journal article·2014-02-14

Field emission from laser cut CNT fibers and films

Steven B. Fairchild, John S. Bulmer, Martin Sparkes, John Boeckl, Marc Cahay, Tyson Back, P. Terrence Murray, Gregg Gruen, Matthew Lange, Nathaniel P. Lockwood, Francisco Orozco, William O’Neill, Catharina Paukner, Krzysztof K. K. Koziol

Journal of Materials Research· Volume 29· Issue 3
Publisher page

Abstract

Field emission (FE) measurements are reported from carbon nanotube (CNT) fibers and laser-patterned free standing films fabricated by direct online condensation from a floating catalyst chemical vapor deposition reactor. Fiber and film cathodes showed stable emission in the 1–2 mA current (I) range at maximum cathode temperatures less than 1000 °C; film cathodes show localized heating at the triangular tips and higher maximum temperatures than the fibers. Fowler-Nordheim (FN) analysis indicated a change in the morphology of the emitters with increasing external electrical field (Eext). Fiber cathodeI-Eextdata are interpreted as FN emission from the fiber tip which is eventually limited by space-charge effects. At higherEext, FN emission from the fiber sidewall occurs. The single fiber cathode stopped emitting abruptly when field induced self-heating effects became significant. For CNT films, self-heating effects can destroy a portion of the film, but FE can still occur from other areas.
Source: expertdata · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Laser Material Processing Techniques · Diamond and Carbon-based Materials Research · Carbon Nanotubes in Composites

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (36)

Show source-provided references
1. 10.1088/0957-4484/19/41/41570310.1088/0957-4484/19/41/415703 ↗
2. 10.1063/1.12203710.1063/1.122037 ↗
3. 10.1016/j.carbon.2012.09.03710.1016/j.carbon.2012.09.037 ↗
4. 10.1063/1.327705410.1063/1.3277054 ↗
5. 10.1063/1.479087410.1063/1.4790874 ↗
6. 10.1116/1.356542810.1116/1.3565428 ↗
7. 10.1007/s00339-007-4009-610.1007/s00339-007-4009-6 ↗
8. 10.1088/0957-4484/20/31/31520110.1088/0957-4484/20/31/315201 ↗
9. 10.1126/science.109498210.1126/science.1094982 ↗
10. 10.1103/PhysRev.21.41910.1103/PhysRev.21.419 ↗
11. 10.1063/1.12625810.1063/1.126258 ↗
12. 10.1103/PhysRevLett.81.144110.1103/PhysRevLett.81.1441 ↗
13. 10.1063/1.12514510.1063/1.125145 ↗
14. 33. Cahay M.M. , Murray P.T. , Back T.C. , Gruen G.J. , Fairchild S.B. , Boeckl J. , Bulmer J. , and Koziol K.K. : Hysteresis during field emission from carbon nanotube fibers synthesized by chemical vapor deposition. Nano Lett. (2013, submitted).
15. 10.1103/PhysRevSeriesI.32.49210.1103/PhysRevSeriesI.32.492 ↗
16. 10.1021/nn201149y10.1021/nn201149y ↗
17. 10.1116/1.59085610.1116/1.590856 ↗
18. 10.1116/1.234872910.1116/1.2348729 ↗
19. 10.1063/1.481751610.1063/1.4817516 ↗
20. Carbon nanotube bundle array cold cathodes for THz vacuum tube sources
21. 10.1116/1.216122310.1116/1.2161223 ↗
22. 10.1016/j.carbon.2012.04.03310.1016/j.carbon.2012.04.033 ↗
23. 10.1021/nl300379210.1021/nl3003792 ↗
24. 22. Fairchild S.B. , Back T.C. , Ferguson J.B. , Boeckl J. , Koemer H. , Maruyama B. , Lange M. , Lockwood N.P. , Cahay M.M. , Behabtu N. , Young C.C. , Averett K. , Murray P.T. , and Pasquali M. : Morphology dependent field emission of carbon nanotube fibers. Adv. Funct. Mater. (2013, submitted).
25. 10.1063/1.223646510.1063/1.2236465 ↗
26. 10.1021/nn101956w10.1021/nn101956w ↗
27. 10.1116/1.352310110.1116/1.3523101 ↗
28. Manohara · 2010 · 7594
29. 10.1007/s00339-012-7376-610.1007/s00339-012-7376-6 ↗
30. 14. Paukner C. and Koziol K.K. : Ultra-pure single wall carbon nanotube fibers continuously spun without promoter. Nature Sci. Rep. (2013, submitted).10.1038/srep03903 ↗
31. 10.1021/nn300111t10.1021/nn300111t ↗
32. 10.1016/S0304-3991(97)00129-010.1016/S0304-3991(97)00129-0 ↗
33. 10.1063/1.349065110.1063/1.3490651 ↗
34. 10.1088/0957-4484/20/32/32570710.1088/0957-4484/20/32/325707 ↗
35. 10.1109/TPS.2012.219532810.1109/TPS.2012.2195328 ↗
36. 10.1126/science.122806110.1126/science.1228061 ↗