Structural, magnetocaloric effect, critical behavior, and spin resonance analysis of monovalent-doped manganites Nd0.6Sr0.4−xMxMnO3 (x = 0.0, 0.1; M = K, Na)
Source abstract
Abstract
In-depth research of the effects of monovalent doping on magnetocaloric properties of manganites Nd0.6Sr0.4−xMxMnO3 (x= 0.0, 0.1; M = K, Na) synthesized by sol–gel were studied. The magnetization-versus-temperature curves reveal a second-order phase transition from ferromagnetic to paramagnetic at the Curie temperature. The Curie temperature is found to decrease from 276 K in the Nd0.6Sr0.4MnO3to 250 K and 248 K in Nd0.6Sr0.3K0.1MnO3and Nd0.6Sr0.3Na0.1MnO3, respectively. The Nd0.6Sr0.3K0.1MnO3has the highest isothermal magnetic entropy change (5.45 J/kg.K), whereas Nd0.6Sr0.3Na0.1MnO3has the highest relative cooling power (144.41 J/Kg), which denotes its potentiality in cooling fields. The charge difference of Sr, K, and Na influence the ratio of Mn4+/Mn3+, causing significant fluctuations in Nd0.6Sr0.4MnO3manganite.Various approaches are used to derive the critical exponents, and they are shown to be consistent with the values predicted by the tricritical mean field. This work highlights that monovalent ions doped are promising for magnetic refrigeration near room temperature.Graphical abstract
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Research context
OpenAlex topics: Magnetic and transport properties of perovskites and related materials · Multiferroics and related materials · Advanced Condensed Matter Physics
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
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