journal article·2010-09Open access

Finite size effects with variable range exchange coupling in thin-film Pd/Fe/Pd trilayers

R.K. Das, R. Misra, S. Tongay, R. Rairigh, A.F. Hebard

Abstract

The magnetic properties of thin-film Pd/Fe/Pd trilayers in which an embedded ~1.5 A-thick ultrathin layer of Fe induces ferromagnetism in the surrounding Pd have been investigated. The thickness of the ferromagnetic trilayer is controlled by varying the thickness of the top Pd layer over a range from 8 A to 56 A. As the thickness of the top Pd layer decreases, or equivalently as the embedded Fe layer moves closer to the top surface, the saturated magnetization normalized to area and the Curie temperature decrease whereas the coercivity increases. These thickness-dependent observations for proximity-polarized thin-film Pd are qualitatively consistent with finite size effects that are well known for regular thin-film ferromagnets. The critical exponent $β$ of the order parameter (magnetization) is found to approach the mean field value of 0.5 as the thickness of the top Pd layer increases. The functional forms for the thickness dependences, which are strongly modified by the nonuniform exchange interaction in the polarized Pd, provide important new insights to understanding nanomagnetism in two-dimensions.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Magnetic properties of thin films · Magnetic Properties and Applications · Theoretical and Computational Physics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (29)

Show source-provided references
1. Ferromagnetism in dilute solutions of cobalt in palladium10.1103/PhysRev.122.1157 ↗
2. Ferromagnetism in Pd-rich palladium–iron alloys10.1080/14786436008235850 ↗
3. Dilute ferromagnetic alloys10.1063/1.1714264 ↗
4. Ferromagnetic transition temperature of dilute Pd–Co, Pd–Fe and Pd–Mn alloys10.1016/0375-9601(73)90315-0 ↗
5. Magnetic-behavior of cobalt, iron and manganese dissolved in palladium10.1080/00018737500101461 ↗
6. Enhanced Fe moment at Pd/Fe interfaces studied by low-temperature conversion electron Mossbauer spectroscopy10.1063/1.1448800 ↗
7. Distribution of magnetic moments in Pd-3d and Ni-3d alloys10.1103/PhysRev.138.A755 ↗
8. Giant moments in palladium10.1103/PhysRevLett.56.1419 ↗
9. Distribution of ferromagnetic polarization induced by iron and cobalt atoms in palladium10.1088/0370-1328/89/1/318 ↗
10. Pd polarization and interfacial moments in Pd–Fe multilayers10.1103/PhysRevB.69.144403 ↗
11. Variation of structure and magnetic properties with thickness of thin Co59Fe26Ni15 films10.1016/j.jmmm.2004.11.247 ↗
12. Thickness-dependent coercivity of ultrathin Co films on a rough substrate: Cu-buffered Si(111)10.1016/S0039-6028(97)00837-6 ↗
13. Composition, structure, stress, and coercivity of electrodeposited soft magnetic CoNiFe films—thickness and substrate dependence10.1149/1.1421346 ↗
14. Influence of nanoporosity and roughness on the thickness-dependent coercivity of iron nanonetworks10.1007/s007060200058 ↗
15. Composition and thickness effect on magnetic properties of electrodeposited nickel–iron thin films10.1149/1.2427928 ↗
16. Remarques sur la theorie des proprietes magnetiques des couches minces et des grains fins10.1051/jphysrad:01956001703025000 ↗
17. Coercive force vs thickness for thin films of nickel–iron10.1103/PhysRev.110.583 ↗
18. Influence of finite size on critical phenomena in Ni films10.1016/0038-1098(74)90276-2 ↗
19. Magnetism in ultrathin film structures10.1088/0034-4885/71/5/056501 ↗
20. Size-dependent curie-temperature in nanoscale MnFe2O4 particles10.1103/PhysRevLett.67.3602 ↗
21. Dimensional crossover in ultrathin Ni(111) films on W(110)10.1103/PhysRevLett.68.1208 ↗
22. Thickness-dependent Curie temperatures of ultrathin magnetic films: effect of the range of spin–spin interactions10.1103/PhysRevLett.86.2665 ↗
23. Thickness-dependent curie-temperature of and its dependence on Gd(0001)/W(110) the growth-conditions10.1103/PhysRevB.47.11571 ↗
24. Magnetism in the few-monolayers limit—a surface magnetooptic Kerr-effect study of the magnetic-behavior of ultrathin films of Co, Ni, and Co–Ni alloys on Cu(100) and Cu(111)10.1103/PhysRevB.49.3962 ↗
25. Spin-wave stiffness of dilute iron–palladium alloys10.1088/0022-3719/1/6/328 ↗
26. Spin polarization in dilute magnetic alloys—with particular reference to palladium alloys10.1143/PTP.34.329 ↗
27. Aharoni · 1996
29. Ab initio calculations of exchange interactions, spin-wave stiffness constants, and curie temperatures of Fe, Co, and Ni10.1103/PhysRevB.64.174402 ↗