon, S.‐J.L. Kang, and I.W. Kim: Dielectric and Raman scattering studies of phase transitions in the (100‐x) Na0.5Bi0.5TiO3‐xSrTiO3 system. J. Appl. Phys. 108, 084102 (2010).10.1063/1.3490781 ↗
14. H. He, X. Lu, M. Li, Y. Wang, Z. Li, Z. Lu, and L. Lu: Thermal and compositional driven relaxor ferroelectric behaviours of lead‐free Bi0.5Na0.5TiO3‐SrTiO3 ceramics. J. Mater. Chem. C 8, 2411 (2020).10.1039/C9TC04864B ↗
15. Y. Hiruma, Y. Imai, Y. Watanabe, H. Nagata, and T. Takenaka: Large electrostrain near the phase transition temperature of (Bi0.5Na0.5) TiO3‐SrTiO3 ferroelectric ceramics. Appl. Phys. Lett. 92, 262904 (2008).10.1063/1.2955533 ↗
16. Y. Zhu, Y. Zhang, B. Xie, P. Fan, M.A. Marwat, W. Ma, C. Wang, B. Yang, J. Xiao, and H. Zhang: Large electric field‐induced strain in AgNbO3‐modified 0.76Bi0.5Na0.5TiO3‐0.24SrTiO3 lead‐free piezoceramics. Ceram. Int. 44, 7851 (2018).10.1016/j.ceramint.2018.01.220 ↗
17. F. Yan, H. Yang, Y. Lin, and T. Wang: Dielectric and ferroelectric properties of SrTiO3‐Bi0.5Na0.5TiO3‐BaAl0.5Nb0.5O3 lead‐free ceramics for high‐energy‐storage applications. Inorg. Chem. 56, 13510 (2017).10.1021/acs.inorgchem.7b02181 ↗
18. C. Cui, Y. Pu, Z. Gao, J. Wan, Y. Guo, C. Hui, Y. Wang, and Y. Cui: Structure, dielectric and relaxor properties in lead‐free ST‐NBT ceramics for high energy storage applications. J. Alloys Compd. 711, 319 (2017).10.1016/j.jallcom.2017.04.023 ↗
19. C. Ang and Z. Yu: High, purely electrostrictive strain in lead‐free dielectrics. Adv. Mater. 18, 103 (2006).10.1002/adma.200500951 ↗
20. J. Li, F. Li, Z. Xu, and S. Zhang: Multilayer lead‐free ceramic capacitors with ultrahigh energy density and efficiency. Adv. Mater. 30, 1802155 (2018).10.1002/adma.201802155 ↗
21. H. Pan, F. Li, Y. Liu, Q. Zhang, M. Wang, S. Lan, Y. Zheng, J. Ma, L. Gu, Y. Shen, P. Yu, S. Zhang, L.‐Q. Chen, Y.‐H. Lin, and C.‐W. Nan: Ultrahigh‐energy density lead‐free dielectric films via polymorphic nanodomain design. Science 365, 578 (2019).10.1126/science.aaw8109 ↗
22. H. Liu: High dielectric permittivity of BiFeO3‐SrTiO3‐CaTiO3 ternary solid solution ceramics. Ceram. Int. 46, 8255 (2020).10.1016/j.ceramint.2019.12.053 ↗
23. G. Liu, W. Jiang, L. Zhang, J. Cai, Z. Wang, K. Liu, X. Liu, Y. Chen, H. Liu, and Y. Yan: Effects of sintering temperature and KBT content on microstructure and electrical properties of (Bi0.5Na0.5) TiO3‐BaTiO3‐(Bi0.5K0.5) TiO3 Pb‐free ceramics. Ceram. Int. 44, 9303 (2018).10.1016/j.ceramint.2018.02.142 ↗
24. E. Aksel, E. Erdem, P. Jakes, J.L. Jones, and R.‐A. Eichel: Defect structure and materials “hardening” in Fe2O3‐doped [Bi0.5Na0.5] TiO3 ferroelectrics. Appl. Phys. Lett. 97, 012903 (2010).10.1063/1.3455888 ↗
25. J.‐H. Cho, J.‐S. Park, S.‐W. Kim, Y.‐H. Jeong, J.‐S. Yun, W.‐I. Park, Y.‐W. Hong, and J.‐H. Paik: Ferroelectric properties and core shell domain structures of Fe‐modified 0.77Bi0.5Na0.5TiO3‐0.23SrTiO3 ceramics. J. Eur. Ceram. Soc. 37, 3313 (2017).10.1016/j.jeurceramsoc.2017.03.070 ↗
26. W. Krauss, D. Schütz, F.A. Mautner, A. Feteira, and K. Reichmann: Piezoelectric properties and phase transition temperatures of the solid solution of (1‐x) (Bi0.5Na0.5) TiO3‐xSrTiO3. J. Eur. Ceram. Soc. 30, 1827 (2010).10.1016/j.jeurceramsoc.2010.02.001 ↗
27. V. Dorcet, P. Marchet, and G. Trolliard: Structural and dielectric studies of the Na0.5Bi0.5TiO3‐BiFeO3 system. J. Eur. Ceram. Soc. 27, 4371 (2007).10.1016/j.jeurceramsoc.2007.02.173 ↗
28. H. Liu and X. Yang: Structural, dielectric, and magnetic properties of BiFeO3‐SrTiO3 solid solution ceramics. Ferroelectrics 500, 310 (2016).10.1080/00150193.2016.1230445 ↗
29. L. Li, H. Liu, G. Wen, and G. Liu: Structural evolution and dielectric response of (1‐x) BiFeO3‐xSrTiO3 ceramics. Ceram. Int. 44, S69 (2018).10.1016/j.ceramint.2018.08.238 ↗
30. J. Chen, J. Cheng, J. Guo, Z. Cheng, J. Wang, H. Liu, and S. Zhang: Excellent thermal stability and aging behaviors in BiFeO3‐BaTiO3 piezoelectric ceramics with rhombohedral phase. J. Am. Ceram. Soc. 103, 374 (2020).10.1111/jace.16755 ↗
31. H. Liu and X. Yang: A brief review on perovskite multiferroics. Ferroelectrics 507, 69 (2017).10.1080/00150193.2017.1283171 ↗
32. L. Liu, D. Shi, M. Knapp, H. Ehrenberg, L. Fang, and J. Chen: Large strain response based on relaxor‐antiferroelectric coherence in Bi0.5Na0.5TiO3‐SrTiO3‐(K0.5Na0.5) NbO3 solid solutions. J. Appl. Phys. 116, 184104 (2014).10.1063/1.4901549 ↗
33. L. Liu, M. Knapp, H. Ehrenberg, L. Fang, L.A. Schmitt, H. Fuess, M. Hoelzel, and M. Hinterstein: The phase diagram of K0.5Na0.5NbO3‐Bi1/2Na1/3. J. Appl. Crystallogr. 49, 574 (2016).10.1107/S1600576716002909 ↗
34. L. Liu, M. Knapp, H. Ehrenberg, L. Fang, H. Fan, L.A. Schmitt, H. Fuess, M. Hoelzel, H. Dammak, M.P. Thi, and M. Hinterstein: Average vs. local structure and composition‐property phase diagram of K0.5Na0.5NbO3‐Bi½Na½TiO3 system. J. Eur. Ceram. Soc. 37, 1387 (2017).10.1016/j.jeurceramsoc.2016.11.024 ↗
35. O. Bidault, P. Goux, M. Kchikech, M. Belkaoumi, and M. Maglione: Space‐charge relaxation in perovskites. Phys. Rev. B 49, 7868 (1994).10.1103/PhysRevB.49.7868 ↗
36. L. Liu, Y. Huang, C. Su, L. Fang, M. Wu, C. Hu, and H. Fan: Space‐charge relaxation and electrical conduction in K0.5Na0.5NbO3 at high temperatures. Appl. Phys. A 104, 1047 (2011).10.1007/s00339-011-6358-4 ↗
37. X. He, S. Zhou, Z. Yuan, Y. Li, Z. Lan, K. Chen, F. Han, X. Lei, and L. Liu: The origin of weak coupling between polar clusters in Ta2O5‐doped 0.94Bi0.5Na0.5TiO3‐0.06BaTiO3. EPL Europhys. Lett. 129, 37004 (2020).10.1209/0295-5075/129/37004 ↗
38. J. Chen, J.E. Daniels, J. Jian, Z. Cheng, J. Cheng, J. Wang, Q. Gu, and S. Zhang: Origin of large electric‐field‐induced strain in pseudo‐cubic BiFeO3‐BaTiO3 ceramics. Acta Mater. 197, 1 (2020).10.1016/j.actamat.2020.07.032 ↗
39. J. Wu, H. Zhang, C.‐H. Huang, C.‐W. Tseng, N. Meng, V. Koval, Y.‐C. Chou, Z. Zhang, and H. Yan: Ultrahigh field‐induced strain in lead‐free ceramics. Nano Energy 76, 105037 (2020).10.1016/j.nanoen.2020.105037 ↗
40. R. Dittmer, W. Jo, D. Damjanovic, and J. Rödel: Lead‐free high‐temperature dielectrics with wide operational range. J. Appl. Phys. 109, 034107 (2011).10.1063/1.3544481 ↗
41. R. Shannon: Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides. Acta Crystallogr. Sect. A 32, 751 (1976).10.1107/S0567739476001551 ↗
42. R.D. Shannon and R.X. Fischer: Empirical electronic polarizabilities in oxides, hydroxides, oxyfluorides, and oxychlorides. Phys Rev B 73, 235111 (2006).10.1103/PhysRevB.73.235111 ↗
43. H. Liu: Universal dielectric relaxation induced giant dielectric permittivity in Mn‐doped PbZrO3 ceramics. Ceram. Int. 45, 10380 (2019).10.1016/j.ceramint.2019.02.096 ↗
44. Z. Xie and H. Liu: A novel method of preparing antiferroelectric silver niobate AgNbO3 ceramics. Ceram. Int. 46, 6955 (2020).10.1016/j.ceramint.2019.11.070 ↗
45. H. Liu: Effect of an electric field on the electrocaloric response of ferroelectrics. Chin. Phys. B 27, 127701 (2018).10.1088/1674-1056/27/12/127701 ↗