Na and O Co-doped Carbon Nitride for Efficient Photocatalytic Hydrogen Evolution
Source abstract
Abstract
Elemental doping is an effective strategy for tuning the band structure of graphite carbon nitride (CN) to enhance its photocatalytic performance.In this study, sodium (Na) and oxygen (O) co-doped carbon nitride (Na/O-CN x , x=1.0, 2.0, 3.0, 4.0) was synthesized via solid-phase reaction of sodium citrate (NaCA) and pure CN powder in the Teflon-sealed autoclave under air conditions at 180 .Surface area of Na/O-CN 3.0 is measured to be 18.8 m 2 /g, increasing by 60.7% compared to that of pure CN (11.7 m 2 /g).Bandgap energy of Na/O-CN 3.0 is determined to be 2.68 eV, marginally lower than that of pure CN (2.70 eV), thereby enhancing its capacity for sunlight absorption.Meanwhile, the incorporation of Na and O atoms into Na/O-CN x is found to effectively reduce recombination rates of photogenerated electron-hole pairs.As a result, Na/O-CN x samples exhibit markedly enhanced photocatalytic hydrogen evolution activity under visible light irradiation.Notably, the optimal Na/O-CN 3.0 sample achieves a photocatalytic hydrogen production rate of 103.2 molg -1 h -1 , which is 8.2 times greater than that of pure CN (11.2 molg -1 h -1 ).Furthermore, a series of Na/O-CN x -yO 2 (y=0, 20%, 40%, 60%, 80%, 100%) samples were prepared by modulating the oxygen content within reaction atmosphere.The catalytic performance evaluations reveal that the incorporation of both Na and O atoms in Na/O-CN 3.0 enhances photocatalytic activity.This study also introduces novel methodologies for synthesis of metal atom-doped CN materials at lower temperature, highlighting the synergistic effect of Na and O atoms in photocatalytic hydrogen production of Na/O-CN x samples.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advanced Photocatalysis Techniques · Advanced Nanomaterials in Catalysis · Electrocatalysts for Energy Conversion
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (59)
Show source-provided references
1. SU C W, PANG L D, QIN M, et al. The spillover effects among fossil fuel, renewables and carbon markets: evidence under the dual dilemma of climate change and energy crises. Energy, 2023, 274: 127304.10.1016/j.energy.2023.127304 ↗
2. LI Y M, ALHARTHI M, AHMAD I, et al. Nexus between renewable energy, natural resources and carbon emissions under the shadow of transboundary trade relationship from South East Asian economies. Energy Strategy Rev., 2022, 41: 100855.10.1016/j.esr.2022.100855 ↗
3. PANG L D, ZHU M N, YU H Y, et al. Is green finance really a blessing for green technology and carbon efficiency? Energy Econ., 2022, 114: 106272.10.1016/j.eneco.2022.106272 ↗
4. INDRAWIRAWAN S, SUN H Q, DUAN X G, et al. Nanocarbons in different structural dimensions (0-3D) for phenol adsorption and metal-free catalytic oxidation. Appl. Catal. B Environ., 2015, 179: 352.10.1016/j.apcatb.2015.05.049 ↗
5. LIN Y Y, HUNG K Y, LIU F Y, et al. Photocatalysts of quaternary composite, bismuth oxyfluoride/bismuth oxyiodide/graphitic carbon nitride: synthesis, characterization, and photocatalytic activity. Mol. Catal., 2022, 528: 112463.10.1016/j.mcat.2022.112463 ↗
6. ZHANG Z, YANG L, LIU J R, et al. Improved oxygen electrocatalysis at FeN4 and CoN4 sites via construction of axial coordination. Chin. Chem. Lett., 2025, 36(2): 110013.10.1016/j.cclet.2024.110013 ↗
7. XU T, DING X T, CHENG H H, et al. Moisture-enabled electricity from hygroscopic materials: a new type of clean energy. Adv. Mater., 2023, 36(12): 2209661.10.1002/adma.202209661 ↗
8. MANDAL D, ANDRADA D M. Oil droplets cut to the chase. Nat. Chem., 2020, 12(12): 1089.10.1038/s41557-020-00588-9 ↗
9. NISHIYAMA H, YAMADA T, NAKABAYASHI M, et al. Photocatalytic solar hydrogen production from water on a 100-m2 scale. Nature, 2021, 598(7880): 304.10.1038/s41586-021-03907-3 ↗
10. TANG D, TAN G L, LI G W, et al. State-of-the-art hydrogen generation techniques and storage methods: a critical review. J. Energy Storage, 2023, 64: 107196.10.1016/j.est.2023.107196 ↗
11. LI C Q, DU X, JIANG S, et al. Constructing direct Z-scheme heterostructure by enwrapping ZnIn2S4 on CdS hollow cube for efficient photocatalytic H2 generation. Adv. Sci., 2022, 9(24): 2201773.10.1002/advs.202201773 ↗
12. HISATOMI T, DOMEN K. Reaction systems for solar hydrogen production via water splitting with particulate semiconductor photocatalysts. Nat. Catal., 2019, 2(5): 387.10.1038/s41929-019-0242-6 ↗
13. YI S S, ZHANG B X, WULAN B R, et al. Non-noble metals applied to solar water splitting. Energy Environ. Sci., 2016, 9(11): 145.
14. JIAO Y Y, LI Y K, WANG J S, et al. Exfoliation-induced exposure of active sites for g-C3N4/N-doped carbon dots heterojunction to improve hydrogen evolution activity. Mol. Catal., 2020, 497: 111223.10.1016/j.mcat.2020.111223 ↗
15. CHU X Y, LUAN B B, HUANG A X, et al. Controlled synthesis of 2D-2D conductive metal-organic framework/g-C3N4 heterojunctions for efficient photocatalytic hydrogen evolution. Dalton Trans., 2024, 53(6): 2534.10.1039/D3DT03894G ↗
16. YANG Y, ZHOU C Y, WANG W J, et al. Recent advances in application of transition metal phosphides for photocatalytic hydrogen production. Chem. Eng. J., 2021, 405: 126547.10.1016/j.cej.2020.126547 ↗
17. SONG B, CHEN M, ZENG G M, et al. Using graphdiyne (GDY) as a catalyst support for enhanced performance in organic pollutant degradation and hydrogen production: a review. J. Hazard. Mater., 2020, 398: 122957.10.1016/j.jhazmat.2020.122957 ↗
18. XIANG Q J, YU J G, JARONIEC M. Synergetic effect of MoS2 and graphene as cocatalysts for enhanced photocatalytic H2 production activity of TiO2 nanoparticles. J. Am. Chem. Soc., 2012, 134(15): 6575.10.1021/ja302846n ↗
19. XIAO S N, DAI W R, LIU X Y, et al. Microwave-induced metal dissolution synthesis of core-shell copper nanowires/ZnS for visible light photocatalytic H2 evolution. Adv. Energy Mater., 2019, 9(22): 1900775.10.1002/aenm.201900775 ↗
20. LI H H, WU Y, LI L, et al. Adjustable photocatalytic ability of monolayer g-C3N4 utilizing single-metal atom: density functional theory. Appl. Surf. Sci., 2018, 457: 735.10.1016/j.apsusc.2018.06.298 ↗
21. SHANG Y Y, MA Y J, CHEN X, et al. Effect of sodium doping on the structure and enhanced photocatalytic hydrogen evolution performance of graphitic carbon nitride. Mol. Catal., 2017, 433: 128.10.1016/j.mcat.2016.12.021 ↗
22. YE Z W, YUE W H, TAYYAB M, et al. Simple one-pot, high-yield synthesis of 2D graphitic carbon nitride nanosheets for photocatalytic hydrogen production. Dalton Trans., 2022, 51(48): 18542.10.1039/D2DT03272D ↗
23. SHI J Y, ZHANG J, CUI Z W, et al. In situ growth of MOF- derived sulfur vacancy-rich CdS nanoparticles on 2D polymers for highly efficient photocatalytic hydrogen generation. Dalton Trans., 2022, 51(15): 5841.10.1039/D1DT04188F ↗
24. HUANG X, WU K Y, SU C, et al. Metal-organic framework Cu-BTC for overall water splitting: a density functional theory study. Chin. Chem. Lett., 2025, 36(4): 109720.10.1016/j.cclet.2024.109720 ↗
25. WANG X C, MAEDA K, THOMAS A, et al. A metal-free polymeric photocatalyst for hydrogen production from water under visible light. Nat. Mater., 2009, 8(1): 76.10.1038/nmat2317 ↗
26. YI S S, YAN J M, WULAN B R, et al. Noble-metal-free cobalt phosphide modified carbon nitride: an efficient photocatalyst for hydrogen generation. Appl. Catal. B Environ., 2017, 200: 477.10.1016/j.apcatb.2016.07.046 ↗
27. HE J J, SUN H Q, INDRAWIRAWAN S, et al. Novel polyoxometalate@g-C3N4 hybrid photocatalysts for degradation of dyes and phenolics. J. Colloid Interface Sci., 2015, 456: 15.10.1016/j.jcis.2015.06.003 ↗
28. LI H H, WU Y, LI C, et al. Design of Pt/t-ZrO2/g-C3N4 efficient photocatalyst for the hydrogen evolution reaction. Appl. Catal. B Environ., 2019, 251: 305.10.1016/j.apcatb.2019.03.079 ↗
29. ZHOU A Q, YANG J M, ZHU X W, et al. Self-assembly construction of NiCo LDH/ultrathin g-C3N4 nanosheets photocatalyst for enhanced CO2 reduction and charge separation mechanism study. Rare Met., 2022, 41(6):2118.10.1007/s12598-022-01960-z ↗
30. ZHU X W, XU H M, BI C Z, et al. Piezo-photocatalysis for efficient charge separation to promote CO2 photoreduction in nanoclusters. Ultrason. Sonochem., 2023, 101: 106653.10.1016/j.ultsonch.2023.106653 ↗
31. WU M, YAN J M, TANG X N, et al. Synthesis of potassium- modified graphitic carbon nitride with high photocatalytic activity for hydrogen evolution. ChemSusChem, 2014, 7(9): 2654.10.1002/cssc.201402180 ↗
32. ZHU Y L, SUN Y Y, KHAN J, et al. NaClO-induced sodium-doped cyano-rich graphitic carbon nitride nanosheets with nitrogen vacancies to boost photocatalytic hydrogen peroxide production. Chem. Eng. J., 2022, 443: 136501.10.1016/j.cej.2022.136501 ↗
33. ZHAO X L, ZHANG Y G, LI F, et al. Salt-air template synthesis of Na and O doped porous graphitic carbon nitride nanorods with exceptional photocatalytic H2 evolution activity. Carbon, 2021, 179: 42.10.1016/j.carbon.2021.04.030 ↗
34. HAN X, KANG Y, SONG S, et al. Sodium ion doped graphitic carbon nitride with high crystallinity for superior photocatalytic hydrogen evolution efficiency. J. Mater. Chem. A, 2023, 11(34): 18213.10.1039/D3TA02887A ↗
35. DOU Q, HOU J H, HUSSAIN A, et al. One-pot synthesis of sodium-doped willow-shaped graphitic carbon nitride for improved photocatalytic activity under visible-light irradiation. J. Colloid Interface Sci., 2022, 624: 79.10.1016/j.jcis.2022.05.085 ↗
36. SUN Z Z, TAN Y Y, SHI X K, et al. General method to introduce π-electrons into oxygen-doped porous carbon nitride for photocatalytic hydrogen evolution and toluene oxidation. ACS Sustainable Chem. Eng., 2024, 12(2): 1051.10.1021/acssuschemeng.3c06962 ↗
37. WANG Y X, WANG H, CHEN F Y, et al. Facile synthesis of oxygen doped carbon nitride hollow microsphere for photocatalysis. Appl. Catal. B Environ., 2018, 231: 43.
38. REN J X, ZHENG Y M, LIN H W, et al. Near-infrared light- activated g-C3N4 with effective n → π* electron transition for H2O2 production. Appl. Surf. Sci., 2023, 638: 158053.10.1016/j.apsusc.2023.158053 ↗
39. WU M, HE X, JING B H, et al. Novel carbon and defects co-modified g-C3N4 for highly efficient photocatalytic degradation of bisphenol A under visible light. J. Hazard. Mater., 2020, 384: 121323.10.1016/j.jhazmat.2019.121323 ↗
40. LI Y H, HO W K, LV K L, et al. Carbon vacancy-induced enhancement of the visible light-driven photocatalytic oxidation of NO over g-C3N4 nanosheets. Appl. Surf. Sci., 2018, 430: 380.10.1016/j.apsusc.2017.06.054 ↗
41. LU X J, WANG Y, ZHANG X Y, et al. NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure for high efficient visible light photodegradation of antibiotic. J. Hazard. Mater., 2018, 341: 10.10.1016/j.jhazmat.2017.07.004 ↗
42. HU S Y, YU A C, LU R. A comparison study of sodium ion- and potassium ion-modified graphitic carbon nitride for photocatalytic hydrogen evolution. RSC Adv., 2021, 11(26): 15701.10.1039/D1RA01395E ↗
43. FANG W J, LIU J Y, YU L, et al. Novel (Na, O) co-doped g-C3N4 with simultaneously enhanced absorption and narrowed bandgap for highly efficient hydrogen evolution. Appl. Catal. B Environ., 2017, 209: 631.10.1016/j.apcatb.2017.03.041 ↗
44. MA R D, GUO X, SHI K X, et al. S-type heterojunction of MOS2/g-C3N4: construction and photocatalysis. J. Inorg. Mater., 2023, 38(10): 1176.10.15541/jim20230096 ↗
45. CHEN X, LI H K, WU Y X, et al. Facile fabrication of novel porous graphitic carbon nitride/copper sulfide nanocomposites with enhanced visible light driven photocatalytic performance. J. Colloid Interface Sci., 2016, 476: 132.10.1016/j.jcis.2016.05.024 ↗
46. KRÖGER J, JIMÉNEZ‐SOLANO A, SAVASCI G, et al. Interfacial engineering for improved photocatalysis in a charge storing 2D carbon nitride: melamine functionalized poly(heptazine imide). Adv. Energy Mater., 2021, 11(6): 2003016.10.1002/aenm.202003016 ↗
47. LIU M Q, JIAO Y Y, QIN J C, et al. Boron doped C3N4 nanodots/ nonmetal element (S, P, F, Br) doped C3N4 nanosheets heterojunction with synergistic effect to boost the photocatalytic hydrogen production performance. Appl. Surf. Sci., 2021, 541: 148558.10.1016/j.apsusc.2020.148558 ↗
48. YANG C W, XUE Z, QIN J Q, et al. Heterogeneous structural defects to prompt charge shuttle in g-C3N4 plane for boosting visible-light photocatalytic activity. Appl. Catal. B Environ., 2019, 259: 118094.10.1016/j.apcatb.2019.118094 ↗
49. SHI L, LIU G, ZHANG Y H, et al. Na, O co-doping and cyano groups synergistically adjust the band structure of g-C3N4 for improving photocatalytic oxygen evolution. Mater. Res. Bull., 2023, 167: 112423.10.1016/j.materresbull.2023.112423 ↗
50. GU J, CHEN H, JIANG F, et al. Visible light photocatalytic mineralization of bisphenol A by carbon and oxygen dual-doped graphitic carbon nitride. J. Colloid Interface Sci., 2019, 540: 97.10.1016/j.jcis.2019.01.023 ↗
51. IQBAL O, ALI H, LI N, et al. A review on the synthesis, properties, and characterizations of graphitic carbon nitride (g-C3N4) for energy conversion and storage applications. Mater. Today Phys., 2023, 34: 101080.10.1016/j.mtphys.2023.101080 ↗
52. OU H H, LIN L H, ZHENG Y, et al. Tri-s-triazine-based crystalline carbon nitride nanosheets for an improved hydrogen evolution. Adv. Mater., 2017, 29(22): 1700008.10.1002/adma.201700008 ↗
53. ZHOU J, YANG Y, ZHANG C Y. A low-temperature solid-phase method to synthesize highly fluorescent carbon nitride dots with tunable emission. Chem. Commun., 2013, 49(77): 8605.10.1039/c3cc42266f ↗
54. ZHANG Y Z, ZONG S C, CHENG C, et al. One-pot annealing preparation of Na-doped graphitic carbon nitride from melamine and organometallic sodium salt for enhanced photocatalytic H2 evolution. Int. J. Hydrog. Energy, 2018, 43(30): 13953.10.1016/j.ijhydene.2018.04.042 ↗
55. GUO F, CHEN J L, ZHANG M W, et al. Deprotonation of g-C3N4 with Na ions for efficient nonsacrificial water splitting under visible light. J. Mater. Chem. A, 2016, 4(28): 10806.10.1039/C6TA03424A ↗
56. WU M, CHEN L B, LUO X, et al. Defective carbon nitride with dual-surface engineering for highly efficient photocatalytic hydrogen evolution under visible light irradiation. Langmuir, 2024, 40(34): 18153.10.1021/acs.langmuir.4c01841 ↗
57. MAKUŁA P, PACIA M, MACYK W. How to correctly determine the band gap energy of modified semiconductor photocatalysts based on UV-Vis spectra. J. Phys. Chem. Lett., 2018, 9(23): 6814.10.1021/acs.jpclett.8b02892 ↗
58. YU H J, SHI R, ZHAO Y X, et al. Alkali-assisted synthesis of nitrogen deficient graphitic carbon nitride with tunable band structures for efficient visible-light-driven hydrogen evolution. Adv. Mater., 2017, 29(26): 1605148.10.1002/adma.201605148 ↗
59. WULANA B R, YI S S, LI S J, et al. Amorphous nickel pyrophosphate modified graphitic carbon nitride: an efficient photocatalyst for hydrogen generation from water splitting. Appl. Catal. B Environ., 2018, 231: 43.10.1016/j.apcatb.2018.02.045 ↗