Graphene Oxide as a Corrosion Inhibitor for Steel Reinforcement in Cement Extract Containing Chlorides
Source abstract
Abstract
This work aims at evaluating the potentiality of using graphene oxide modified with polycarboxylate-based superplasticizer as a corrosion inhibitor additive for reinforcement steel, by incorporating 0.002 and 0.05 wt.% of graphene oxide (GO) in the cement extract. Electrochemical impedance spectroscopy, linear polarization resistance, and X-ray photoelectron spectroscopy were used to investigate the inhibitive effect of GO against steel corrosion. The results indicated that the ratio of 1:8 of GO: polycarboxylate achieved the best level of GO dispersion in the cement extract. Besides, the amount of 0.002 wt.% GO gave the most promising results toward the corrosion inhibiting effect for steel in the studied environment.
Source: expertdata · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Corrosion Behavior and Inhibition · Concrete Corrosion and Durability · Smart Materials for Construction
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (54)
Show source-provided references
1. Z. Zhang, H. Ba, and Z. Wu, Sustainable Corrosion Inhibitor for Steel in Simulated Concrete Pore Solution by Maize Gluten Meal Extract: Electrochemical and Adsorption Behavior Studies, Constr. Build. Mater., 2019 https://doi.org/10.1016/j.conbuildmat.2019.11708010.1016/j.conbuildmat.2019.117080 ↗
2. D.A. Koleva, An Innovative Approach to Control Steel Reinforcement Corrosion by Self-Healing, Mater., 2018, 11, p 309. https://doi.org/10.3390/ma1102030910.3390/ma11020309 ↗
3. S. Chuah, W. Li, S.J. Chen, J.G. Sanjayan, and W.H. Duan, Investigation on Dispersion of Graphene Oxide in Cement Composite using Different Surfactant Treatments, Constr. Build. Mater., 2018, 161, p 519–527. https://doi.org/10.1016/j.conbuildmat.2017.11.15410.1016/j.conbuildmat.2017.11.154 ↗
4. M.A. Asaad, M. Ismail, M.M. Tahir, G.F. Huseien, P.B. Raja, and Y.P. Asmara, Enhanced Corrosion Resistance of Reinforced Concrete: Role of Emerging Eco-friendly Elaeis Guineensis/Silver Nanoparticles Inhibitor, Constr. Build. Mater., 2018, 188, p 555–568. https://doi.org/10.1016/j.conbuildmat.2018.08.14010.1016/j.conbuildmat.2018.08.140 ↗
5. Y. Liu, Z. Song, W. Wang, L. Jiang, Y. Zhang, M. Guo, F. Song, and N. Xu, Effect of Ginger Extract as Green Inhibitor on Chloride-Induced Corrosion of Carbon Steel in Simulated Concrete Pore Solutions, J. Clean. Prod., 2019, 214, p 298–307. https://doi.org/10.1016/j.jclepro.2018.12.29910.1016/j.jclepro.2018.12.299 ↗
6. D. Dimov, I. Amit, O. Gorrie, M.D. Barnes, N.J. Townsend, A.I.S. Neves, F. Withers, S. Russo, and M.F. Craciun, Ultrahigh Performance Nanoengineered Graphene-Concrete Composites for Multifunctional Applications, Adv. Funct. Mater., 2018, 28, p 1705183. https://doi.org/10.1002/adfm.20170518310.1002/adfm.201705183 ↗
7. S.C. Paul, A.S. van Rooyen, G.P.A.G. van Zijl, and L.F. Petrik, Properties of Cement-Based Composites using Nanoparticles: A Comprehensive Review, Constr. Build. Mater., 2018, 189, p 1019–1034. https://doi.org/10.1016/j.conbuildmat.2018.09.06210.1016/j.conbuildmat.2018.09.062 ↗
8. L. Zhao, X. Guo, L. Song, Y. Song, G. Dai, and J. Liu, An Intensive Review on the Role of Graphene Oxide in Cement-Based Materials, Constr. Build. Mater., 2020, 241, p 117939. https://doi.org/10.1016/j.conbuildmat.2019.11793910.1016/j.conbuildmat.2019.117939 ↗
9. S. Chuah, Z. Pan, J.G. Sanjayan, C.M. Wang, and W.H. Duan, Nano Reinforced Cement and Concrete Composites and New Perspective from Graphene Oxide, Constr. Build. Mater., 2014, 73, p 113–124. https://doi.org/10.1016/j.conbuildmat.2014.09.04010.1016/j.conbuildmat.2014.09.040 ↗
10. L. Zhao, X. Guo, Y. Liu, C. Ge, Z. Chen, L. Guo, X. Shu, and J. Liu, Investigation of Dispersion Behavior of GO Modified by Different Water Reducing Agents in Cement Pore Solution, Carbon N Y., 2018, 127, p 255–269. https://doi.org/10.1016/j.carbon.2017.11.01610.1016/j.carbon.2017.11.016 ↗
11. A. Mohammed, J.G. Sanjayan, W.H. Duan, and A. Nazari, Incorporating Graphene Oxide in Cement Composites: A Study of Transport Properties, Constr. Build. Mater., 2015, 84, p 341–347. https://doi.org/10.1016/j.conbuildmat.2015.01.08310.1016/j.conbuildmat.2015.01.083 ↗
12. K. Chintalapudi and R.M.R. Pannem, An Intense Review on the Performance of Graphene Oxide and Reduced Graphene Oxide in an Admixed Cement System, Constr. Build. Mater., 2020, 259, p 120598. https://doi.org/10.1016/j.conbuildmat.2020.12059810.1016/j.conbuildmat.2020.120598 ↗
13. C. Liu, X. Huang, Y.Y. Wu, X. Deng, and Z. Zheng, The Effect of Graphene Oxide on the Mechanical Properties, Impermeability and Corrosion Resistance of Cement Mortar Containing Mineral Admixtures, Constr. Build. Mater., 2021, 288, p 123059. https://doi.org/10.1016/j.conbuildmat.2021.12305910.1016/j.conbuildmat.2021.123059 ↗
14. I. Papanikolaou, L. Ribeiro de Souza, C. Litina, and A. Al-Tabbaa, Investigation of the Dispersion of Multi-layer Graphene Nanoplatelets in Cement Composites using Different Superplasticiser Treatments, Constr. Build. Mater., 2021, 293, p 123543. https://doi.org/10.1016/j.conbuildmat.2021.12354310.1016/j.conbuildmat.2021.123543 ↗
15. M.D.C. Camacho, O. Galao, F.J. Baeza, E. Zornoza, and P. Garcés, Mechanical Properties and Durability of CNT Cement Composites, Materials, 2014, 7, p 1640–1651. https://doi.org/10.3390/ma703164010.3390/ma7031640 ↗
16. X. Li, A.H. Korayem, C. Li, Y. Liu, H. He, J.G. Sanjayan, and W.H. Duan, Incorporation of Graphene Oxide and Silica Fume into Cement Paste: A Study of Dispersion and Compressive Strength, Constr. Build. Mater., 2016, 123, p 327–335. https://doi.org/10.1016/j.conbuildmat.2016.07.02210.1016/j.conbuildmat.2016.07.022 ↗
17. W.J. Long, C. Fang, J. Wei, and H. Li, Stability of GO Modified by Different Dispersants in Cement Paste and its Related Mechanism, Materials (Basel), 2018, 11, p 834. https://doi.org/10.3390/ma1105083410.3390/ma11050834 ↗
18. T.S. Qureshi, D.K. Panesar, B. Sidhureddy, A. Chen, and P.C. Wood, Nano-cement Composite with Graphene Oxide Produced from Epigenetic Graphite Deposit, Compos. Part B: Eng., 2019, 159, p 248–258. https://doi.org/10.1016/j.compositesb.2018.09.09510.1016/j.compositesb.2018.09.095 ↗
19. X. Feng, R. Shi, X. Lu, Y. Xu, X. Huang, and D. Chen, The Corrosion Inhibition Efficiency of Aluminum Tripolyphosphate on Carbon Steel in Carbonated Concrete Pore Solution, Corr. Sci., 2017, 124, p 150–159. https://doi.org/10.1016/j.corsci.2017.05.01810.1016/j.corsci.2017.05.018 ↗
20. Z. Lu, A. Hanif, C. Ning, H. Shao, R. Yin, and Z. Li, Steric Stabilization of Graphene Oxide in Alkaline Cementitious Solutions: Mechanical Enhancement of Cement Composite, Mater. Des., 2017, 127, p 154–161. https://doi.org/10.1016/j.matdes.2017.04.08310.1016/j.matdes.2017.04.083 ↗
21. G. Pavoski, T.G. Maraschin, F.C. Fim, N.M. Balzaretti, G.L.B. Galland, C.S. Moura, and N.R.S. Basso, Few Layer Reduced Graphene Oxide: Evaluation of the Best Experimental Conditions for Easy Production, Mater. Res. Ibero-am. J. Mater., 2016, 20, p 53–61. https://doi.org/10.1590/1980-5373-MR-2015-052810.1590/1980-5373-MR-2015-0528 ↗
22. S. Sun and P. Wu, A One-step Strategy for Thermal- and pH-Responsive Graphene Oxide Interpenetrating Polymer Hydrogel Networks, J. Mater. Chem., 2011, 21, p 4095–4097. https://doi.org/10.1039/C1JM10276A10.1039/C1JM10276A ↗
23. D.R. Dreyer, S. Park, C.W. Bielawski, and R.S. Ruoff, The Chemistry of Graphene Oxide, Chem. Soc. Rev., 2010, 39, p 228–240. https://doi.org/10.1039/B917103G10.1039/B917103G ↗
24. M. Corso, L.K. Berto, A.C.D. Albuquerque, J.H. Oliveira, S.L. Favaro, and L.C.S.H. Rezende, Incorporação de Óxido de Grafeno em Argamassa de Revestimento: Uma Visão Sustentável (Incorporation of Graphene Oxide in Coating Mortar: A Sustainable Vision), Ambiente Construído, 2020, 20, p 297–312. (in portuguese)10.1590/s1678-86212020000100375 ↗
25. Q. Lai, S. Zhu, X. Luo, M. Zou, and S. Huang, Ultraviolet-visible Spectroscopy of Graphene Oxides, AIP Adv., 2012, 2, p 032146. https://doi.org/10.1063/1.474781710.1063/1.4747817 ↗
26. D. Wang, J. Ming, and J. Shi, Enhanced Corrosion Resistance of Rebar in Carbonated Concrete Pore Solutions by Na2HPO4 and Benzotriazole, Corr. Sci., 2020, 174, p 108830. https://doi.org/10.1016/j.corsci.2020.10883010.1016/j.corsci.2020.108830 ↗
27. X. Zhou, H. Yang, and F. Wang, Investigation on the Inhibition Behavior of a Pentaerythritol Glycoside for Carbon Steel in 3.5% NaCl Saturated Ca(OH)2 Solution, Corr. Sci., 2012, 54, p 193–200. https://doi.org/10.1016/j.corsci.2011.09.01810.1016/j.corsci.2011.09.018 ↗
28. F. Zhi, L. Jiang, M. Jin, P. Xu, B. Xiao, Q. Jiang, L. Chen, and Y. Gu, Inhibition Effect and Mechanism of Polyacrylamide for Steel Corrosion in Simulated Concrete Pore Solution, Constr. Build. Mater., 2020, 259, p 120425. https://doi.org/10.1016/j.conbuildmat.2020.12042510.1016/j.conbuildmat.2020.120425 ↗
29. Y. Tian, C. Dong, G. Wang, X. Cheng, and X. Li, The Effect of Nickel on Corrosion Behaviour of High-strength Low Alloy Steel Rebar in Simulated Concrete Pore Solution, Constr. Build. Mater., 2020, 246, p 118462. https://doi.org/10.1016/j.conbuildmat.2020.11846210.1016/j.conbuildmat.2020.118462 ↗
30. Y. Tang, F. Zhang, S. Hu, Z. Cao, Z. Wu, and W. Jing, Novel Benzimidazole Derivatives as Corrosion Inhibitors of Mild Steel in the Acidic Media. Part I: Gravimetric, Electrochemical, SEM and XPS Studies, Corr. Sci., 2013, 74, p 271–282. https://doi.org/10.1016/j.corsci.2013.04.05310.1016/j.corsci.2013.04.053 ↗
31. F. Tang, G. Chen, J.S. Volz, R.K. Brow, and M.L. Koenigstein, Cement-modified Enamel Coating for Enhanced Corrosion Resistance of Steel Reinforcing Bars, Cem. Concr. Comp., 2013, 35, p 171–180. https://doi.org/10.1016/j.cemconcomp.2012.08.00910.1016/j.cemconcomp.2012.08.009 ↗
32. H.S. Lee, H.M. Yang, J.K. Singh, S.K. Prasad, and B. Yoo, Corrosion Mitigation of Steel Rebars in Chloride Contaminated Concrete Pore Solution using Inhibitor: An Electrochemical Investigation, Constr. Build. Mater., 2018, 173, p 443–451. https://doi.org/10.1016/j.conbuildmat.2018.04.06910.1016/j.conbuildmat.2018.04.069 ↗
33. G. Liu, Y. Zhang, Z. Ni, and R. Huang, Corrosion Behavior of Steel Submitted to Chloride and Sulphate Ions in Simulated Concrete Pore Solution, Constr. Build. Mater., 2016, 115, p 1–5. https://doi.org/10.1016/j.conbuildmat.2016.03.21310.1016/j.conbuildmat.2016.03.213 ↗
34. Q. Liu, Z. Song, H. Han, S. Donkor, L. Jiang, W. Wang, and H. Chu, A Novel Green Reinforcement Corrosion Inhibitor Extracted from Waste Platanus Acerifolia Leaves, Constr. Build. Mater., 2020, 260, p 119695. https://doi.org/10.1016/j.conbuildmat.2020.11969510.1016/j.conbuildmat.2020.119695 ↗
35. C.Q. Ye, R.G. Hu, S.G. Dong, X.J. Zhang, R.Q. Hou, R.G. Du, C.J. Lin, and J.S. Pan, EIS Analysis on Chloride-Induced Corrosion Behavior of Reinforcement Steel in Simulated Carbonated Concrete Pore Solutions, J. Electroanal. Chem., 2013, 688, p 275–281. https://doi.org/10.1016/j.jelechem.2012.09.01210.1016/j.jelechem.2012.09.012 ↗
36. M.E. Orazem, B. Tribollet, Electrochemical Impedance Spectroscopy, New Jersey, 2008. http://w.electrochem.org.10.1002/9780470381588 ↗
37. R.L. Hurt and J.R. MacDonald, Distributed Circuit Elements in Impedance Spectroscopy: A Unified Treatment of Conductive and Dielectric Systems, Solid State Ion., 1986, 20, p 111–124. https://doi.org/10.1016/0167-2738(86)90018-410.1016/0167-2738(86)90018-4 ↗
38. J.R. MacDonald, Note on the Parameterization of the Constant-Phase Admittance Element, Solid State Ion., 1984, 13, p 147–149. https://doi.org/10.1016/0167-2738(84)90049-310.1016/0167-2738(84)90049-3 ↗
39. S.B. Jiang, L.H. Jiang, Z.Y. Wang, M. Jin, S. Bai, S. Song, and X. Yan, Deoxyribonucleic Acid as an Inhibitor for Chloride-Induced Corrosion of Reinforcing Steel in Simulated Concrete Pore Solutions, Constr. Build. Mater., 2017, 150, p 238–247. https://doi.org/10.1016/j.conbuildmat.2017.05.15710.1016/j.conbuildmat.2017.05.157 ↗
40. M.G. Sohail, R. Kahraman, N.A. Alnuaimi, B. Gencturk, W. Alnahhal, M. Dawood, and A. Belarbi, Electrochemical Behavior of Mild and Corrosion Resistant Concrete Reinforcing Steels, Constr. Build. Mater., 2020, 232, p 117205. https://doi.org/10.1016/j.conbuildmat.2019.11720510.1016/j.conbuildmat.2019.117205 ↗
41. Y. Tian, C. Dong, G. Wang, X. Cheng, and X. Li, The Effect of Nickel on Corrosion Behaviour of High-Strength Low Alloy Steel Rebar in Simulated Concrete Pore Solution, Constr. Build. Mater., 2020, 2020, p 246. https://doi.org/10.1016/j.conbuildmat.2020.11846210.1016/j.conbuildmat.2020.118462 ↗
42. Y. Wang, Y. Zuo, and Y. Tang, Inhibition Effect and Mechanism of Sodium Oleate on Passivation and Pitting Corrosion of Steel in Simulated Concrete Pore Solution, Constr. Build. Mater., 2018, 167, p 197–204. https://doi.org/10.1016/j.conbuildmat.2018.01.17010.1016/j.conbuildmat.2018.01.170 ↗
43. J. Shi, J. Ming, D. Wang, and M. Wu, Improved Corrosion Resistance of a new 6% Cr Steel in Simulated Concrete Pore Solution Contaminated by Chlorides, Corr. Sci., 2020, 2020, p 174. https://doi.org/10.1016/j.corsci.2020.10885110.1016/j.corsci.2020.108851 ↗
44. A. Zarrouk, B. Hammouti, T. Lakhlifi, M. Traisnel, H. Vezin, and F. Bentiss, New 1H-pyrrole-2,5-dione Derivatives as Efficient Organic Inhibitors of Carbon Steel Corrosion in Hydrochloric Acid Medium: Electrochemical, XPS and DFT Studies, Corr. Sci., 2015, 90, p 572–584. https://doi.org/10.1016/j.corsci.2014.10.05210.1016/j.corsci.2014.10.052 ↗
45. P. Ghods, O.B. Isgor, J.R. Brown, F. Bensebaa, and D. Kingston, XPS Depth Profiling Study on the Passive Oxide Film of Carbon Steel in Saturated Calcium Hydroxide Solution and the Effect of Chloride on the Film Properties, Appl. Surf. Sci., 2011, 257, p 4669–4677. https://doi.org/10.1016/j.apsusc.2010.12.12010.1016/j.apsusc.2010.12.120 ↗
46. R. Al-Gaashani, Y. Zakaria, O.S. Lee, J. Ponraj, V. Kochkodan and M.A. Atieh, Effects of Preparation Temperature on Production of Graphene Oxide by Novel Chemical Processing, Cer. Int., 2021, 47, p 10113–10122. https://doi.org/10.1016/j.ceramint.2020.12.15910.1016/j.ceramint.2020.12.159 ↗
47. N.N. Taheri, B. Ramezanzadeh, M. Mahdavian, and G. Bahlakeh, In-situ Synthesis of Zn Doped Polyaniline on Graphene Oxide for Inhibition of Mild Steel Corrosion in 3.5 wt.% Chloride Solution, J. Ind. Eng. Chem., 2018, 63, p 322–339. https://doi.org/10.1016/j.jiec.2018.02.03310.1016/j.jiec.2018.02.033 ↗
48. H. Cen and Z. Chen, Amide Functionalized Graphene Oxide as Novel and Effective Corrosion Inhibitor of Carbon Steel in CO2-Saturated NaCl Solution, Coll. Surf. A Physicochem. Eng. Asp., 2021 https://doi.org/10.1016/j.colsurfa.2021.12621610.1016/j.colsurfa.2021.126216 ↗
49. X. Xing, X. Xu, J. Wang, and W. Hu, Preparation and Inhibition Behavior of ZnMoO4/reduced Graphene Oxide Composite for Q235 Steel in NaCl Solution, Appl. Surf. Sci., 2019, 479, p 835–846. https://doi.org/10.1016/j.apsusc.2019.02.14910.1016/j.apsusc.2019.02.149 ↗
50. Q. Liu, R. Ma, A. Du, X. Zhang, Y. Fan, X. Zhao, S. Zhang, and X. Cao, Investigation on Structure and Corrosion Resistance of Complex Inorganic Passive Film Based on Graphene Oxide, Corr. Sci., 2019, 150, p 64–75. https://doi.org/10.1016/j.corsci.2019.01.02210.1016/j.corsci.2019.01.022 ↗
51. M. Morcillo, I. Díaz, H. Cano, B. Chico, and D. de la Fuente, Atmospheric Corrosion of Weathering Steels. Overview for Engineers. Part II: Testing, Inspection, Maintenance, Constr. Build. Mater., 2019, 222, p 750–765. https://doi.org/10.1016/j.conbuildmat.2019.06.15510.1016/j.conbuildmat.2019.06.155 ↗
52. M. Sun, C. Du, Z. Liu, C. Liu, X. Li, and Y. Wu, Fundamental Understanding on the Effect of Cr on Corrosion Resistance of Weathering Steel in Simulated Tropical Marine Atmosphere, Corr. Sci., 2021, 186, p 109427. https://doi.org/10.1016/j.corsci.2021.10942710.1016/j.corsci.2021.109427 ↗
53. M. Sun, X. Yang, C. Du, Z. Liu, Y. Li, Y. Wu, H. San, X. Su, and X. Li, Distinct Beneficial Effect of Sn on the Corrosion Resistance of Cr-Mo Low Alloy Steel, J. Mater. Sci. Technol., 2021, 81, p 175–189. https://doi.org/10.1016/j.jmst.2020.12.01410.1016/j.jmst.2020.12.014 ↗
54. T. Kamimura, S. Hara, H. Miyuki, M. Yamashita, and H. Uchida, Composition and Protective Ability of Rust Layer Formed on Weathering Steel Exposed to Various Environments, Corros. Sci., 2006, 48, p 2799–2812. https://doi.org/10.1016/j.corsci.2005.10.00410.1016/j.corsci.2005.10.004 ↗