journal article·2022-10-14

Understanding electro-mechanical-thermal coupling in solid-state lithium metal batteries via phase-field modeling

Zhe-Tao Sun, Shou-Hang Bo

Journal of Materials Research· Volume 37· Issue 19
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Abstract

AbstractSolid-state batteries, based on a solid electrolyte and an energy-dense metal anode, are considered promising next-generation energy-storage devices. Phase-filed method, as a mesoscale method, covers a much wider range of length scales, from the atomic to the continuum scale, compared with those of first principles and finite-element methods. However, phase-field modeling strategies of conventional lithium-ion batteries cannot be directly applied to solid-state systems with strong coupling between different physical fields. A timely review on phase-field modeling of solid-state batteries that discusses the principles, strengths, and limitations of such a simulation method is therefore critical. This review will provide a brief introduction for electrochemists who are new to the phase-field method as well as simulation scientists who are new to solid-state batteries. We hope that this review will motivate further studies in multiphysics coupling effects, e.g., chemo-mechanical, and chemo-thermal, which is critical to fully unlocking the potential of solid-state batteries.Graphical abstract
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Research context

OpenAlex topics: Advancements in Battery Materials · Advanced Battery Materials and Technologies · Advanced Battery Technologies Research

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