journal article·2026Open access

Enhancing Durability of Pt Catalysts in the Oxygen Reduction Reaction by Confinement Effect of Mesoporous Carbon

Yinghe HUANG, Renxing HUANG, Yuxing SHI, Yijie LEI, Tao YU, Cheng WANG, Jun GU

Journal of Inorganic Materials· Volume 41· Issue 3

Abstract

Pt NPs 30000 (ADT) 0.46 nm Pt NPs 0.79 nm (ECSA) 24.18%(32.33%) IPMC Pt NPs (Ostwald)
Only a short abstract or summary was supplied by the source.
Source: openalex_inverted_index · Quality: short

Research context

OpenAlex topics: Fuel Cells and Related Materials · Catalytic Processes in Materials Science · Electrocatalysts for Energy Conversion

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (35)

Show source-provided references
1. STAMBOULI A B. Fuel cells: the expectations for an environmental-friendly and sustainable source of energy. Renewable & Sustainable Energy Reviews , 2011, 15: 4507.10.1016/j.rser.2011.07.100 ↗
2. LI J R, LIU M X, LIU X, et al . The recent progress of oxygen reduction electrocatalysts used at fuel cell level. Small Methods , 2024, 8: 2301249.10.1002/smtd.202301249 ↗
3. ZHAO W H, XU G T, DONG W Y, et al . Progress and perspective for in situ studies of oxygen reduction reaction in proton exchange membrane fuel cells. Advanced Science , 2023, 10: 2300550.10.1002/advs.202300550 ↗
4. LE T D, AHEMAD M J, KIM D S, et al . Synergistic effect of Pt-Ni dual single-atoms and alloy nanoparticles as a high-efficiency electrocatalyst to minimize Pt utilization at cathode in polymer electrolyte membrane fuel cells. Journal of Colloid and Interface Science , 2023, 634: 930.10.1016/j.jcis.2022.12.061 ↗
5. FISSEHA G, YU Y N, LU S J, et al . A novel core-shell nanostructure of Ti-Au nanocrystal with PtNi alloy skin: enhancing the durability for oxygen reduction reaction. Chinese Journal of Catalysis , 2024, 56: 8110.1016/S1872-2067(23)64568-1 ↗
6. SHU Q H, ZHANG J, HU B, et al . Rational design of a high-durability pt-based ORR catalyst supported on Mn/N codoped carbon sheets for PEMFCs. Energy & Fuels , 2022, 36: 1707.10.1021/acs.energyfuels.1c04306 ↗
7. MOGHADAMESFAHANI R A, VANKOVA S K, EASTON E B, et al . A hybrid Pt/NbO/CNTs catalyst with high activity and durability for oxygen reduction reaction in PEMFC. Renewable Energy , 2020, 154: 913.10.1016/j.renene.2020.03.029 ↗
8. LI M, LIU F, PEI S, et al . Synthesis of platinum nanocrystals dispersed on nitrogen-doped hierarchically porous carbon with enhanced oxygen reduction reaction activity and durability. Nanomaterials , 2023, 13(3): 444.10.3390/nano13030444 ↗
9. CHEN L G, ZHAO W, REN Y C, et al . Study on attenuation mechanism and durability improvement of platinum-carbon catalysts for proton exchange membrane fuel cells. Journal of the Electrochemical Society , 2024, 171: 094509.10.1149/1945-7111/ad7aa3 ↗
10. SONG Z X, WANG B Q, CHENG N C, et al . Atomic layer deposited tantalum oxide to anchor Pt/C for a highly stable catalyst in PEMFCs. Journal of Materials Chemistry A , 2017, 5: 9760.10.1039/C7TA01926B ↗
11. BOGAR M, YAKOVLEV Y, SANDBECK D J S, et al . Interplay among dealloying, ostwald ripening, and coalescence in PtXNi100-X bimetallic alloys under fuel-cell-related conditions. ACS Catalysis , 2021, 11: 11360.10.1021/acscatal.1c01111 ↗
12. LI S B, YIN P, XU C, et al . Entropy-driven Ostwald ripening reversal promotes the formation of low-platinum intermetallic fuel cell catalysts. Small , 2024, 20: 2401134.10.1002/smll.202401134 ↗
13. DONG Y H, ZHANG D, LI D G, et al . Control of Ostwald ripening. Science China-Materials , 2023, 66: 1249.10.1007/s40843-022-2233-3 ↗
14. LI X F, SU F Y, XIE L J, et al . Carbon corrosion induced by surface defects accelerates degradation of platinum/graphene catalysts in oxygen reduction reaction. Small , 2024, 20: 2310940.10.1002/smll.202310940 ↗
15. GARCIA-CARDONA J L, SIRES I, MAZZUCATO M, et al . On the viability of chitosan-derived mesoporous carbons as supports for PtCu electrocatalysts in PEMFC. Electrochimica Acta , 2023, 442: 141911.10.1016/j.electacta.2023.141911 ↗
16. JAVED H, PANI S, ANTONY J, et al . Synthesis of mesoporous carbon spheres via a soft-template route for catalyst supports in PEMFC cathodes. Soft Matter , 2021, 17: 7743.10.1039/D1SM00450F ↗
17. SHAHGALDI S, HAMELIN J. Improved carbon nanostructures as a novel catalyst support in the cathode side of PEMFC: a critical review. Carbon , 2015, 94: 705.10.1016/j.carbon.2015.07.055 ↗
18. CAO L J, ZHU H W, LI Y D, et al . Anchored and confined Pt nanoparticles in radial mesoporous hollow carbon spheres enhancing oxygen reduction reaction stability. New Journal of Chemistry , 2023, 47: 10866.10.1039/D3NJ01406A ↗
19. GALEANO C, MEIER J C, PEINECKE V, et al . Toward highly stable electrocatalysts via nanoparticle pore confinement. Journal of the American Chemical Society , 2012, 134: 20457.10.1021/ja308570c ↗
20. MASHINDI V, MENTE P, PHAAHLAMOHLAKA T N, et al . Platinum nanocatalysts supported on defective hollow carbon spheres: oxygen reduction reaction durability studies. Frontiers in Chemistry , 2022, 10: 839867.10.3389/fchem.2022.839867 ↗
21. YARLAGADDA V, CARPENTER M K, MOYLAN T E, et al . Boosting fuel cell performance with accessible carbon mesopores. ACS Energy Letters , 2018, 3: 618.10.1021/acsenergylett.8b00186 ↗
22. PENG L, PENG H, HUNG C T, et al . Programmable synthesis of radially gradient-structured mesoporous carbon nanospheres with tunable core-shell architectures. Chem , 2021, 7: 1020.10.1016/j.chempr.2021.01.001 ↗
23. LIU H, CUI W H, SHEN Y F, et al . Hierarchical carbon with microporous core and mesoporous shell for efficient oxygen reduction application. Microporous and Mesoporous Materials , 2024, 368: 113011.10.1016/j.micromeso.2024.113011 ↗
24. QIAO Z, HWANG S, LI X, et al . 3D porous graphitic nanocarbon for enhancing the performance and durability of Pt catalysts: a balance between graphitization and hierarchical porosity. Energy & Environmental Science , 2019, 12: 2830.10.1039/C9EE01899A ↗
25. WANG S J, NIU M, ZHENG J, et al . Hollow porous CoP-carbon nanocages for hydrogen evolution reactions. ACS Applied Nano Materials , 2024, 7: 12821.10.1021/acsanm.4c01350 ↗
26. XIE M, CHU T K, WANG X L, et al . Effect of mesoporous carbon on oxygen reduction reaction activity as cathode catalyst support for proton exchange membrane fuel cell. International Journal of Hydrogen Energy , 2022, 47: 28074.10.1016/j.ijhydene.2022.06.131 ↗
27. HUANG L, WEI M, QI R J, et al . An integrated platinum-nanocarbon electrocatalyst for efficient oxygen reduction. Nature Communications , 2022, 13: 6703.10.1038/s41467-022-34444-w ↗
28. HUANG Y H, GU J, HU Y D, et al . Preparation of mesoporous carbon with adjustable diameter and pore size. Diamond and Related Materials , 2022, 130: 109515.10.1016/j.diamond.2022.109515 ↗
29. FERRO G, ROIRON C, WANG H S, et al . Designer electrocatalysts for the oxygen reduction reaction with controlled platinum nanoparticle locality. Advanced Energy Materials , 2024, 15(25): 2403165.10.1002/aenm.202403165 ↗
30. JEONG Y, CUI M C, CHOI J, et al . Development of modified mesoporous carbon (CMK-3) for improved adsorption of bisphenol-A. Chemosphere , 2020, 238: 124559.10.1016/j.chemosphere.2019.124559 ↗
31. ZOU J, FAN C Y, JIANG Y, et al . A preliminary study on assessing the Brunauer-Emmett-Teller analysis for disordered carbonaceous materials. Microporous and Mesoporous Materials , 2021, 327: 111411.10.1016/j.micromeso.2021.111411 ↗
32. ABBASLOU R M, VOSOUGHI V, DALAI A K. Comparison of nitrogen adsorption and transmission electron microscopy analyses for structural characterization of carbon nanotubes. Applied Surface Science , 2017, 419: 817.10.1016/j.apsusc.2017.04.253 ↗
33. GARSANY Y, BATURINA O A, SWIDER L K E, et al . Experimental methods for quantifying the activity of platinum electrocatalysts for the oxygen reduction reaction. Analytical Chemistry , 2010, 82: 6321.10.1021/ac100306c ↗
34. ZHU S J, HUANG Y H, YU T, et al . Enhance the durability of the oxygen reduction reaction catalyst through the synergy of improved graphitization and nitrogen doping of carbon carrier. International Journal of Hydrogen Energy , 2024, 51: 956.10.1016/j.ijhydene.2023.10.272 ↗
35. ZHANG C, FENG Z X, LEI Y J, et al . Batch synthesis of high activity and durability carbon supported platinum catalysts for oxygen reduction reaction using a new facile continuous microwave pipeline technology. Journal of Colloid and Interface Science , 2022, 628: 174.10.1016/j.jcis.2022.08.058 ↗