journal article·2025-10

Local control of perpendicular magnetic anisotropy of Pd/Co multilayers via ion bombardment

Eugenia Sebastiani-Tofano, Ana Parente, Pedro L. Alcázar Ruano, Manuel Abuín, Álvaro González-García, Jesús López-Sánchez, Juan Rubio-Zuazo, Miguel Manso Silván, Arantzazu Mascaraque, Miguel Ángel González Barrio, Mariela Menghini, Ivan K. Schuller, Ali C. Basaran, Elvira M. González, Oscar Rodríguez de la Fuente, Álvaro Muñoz-Noval

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Abstract

In this work, we have controlled locally the magnetic anisotropy of PdCo multilayers using ion beam modification. First, we have used techniques with different probing depths to confirm that cobalt is partially oxidized in the Pd/Co multilayers exhibiting PMA fabricated by sputtering, presumably due to the diffusion of atmospheric oxygen migrated through the Pd capping layer. Then, low energy ion bombardment has been employed to induce a structural disorder in the upper layers of the multilayer, gradually reducing the PMA at local scale with increasing ion doses. Medium ion doses lead to a marked decline in PMA, resulting in equivalent magnetic anisotropy directions and the loss of characteristic labyrinthine magnetic domain morphology. High ion doses completely suppress PMA, yielding a typical in-plane shape anisotropy. By combining controlled PMA reduction via lithographic techniques, we create elongated structures displaying distinct magnetic responses; bombarded regions exhibit reduced PMA, whereas adjacent regions maintain their PMA. Notably, regions with reduced PMA do not disrupt the distribution of perpendicular magnetic domains in neighboring PMA regions, even at widths as narrow as 500 nm, demonstrating the robustness of the PMA domain structure.
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Research context

OpenAlex topics: Magnetic properties of thin films · Advanced Memory and Neural Computing · Theoretical and Computational Physics

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References (57)

Show source-provided references
1. Recent developments in perpendicular magnetic anisotropy thin films for data storage applications10.1016/j.vacuum.2017.01.031 ↗
2. Perpendicular recording media for hard disk drives10.1063/1.2750414 ↗
3. Sputtered hexagonal ba-ferrite films for high-density magnetic recording media10.1063/1.361639 ↗
4. The emergence of spin electronics in data storage10.1038/nmat2024 ↗
5. Spintronics based random access memory: a review10.1016/j.mattod.2017.07.007 ↗
6. Khvalkovskiy · J. Phys. D Appl. Phys. · 2013 · 46
7. High-Resolution rotation-measuring system for mems ultrasonic motors using tunneling magnetoresistance sensors10.3390/mi15081028 ↗
8. Z. Zhou, K. Zhang, Q. Leng, Tunneling Magnetoresistance (TMR) Materials and Devices for Magnetic Sensors, in: K. Wang, M. Yang, J. Luo (Eds.), Spintronics, Wiley, 2022. https://doi.org/10.1002/9781119698968.ch3.10.1002/9781119698968.ch3 ↗
9. Electric-field tunable magnetic-field-sensor based on CoFeB/MgO magnetic tunnel junction10.1063/1.4882178 ↗
10. Precise magnetic sensors for navigation and prospection10.1007/s10948-014-2636-7 ↗
11. Magnetic sensors for navigation applications: an overview10.1017/S0373463313000544 ↗
12. L.A. Knauss, S.I. Woods, A. Orozco, Current Imaging Using Magnetic Field Sensors, in: Microelectronics Failure Analysis Desk Reference, fifth ed., ASM International, 2004, pp. 303–31.
13. Ultrasensitive magnetic field sensors for biomedical applications10.3390/s20061569 ↗
14. Improvement of the sensor system in magnetic flux leakage-type nondestructive testing (NDT)10.1109/20.996326 ↗
15. A novel high sensitivity sensor for remote field eddy current non-destructive testing based on orthogonal magnetic field10.3390/s141224098 ↗
16. A review on non-destructive evaluation of construction materials and structures using magnetic sensors10.1016/j.conbuildmat.2023.132460 ↗
17. Noncollinear spin texture-driven torque in deterministic spin–orbit torque-induced magnetization switching10.1038/s44306-024-00048-x ↗
18. Superconducting imprint of magnetic textures in ferromagnets with perpendicular magnetic anisotropy10.1038/s41598-021-99963-w ↗
19. Observation of magnetic skyrmion bubbles in a van der waals ferromagnet Fe3GeTe210.1021/acs.nanolett.9b03453 ↗
20. Chirality flips of skyrmion bubbles10.1038/s41467-022-33700-3 ↗
21. Generation of magnetic skyrmion bubbles by inhomogeneous spin hall currents10.1103/PhysRevB.93.094407 ↗
22. Large Dzyaloshinskii–moriya interaction and room-temperature nanoscale skyrmions in CoFeB/MgO heterostructures
23. Disclosing the nature of asymmetric interface magnetism in Co/Pt multilayers10.1021/acsami.1c22341 ↗
24. Strong perpendicular magnetic anisotropy of Pt/Co/AlN structure
25. Effect of increasing interaction interface on perpendicular magnetic anisotropy of Pd/Co2MnSi/Pd multilayers10.1016/j.jallcom.2021.163114 ↗
26. Magnetic anisotropy in metallic multilayers10.1088/0034-4885/59/11/002 ↗
27. Tuning of interfacial perpendicular magnetic anisotropy and domain structures in magnetic thin film multilayers10.1088/1361-6463/ab1c42 ↗
28. Ion bombardment of reconstructed metal surfaces: from two-dimensional dislocation dipoles to vacancy pits10.1103/PhysRevB.63.085420 ↗
29. Characterising and controlling surface defects10.1140/epjb/e2004-00231-9 ↗
30. Dislocation emission at the onset of plasticity during nanoindentation in gold10.1080/14786430701798951 ↗
31. Formation of a magnetite/hematite epitaxial bilayer generated with low energy ion bombardment10.1063/1.4977491 ↗
32. Spectromicroscopic study of the transformation with low energy ions of a hematite thin film into a magnetite/hematite epitaxial bilayer10.1016/j.ultramic.2023.113855 ↗
33. Formation of titanium monoxide (001) single-crystalline thin film induced by ion bombardment of titanium dioxide (110)10.1038/ncomms7147 ↗
34. Exchange bias: the antiferromagnetic bulk matters10.1063/1.4893457 ↗
35. Emergence of exchange bias and giant coercive field enhancement by internal magnetic frustration in La0.67Sr0.33MnO3 thin films10.1016/j.jmmm.2022.169077 ↗
36. Tuning Perpendicular Anisotropy Gradient in Co/Pd Multilayers by Ion Irradiation10.1063/1.4893569 ↗
37. Realization of ground-state artificial skyrmion lattices at room temperature10.1038/ncomms9462 ↗
38. Chemically driven isothermal closed space vapor transport of MoO2: thin films, flakes and in situ tellurization10.1039/C8TC01685B ↗
39. SIMNRA, a simulation program for the analysis of NRA, RBS and ERDA, application of accelerators in research and industry10.1063/1.59188 ↗
40. ATHENA, ARTEMIS, HEPHAESTUS: data analysis for X-ray absorption spectroscopy using IFEFFIT10.1107/S0909049505012719 ↗
41. Disorder-induced microscopic magnetic memory
42. Exotic topological magnetic states in thin Co/Pd ferromagnetic films10.1002/andp.202300480 ↗
43. Tuning 2D magnetism in cobalt monoxide nanosheets via in situ nickel-doping
44. Perpendicular magnetic anisotropy at transition metal/oxide interfaces and applications10.1103/RevModPhys.89.025008 ↗
45. Perpendicular magnetic anisotropy in a sputter deposited nanocrystalline high entropy alloy thin film10.1016/j.jallcom.2022.167337 ↗
46. Effects of interfacial nanoengineering through an artificial oxidation of epitaxial Pd/Co ultrathin films on perpendicular magnetic anisotropy and the dzyaloshinskii–moriya interaction10.1021/acsaelm.4c00466 ↗
47. Influence of superparamagnetism on exchange anisotropy at CoO/[Co/Pd] interfaces10.1021/acsami.6b08532 ↗
48. Influence of thermal annealing on the perpendicular magnetic anisotropy of Pt/Co/AlOx trilayers10.1103/PhysRevB.79.024423 ↗
49. Kinetics of ion migration in the electric field-driven manipulation of magnetic anisotropy of Pt/Co/oxide multilayers10.1002/smll.202102427 ↗
50. Magneto-ionic control of interfacial magnetism10.1038/nmat4134 ↗
51. Reversible control of Co magnetism by voltage-induced oxidation10.1103/PhysRevLett.113.267202 ↗
52. Role of oxygen ion migration in the electrical control of magnetism in Pt/Co/Ni/HfO2 films10.1021/acs.jpcc.5b10794 ↗
53. Ultrathin Co-O oxide layer-driven perpendicular magnetic anisotropy in a CoO/[Co/Pd]m multilayer matrix upon annealing10.1038/srep37503 ↗
54. Gibbs free energy of formation and heat capacity of PdO: a new calibration of the Pd–PdO buffer to high temperatures and pressures10.1016/0016-7037(96)00115-9 ↗
55. Ion-irradiation-induced cobalt/cobalt oxide heterostructures: printing 3D interfaces10.1021/acsami.9b13503 ↗
56. J.F. Ziegler, SRIM-2003, Nucl. Instrum. Methods Phys. Res., Sect. B 219–220 (2004) 1027–1036. https://doi.org/10.1016/j.nimb.2004.01.208.10.1016/j.nimb.2004.01.208 ↗
57. Frontiers of magnetic force microscopy10.1063/1.5050712 ↗