What causes the variation in superconducting properties of UTe2?
Source abstract
Abstract
Reaching a consensus on the superconducting order parameter of unconventional superconductors remains a central challenge in the field of magnetically-mediated superconductivity. Though UTe$2$ is largely accepted as a rare example of an odd-parity superconductor, its precise order parameter remains highly debated, even at ambient conditions. A key underlying issue is the large sample-to-sample variation in superconducting properties at zero applied pressure and magnetic field. Here, we investigate the origin of the observed variation by means of single crystal x-ray diffraction (SC-XRD) and scanning transmission electron microscopy (STEM) measurements. Our results reveal highly ordered crystalline lattices, in agreement with the expected $Immm$ structure, and no signs of uranium vacancies. Tiny amounts of interstitial defects, however, are observed on the Te2 layers that host Te chains along the b axis. We argue that these defects give rise to slightly enhanced atomic displacement parameters observed in SC-XRD data and are enough to disrupt the unconventional superconducting state in UTe$2$. Our findings highlight the need to focus future order parameter determination efforts on single crystals of UTe$2$ with minimal amounts of structural disorder.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Rare-earth and actinide compounds · Iron-based superconductors research · Topological Materials and Phenomena
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (58)
Show source-provided references
1. Theory of superconductivity10.1103/PhysRev.108.1175 ↗
2. Tinkham · 2004
3. A common thread: The pairing interaction for unconventional superconductors10.1103/RevModPhys.84.1383 ↗
4. Unconventional superconductivity10.1080/00018732.2017.1331615 ↗
5. Topological superconductors: a review10.1088/1361-6633/aa6ac7 ↗
6. Phenomenological theory of unconventional superconductivity10.1103/RevModPhys.63.239 ↗
7. Still mystery after all these years — Unconventional superconductivity of Sr2RuO4—10.7566/JPSJ.93.062001 ↗
8. Unconventional superconductivity in UTe2
9. A review of UTe2 at high magnetic fields10.1088/1361-6633/acfb93 ↗
10. Large reduction in the a-axis Knight shift on UTe2 with Tc = 2.1 K10.7566/JPSJ.92.063701 ↗
11. Point-node gap structure of the spin–triplet superconductor UTe210.1103/PhysRevB.100.220504 ↗
12. Periodic anderson model for magnetism and superconductivity in UTe210.1103/PhysRevB.103.094504 ↗
13. Multicomponent superconducting order parameter in UTe210.1126/science.abb0272 ↗
14. Nonunitary triplet superconductivity tuned by field-controlled magnetization: URhGe, UCoGe, and UTe210.1103/PhysRevB.104.014514 ↗
15. Chiral superconductivity in UTe2 via emergent C4 symmetry and spin–orbit coupling10.1103/PhysRevB.106.014502 ↗
16. Theory of the low-and high-field superconducting phases of UTe210.1103/PhysRevB.107.214510 ↗
17. Lee · 2023
18. Orientation of point nodes and nonunitary triplet pairing tuned by the easy-axis magnetization in UTe210.1103/PhysRevResearch.2.032014 ↗
19. Anomalous normal fluid response in a chiral superconductor UTe210.1038/s41467-021-22906-6 ↗
20. Chiral superconductivity in UTe2 probed by anisotropic low-energy excitations10.1038/s41467-023-38688-y ↗
21. Microscopic imaging homogeneous and single phase superfluid density in UTe210.1103/PhysRevLett.130.196003 ↗
22. Pairing symmetries of multiple superconducting phases in UTe2: Competition between ferromagnetic and antiferromagnetic fluctuations10.1103/PhysRevB.109.064516 ↗
23. Pair kondo effect: A mechanism for time-reversal symmetry breaking superconductivity in UTe210.1103/PhysRevB.109.184501 ↗
24. Thermodynamic transitions and topology of spin–triplet superconductivity: Application to UTe210.1103/PhysRevB.109.054521 ↗
25. Christiansen · 2025
26. Yamazaki · 2025
27. Single-component superconductivity in UTe2 at ambient pressure10.1038/s41567-024-02493-1 ↗
28. Composition dependence of the superconducting properties of UTe2
29. Single thermodynamic transition at 2 K in superconducting UTe2 single crystals10.1038/s43246-022-00254-2 ↗
30. Investigating the limits of superconductivity in UTe2
31. Single crystal growth of superconducting UTe2 by molten salt flux method
32. Molten salt flux liquid transport method for ultra clean single crystals UTe210.7566/JPSJ.93.043703 ↗
33. Thermodynamic and electrical transport properties of UTe2 under uniaxial stress10.1103/PhysRevB.106.L121101 ↗
34. Fate of time-reversal symmetry breaking in UTe2
35. Fully gapped pairing state in spin–triplet superconductor UTe210.1126/sciadv.adk3772 ↗
36. Robust nodal behavior in the thermal conductivity of superconducting UTe2
37. Gu · 2025
38. Sharma · 2025
39. Low energy band structure and symmetries of UTe2 from angle-resolved photoemission spectroscopy10.1103/PhysRevLett.124.076401 ↗
40. Stabilization of U 5f2 configuration in UTe2 through U 6 d dimers in the presence of Te2 chains10.1103/PhysRevResearch.6.033299 ↗
41. Effect of uranium deficiency on normal and superconducting properties in unconventional superconductor UTe2
42. Magnetic-field-sensitive charge density waves in the superconductor UTe210.1038/s41586-023-06005-8 ↗
43. Detection of a pair density wave state in UTe210.1038/s41586-023-05919-7 ↗
44. Inhomogeneous high temperature melting and decoupling of charge density waves in spin–triplet superconductor UTe210.1038/s41467-024-48844-7 ↗
45. Absence of bulk charge density wave order in the normal state of UTe210.1038/s41467-024-53739-8 ↗
46. Absence of a bulk signature of a charge density wave in hard x-ray measurements of UTe210.1103/PhysRevB.110.145101 ↗
47. Absence of a bulk thermodynamic phase transition to a density wave phase in UTe210.1103/PhysRevB.110.144507 ↗
48. Szabo · 2025
49. Talavera · 2025
50. A ‘checkerboard’ electronic crystal state in lightly hole-doped Ca2−xNaxCuO2Cl210.1038/nature02861 ↗
51. Surface pinning of fluctuating charge order: An extraordinary surface phase transition
52. Binder · 1983 · vol. 8
53. Enhanced triplet superconductivity in next-generation ultraclean UTe210.1073/pnas.2403067121 ↗
54. Orphan high field superconductivity in non-superconducting uranium ditelluride10.1038/s41467-024-47090-1 ↗
55. Hydrostatic pressure studies on non-superconducting UTe210.7566/JPSJ.93.055001 ↗
56. Tracking aluminium impurities in single crystals of the heavy-fermion superconductor UBe1310.1038/s41598-018-28991-w ↗
57. Image registration of low signal-to-noise cryo-stem data10.1016/j.ultramic.2018.04.008 ↗
58. Crystal structure refinement with SHELXL10.1107/S2053229614024218 ↗