journal article·2022Open access

Microstructure and Mechanical Properties of SiC Joint Brazed by Al-Ti Alloys as Filler Metal

Puhao XU, Xiangzhao ZHANG, Guiwu LIU, Mingfen ZHANG, Xinyi GUI, Guanjun QIAO

Journal of Inorganic Materials· Volume 37· Issue 6

Abstract

SiC ceramic has excellent overall properties, and joining it to other materials with high joint strength is an important issue in the actual applications. Brazing of SiC ceramic to itself was performed using the as-fabricated Al-(10, 20, 30, 40)Ti alloys with nominal Ti concentrations of 10%, 20%, 30%, and 40% at 1550 30 min. The average joint shear strength fluctuates in the range of ~100-260 MPa with the interlayer thickness of ~50 m. Moreover, the average strength SiC/Al-20Ti/SiC joint is increased markedly with the interlayer thickness decreasing from ~100 to 25 m, reaching the maximum of ~315 MPa. Meanwhile, the (Al) phase in the interlayers is reduced gradually till disappear with the thinnest brazing interlayer, leaving the Al 4 C 3 , TiC and (Al,Si) 3 Ti phases in the interlayer. The joint fractures of SiC/Al-20Ti/SiC joint mainly occur in the SiC ceramic substrate near the interlayer/ceramic interface.
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Research context

OpenAlex topics: Aluminum Alloys Composites Properties · Metal Alloys Wear and Properties · Advanced materials and composites

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References (37)

Show source-provided references
1. LIU G W, ZHANG X Z, YANG J, et al. Recent advances in joining of SiC-based materials (monolithic SiC and SiCf/SiC composites): joining processes, joint strength, and interfacial behavior. Journal of Advanced Ceramics, 2019, 8(1): 19-38.10.1007/s40145-018-0297-x ↗
2. ZHAO S, YANG Z C, ZHOU X G. Fracture behavior of SiC/SiC composites with different interfaces. Journal of Inorganic Materials, 2016, 31(1): 58-62.10.15541/jim20150278 ↗
3. FERNIE J, DREW R, KNOWLES K. Joining of engineering ceramics. International Materials Reviews, 2009, 54: 283-331.10.1179/174328009X461078 ↗
4. YOON D H, REIMANIS I E. A review on the joining of SiC for high-temperature applications. Journal of the Korean Ceramic Society, 2020, 57(5): 246-270.10.1007/s43207-020-00021-4 ↗
5. VALENZA F, GAMBARO S, MUOLO M L, et al. Wetting of SiC by Al-Ti alloys and joining by in-situ formation of interfacial Ti3Si(Al)C2. Journal of the European Ceramic Society, 2018, 38(11): 3727-3734.10.1016/j.jeurceramsoc.2018.04.025 ↗
6. LIU Y, HUANG Z R, LIU X J. Joining of sintered silicon carbide using ternary Ag-Cu-Ti active brazing alloy. Ceramics International, 2009, 35(8): 3479-3484.10.1016/j.ceramint.2009.03.016 ↗
7. XIONG H P, WEI M, XIE Y H, et al. Control of interfacial reactions and strength of the SiC/SiC joints brazed with newly- developed Co-based brazing alloy. Journal of Materials Research, 2007, 22(10): 2727-2736.10.1557/JMR.2007.0370 ↗
8. KOLTSOV A, HODAJ F, EUSTATHOPOULOS N. Brazing of AlN to SiC by Pr silicides: physicochemichal aspects. Materials Science and Engineering: A, 2008, 495(1/2): 259-264.10.1016/j.msea.2007.11.092 ↗
9. RICCARDI B, NANNETTI C A, WOLTERSDORF J, et al. Joining of SiC based ceramics and composites with Si-16Ti and Si-18Cr eutectic alloys. International Journal of Materials & Product Technology, 2004, 20(5): 440-451.10.1504/IJMPT.2004.004778 ↗
10. ZHAO S T, ZHAGN X Z, LIU G W, et al. Surface metallization of SiC ceramic by Mo-Ni-Si coatings for improving its wettability by molten Ag. Rare Metal Materials and Engineering, 2018, 47(3): 759-765.10.1016/S1875-5372(18)30105-X ↗
11. LIU G W, MUOLO M L, VALENZA F, et al. Survey on wetting of SiC by molten metals. Ceramics International, 2010, 36(4): 1177-1188.10.1016/j.ceramint.2010.01.001 ↗
12. ZHAO H T, HUANG J H, ZHANG H, et al. Vacuum brazing of Si/SiC ceramic and low expansion titanium alloy by using Cu-Ti fillers. Rare Metal Materials and Engineering, 2007, 36(12): 2184-2188.
13. LI J K, LIU L, LIU X. Joining of SiC ceramic by 22Ti-78Si high- temperature rutectic brazing alloy. Journal of Inorganic Materials, 2011, 26(12): 1314-1318.10.3724/SP.J.1077.2011.01314 ↗
14. FU W, SONG X G, TIAN R C, et al. Wettability and joining of SiC by Sn-Ti: Microstructure and mechanical properties. Journal of Materials Science and Technology, 2020, 40: 15-23.10.1016/j.jmst.2019.08.040 ↗
15. XU P H, GUI X Y, ZHANG X Z, et al. Wetting and interfacial behavior of Al-Ti/4H-SiC system: A combined study of experiment and DFT simulation. Ceramics International, 2021, 47: 69-77.10.1016/j.ceramint.2021.08.149 ↗
16. HAO Z T, WANG D P, YANG Z W, et al. Microstructural evolution and mechanical properties of FeNi42alloy and SiC ceramic joint vacuum brazed with Ag-based filler metals. Ceramics International, 2020, 46(8): 12795-12805.10.1016/j.ceramint.2020.02.049 ↗
17. PRAKASH P, MOHANDAS T, RAJU P D. Microstructural characterization of SiC ceramic and SiC-metal active metal brazed joints. Scripta Materialia, 2005, 52(11): 1169-1173.10.1016/j.scriptamat.2005.01.034 ↗
18. TIAN W B, SUN Z M, ZHANG P, et al. Brazing of silicon carbide ceramics with Ni-Si-Ti powder mixtures. Journal of the Australian Ceramic Society, 2017, 53(2): 511-516.10.1007/s41779-017-0061-7 ↗
19. SUDMEYER I, HETTESHEIMER T, ROHDE M. On the shear strength of laser brazed SiC-steel joints: effects of braze metal fillers and surface patterning. Ceramics International, 2010, 36(3): 1083-1090.10.1016/j.ceramint.2009.12.010 ↗
20. CHEN Z B, HU S P, SONG X G, et al. Brazing of SiC ceramics pretreated by chromium coating using inactive AgCu filler metal. International Journal of Applied Ceramic Technology, 2020, 17(6): 2591-2597.10.1111/ijac.13605 ↗
21. LIU Y, ZHU Y Z, YANG Y, et al. Microstructure of reaction layer and its effect on the joining strength of SiC/SiC joints brazed using Ag-Cu-In-Ti alloy. Journal of Advanced Ceramics, 2014, 3(1): 71-75.10.1007/s40145-014-0095-z ↗
22. MOSZNER F, MATA-OSORO G, CHIODI M, et al. Mechanical behavior of SiC joints brazed using an active Ag-Cu-In-Ti braze at elevated temperatures. International Journal of Applied Ceramic Technology, 2017, 14(4): 703-711.10.1111/ijac.12689 ↗
23. HE H M, LU C Y, HE H M, et al. Characterization of SiC ceramic joints brazed using Au-Ni-Pd-Ti high-temperature filler alloy. Materials, 2019, 12(6): 931.10.3390/ma12060931 ↗
24. QIN Q, ZHANG J, LU CJ, et al. Microstructure and mechanical properties of the SiC/Zr4 joints brazed with TiZrNiCu filler for nuclear application. Progress in Natural Science-Materials International, 2018, 28(3): 124-131.10.1016/j.pnsc.2018.04.006 ↗
25. XIONG H P, WEI M, XIE Y H, et al. Brazing of SiC to a wrought nickel-based superalloy using CoFeNi(Si, B)CrTi filler metal. Materials Letters, 2007, 61(25): 4662-4665.10.1016/j.matlet.2007.03.003 ↗
26. SONG X G, CHEN Z B, HU S P, et al. Wetting behavior and brazing of titanium-coated SiC ceramics using Sn0.3Ag0.7Cu filler. Journal of the American Ceramic Society, 2019, 103(2): 912-920.10.1111/jace.16827 ↗
27. CHEN Z B, BIAN H, NIU C N, et al. Titanium-deposition assisted brazing of SiC ceramics using inactive AgCu filler. Materials Characterization, 2018, 142: 219-222.10.1016/j.matchar.2018.05.054 ↗
28. DAI X Y, CAO J, CHEN Z, et al. Brazing SiC ceramic using novel B4C reinforced Ag-Cu-Ti composite filler. Ceramics International, 2016, 42(5): 6319-6328.10.1016/j.ceramint.2016.01.021 ↗
29. LIU Y, QI Q, ZHU Y, et al. Microstructure and joining strength evaluation of SiC/SiC joints brazed with SiCp/Ag-Cu-Ti hybrid tapes. Journal of Adhesion Science and Technology, 2015, 29(15): 1563-1571.10.1080/01694243.2015.1034925 ↗
30. LI Z, WEI R W, WEN Q, et al. Microstructure and mechanical properties of SiC ceramic joints vacuum brazed with in-situ formed SiC particulate reinforced Si-24Ti alloy. Vacuum, 2019, 173: 109160.10.1016/j.vacuum.2019.109160 ↗
31. ZHONG Z H, HOU G X, ZHU Z X, et al. Microstructure and mechanical strength of SiC joints brazed with Cr3C2 particulate reinforced Ag-Cu-Ti brazing alloy. Ceramics International, 2018, 44(10): 11862-11868.10.1016/j.ceramint.2018.04.002 ↗
32. SONG Y Y, LIU D, HU S P, et al. Graphene nanoplatelets reinforced AgCuTi composite filler for brazing SiC ceramic. Journal of the European Ceramic Society, 2019, 39(4): 696-704.10.1016/j.jeurceramsoc.2018.11.046 ↗
33. ZHOU X B, LI Y B, LI Y F, et al. Residual thermal stress of SiC/Ti3SiC2/SiC joints calculation and relaxed by post-annealing. International Journal of Applied Ceramic Technology, 2018, 15: 1157-1165.10.1111/ijac.12900 ↗
34. ZHOU X B, HAN Y H, SHEN X F, et al. Fast joining SiC ceramics with Ti3SiC2 tape film by electric field-assisted sintering technology. Journal of Nuclear Materials, 2015, 466: 322-327.10.1016/j.jnucmat.2015.08.004 ↗
35. YANG D X, ZHOU Y, YAN X H, et al. Highly conductive wear resistant Cu/Ti3SiC2(TiC/SiC) co-continuous composites via vacuum infiltration process. Journal of Advanced Ceramics, 2020, 9(1): 83-93.10.1007/s40145-019-0350-4 ↗
36. ZHANG X Z, LIU G W, TAO J N, et al. Brazing of WC-8Co cemented carbide to steel using Cu-Ni-Al alloys as filler metal: microstructures and joint mechanical behavior. Journal of Materials Science and Technology, 2018, 34(7): 1180-1188.10.1016/j.jmst.2017.11.040 ↗
37. ZHOU X B, JING L, KWON Y D, et al. Fabrication of SiCw/Ti3SiC2 composites with improved thermal conductivity and mechanical properties using spark plasma sintering. Journal of Advanced Ceramics, 2020, 9(4): 462-470.10.1007/s40145-020-0389-2 ↗