Perspective of MXetronics
Source abstract
Abstract
Atomic-thin transition metal carbonitrides (MXenes), as an emerging class of two-dimensional (2D) materials, become a highly active research topic.Since the discovery of graphene nearly 20 years ago, many 2D materials (graphene, transition metal dichalcogenides, and black phosphorus) have been extensively studied in the field of micro-nano electronics.However, research on MXenes-based micro-nano electronics has just begun.MXenes exhibit rich elemental compositions and unique physicochemical properties, such as hydrophilicity, tunable work function, adjustable functional groups, fast ion and electron transport, superconductivity, surface plasmons, photo-thermo-electricity, electromagnetic absorption, and some MXenes also possess high conductivity.These characteristics make MXenes hold great potential for device applications at the microscale or even nanoscale.In recent years, the Alshareef research group has been dedicated to bringing MXenes into the field of micro-nano electronics and has defined the emerging academic field of MXene electronics, known as MXetronics, in 2019.This perspective article briefly summarizes and evaluates representative research progress in this field, including the challenges in synthesis, processing, property investigation, and device applications at the microelectronic level.Furthermore, we will propose several key research directions and unexplored subfields in this area.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advanced MEMS and NEMS Technologies · Photonic and Optical Devices · Sensor Technology and Measurement Systems
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (31)
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1. NOVOSELOV K S, GEIM A K, MOROZOV S V, et al. Electric field effect in atomically thin carbon films. Science, 2004, 306(5696): 666.10.1126/science.1102896 ↗
2. XU X, GUO T, LANZA M, et al. Status and prospects of MXene-based nanoelectronic devices. Matter, 2023, 6(3): 800.10.1016/j.matt.2023.01.019 ↗
3. NAGUIB M, KURTOGLU M, PRESSER V, et al. Two-dimensional nanocrystals produced by exfoliation of Ti3AlC2. Advanced Materials, 2011, 23(37): 4248.10.1002/adma.201102306 ↗
4. WANG H, YAO Z, ACAUAN L, et al. Toward MXene interconnects. Matter, 2021, 4(5): 1447.10.1016/j.matt.2021.04.008 ↗
5. KHAZAEI M, ARAI M, SASAKI T, et al. Novel electronic and magnetic properties of two-dimensional transition metal carbides and nitrides. Advanced Functional Materials, 2013, 23(17): 2185.10.1002/adfm.201202502 ↗
6. KAMYSBAYEV V, FILATOV A S, HU H, et al. Covalent surface modifications and superconductivity of two-dimensional metal carbide MXenes. Science, 2020, 369(6506): 979.10.1126/science.aba8311 ↗
7. LIU Y, XIAO H, GODDARD W A. Schottky-barrier-free contacts with two-dimensional semiconductors by surface-engineered MXenes. Journal of the American Chemical Society, 2016, 138(49): 15853.10.1021/jacs.6b10834 ↗
8. EL-DEMELLAWI J K, LOPATIN S, YIN J, et al. Tunable multipolar surface plasmons in 2D Ti3C2Tx MXene flakes. ACS Nano, 2018, 12(8): 8485.10.1021/acsnano.8b04029 ↗
9. LIPATOV A, GOAD A, LOES M J, et al. High electrical conductivity and breakdown current density of individual monolayer Ti3C2Tx MXene flakes. Matter, 2021, 4(4): 1413.10.1016/j.matt.2021.01.021 ↗
10. LIPATOV A, LOES M J, VOROBEVA N S, et al. High breakdown current density in monolayer Nb4C3Tx MXene. ACS Materials Letters, 2021, 3(8): 1088.10.1021/acsmaterialslett.1c00324 ↗
11. HU C, WEI Z, LI L, et al. Strategy toward semiconducting Ti3C2Tx- MXene: phenylsulfonic acid groups modified Ti3C2Tx as photosensitive material for flexible visual sensory-neuromorphic system. Advanced Functional Materials, DOI: 10.1002/adfm.202302188.10.1002/adfm.202302188 ↗
12. HU C, DU Z, WEI Z, et al. Functionalized Ti3C2Tx MXene with layer-dependent band gap for flexible NIR photodetectors. Applied Physics Reviews, 2023, 10: 021402.10.1063/5.0140861 ↗
13. LI Y, SHAO H, LIN Z, et al. A general Lewis acidic etching route for preparing MXenes with enhanced electrochemical performance in non-aqueous electrolyte. Nature Materials, 2020, 19(8): 894.10.1038/s41563-020-0657-0 ↗
14. WANG D, ZHOU C, FILATOV A S, et al. Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes. Science, 2023, 379(6638): 1242.10.1126/science.add9204 ↗
15. WU H, ALMALKI M, XU X, et al. MXene-derived metal-organic frameworks. Journal of the American Chemical Society, 2019, 141(51): 20037.10.1021/jacs.9b11446 ↗
16. ZHANG Y Z, WANG Y, JIANG Q, et al. MXene printing and patterned coating for device applications. Advanced Materials, 2020, 32(21): 1908486.10.1002/adma.201908486 ↗
17. GUO T, XU X, LIU C, et al. Large-area metal-semiconductor heterojunctions realized via MXene-induced two-dimensional surface polarization. ACS Nano, 2023, 17(9): 8324.10.1021/acsnano.2c12684 ↗
18. WANG Z, KIM H, ALSHAREEF H N. Oxide thin-film electronics using all-MXene electrical contacts. Advanced Materials, 2018, 30(15): 1706656.10.1002/adma.201706656 ↗
19. KIM H, WANG Z, ALSHAREEF H N. MXetronics: electronic and photonic applications of MXenes. Nano Energy, 2019, 60: 179.10.1016/j.nanoen.2019.03.020 ↗
20. KIM H, ALSHAREEF H N. MXetronics: MXene-enabled electronic and photonic devices. ACS Materials Letters, 2019, 2(1): 55.10.1021/acsmaterialslett.9b00419 ↗
21. XU X, WU H, HE X, et al. Iontronics using V2CTx MXene- derived metal-organic framework solid electrolytes. ACS Nano, 2020, 14(8): 9840.10.1021/acsnano.0c02497 ↗
22. KIM H, NUGRAHA M I, GUAN X, et al. All-solution-processed quantum dot electrical double-layer transistors enhanced by surface charges of Ti3C2Tx MXene contacts. ACS Nano, 2021, 15(3): 5221.10.1021/acsnano.0c10471 ↗
23. XU X, GUO T, HOTA M K, et al. High-yield Ti3C2Tx MXene-MoS2 integrated circuits. Advanced Materials, 2022, 34(48): 2107370.10.1002/adma.202107370 ↗
24. WANG C, XU X, TYAGI S, et al. Ti3C2Tx MXene van der Waals gate contact for GaN high electron mobility transistors. Advanced Materials, 35: 2211738.10.1002/adma.202211738 ↗
25. XU X, WANG Z, LOPATIN S, et al. Wafer-scale quasi-single crystalline MoS2 realized by epitaxial phase conversion. 2D Materials, 2019, 6(1): 015030.10.1088/2053-1583/aaf3e9 ↗
26. XU X, DAS G, HE X, et al. High-performance monolayer MoS2 films at the wafer scale by two-step growth. Advanced Functional Materials, 2019, 29(32): 1901070.10.1002/adfm.201901070 ↗
27. XU X, ZHANG C, HOTA M K, et al. Enhanced quality of wafer-scale MoS2 films by a capping layer annealing process. Advanced Functional Materials, 2020, 30(11): 1908040.10.1002/adfm.201908040 ↗
28. XU X, GUO T, KIM H, et al. Growth of 2D Materials at the wafer scale. Advanced Materials, 2022, 34(14): 2108258.10.1002/adma.202108258 ↗
29. LYU B, CHOI Y, JING H, et al. 2D MXene-TiO2 core-shell nanosheets as a data-storage medium in memory devices. Advanced Materials, 2020, 32(17): 1907633.10.1002/adma.201907633 ↗
30. MELIANAS A, KANG M A, VAHIDMOHAMMADI A, et al. High-speed ionic synaptic memory based on 2D titanium carbide MXene. Advanced Functional Materials, 2022, 32(12): 2109970.10.1002/adfm.202109970 ↗
31. LI B, ZHU Q B, CUI C, et al. Patterning of wafer-scale MXene films for high-performance image sensor arrays. Advanced Materials, 2022, 34(17): 2201298.10.1002/adma.202201298 ↗