Entangled nematic disclinations using multi-particle collision dynamics
Source abstract
Abstract
Colloids dispersed in nematic liquid crystals form topological composites in which colloid-associated defects mediate interactions while adhering to fundamental topological constraints. Better realising the promise of such materials requires numerical methods that model nematic inclusions in dynamic and complex scenarios. We employ a mesoscale approach for simulating colloids as mobile surfaces embedded in a fluctuating nematohydrodynamic medium to study the kinetics of colloidal entanglement. In addition to reproducing far-field interactions, topological properties of disclination loops are resolved to reveal their metastable states and topological transitions during relaxation towards ground state. The intrinsic hydrodynamic fluctuations distinguish formerly unexplored far-from-equilibrium disclination states, including configurations with localised positive winding profiles. The adaptability and precision of this numerical approach offers promising avenues for studying the dynamics of colloids and topological defects in designed and out-of-equilibrium situations.
Source: openalex_inverted_index · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Liquid Crystal Research Advancements · Micro and Nano Robotics · Pickering emulsions and particle stabilization
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
School of Physics and Astronomy, The University of Edinburgh, Peter Guthrie Tait Road, Edinburgh, EH9 3FD, UK
Department of Physics and Astronomy, Johns Hopkins University, Baltimore, MD, USA
Funding
H2020 European Research Council
References (85)
Show source-provided references
1. Stark · Phys. Rep. · 2001 · 351 · 38710.1016/S0370-1573(00)00144-7 ↗
2. Smalyukh · Annu. Rev. Condens. Matter Phys. · 2018 · 9 · 20710.1146/annurev-conmatphys-033117-054102 ↗
3. Lavrentovich · Proc. Natl. Acad. Sci. U. S. A. · 2011 · 108 · 514310.1073/pnas.1102130108 ↗
4. Wood · Science · 2011 · 334 · 7910.1126/science.1209997 ↗
5. Muševič · Science · 2006 · 313 · 95410.1126/science.1129660 ↗
6. Čopar · Phys. Rev. Lett. · 2011 · 106 · 17780110.1103/PhysRevLett.106.177801 ↗
7. Čopar · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2011 · 84 · 05170210.1103/PhysRevE.84.051702 ↗
8. Tasinkevych · Eur. Phys. J. E: Soft Matter Biol. Phys. · 2002 · 9 · 34110.1140/epje/i2002-10087-y ↗
9. Alexander · Rev. Mod. Phys. · 2012 · 84 · 49710.1103/RevModPhys.84.497 ↗
10. Terentjev · Phys. Rev. E: Stat. Phys., Plasmas, Fluids, Relat. Interdiscip. Top. · 1995 · 51 · 133010.1103/PhysRevE.51.1330 ↗
11. Gu · Phys. Rev. Lett. · 2000 · 85 · 471910.1103/PhysRevLett.85.4719 ↗
12. Mermin · Rev. Mod. Phys. · 1979 · 51 · 59110.1103/RevModPhys.51.591 ↗
13. Čopar · Phys. Rep. · 2014 · 538 · 110.1016/j.physrep.2014.01.001 ↗
14. Lintuvuori · Phys. Rev. Lett. · 2011 · 107 · 26780210.1103/PhysRevLett.107.267802 ↗
15. Shendruk · Soft Matter · 2015 · 11 · 510110.1039/C5SM00839E ↗
16. Híjar · Condens. Matter Phys. · 2019 · 22 · 1360110.5488/CMP.22.13601 ↗
17. Lee · J. Chem. Phys. · 2015 · 142 · 16411010.1063/1.4919310 ↗
18. Lee · Soft Matter · 2017 · 13 · 881610.1039/C7SM02055D ↗
19. Mandal · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2019 · 99 · 06331910.1103/PhysRevE.99.063319 ↗
20. Mandal · Eur. Phys. J. E: Soft Matter Biol. Phys. · 2021 · 44 · 6410.1140/epje/s10189-021-00072-3 ↗
21. Híjar · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2020 · 102 · 06270510.1103/PhysRevE.102.062705 ↗
22. Wamsler · Soft Matter · 2024 · 20 · 395410.1039/D3SM01536J ↗
23. Kozhukhov · Sci. Adv. · 2022 · 8 · eabo578810.1126/sciadv.abo5788 ↗
24. Macas-Durán · Soft Matter · 2023 · 19 · 805210.1039/D3SM00481C ↗
25. Senyuk · Nature · 2013 · 493 · 20010.1038/nature11710 ↗
26. Ravnik · Soft Matter · 2009 · 5 · 26910.1039/b810933h ↗
27. Malevanets · J. Chem. Phys. · 1999 · 110 · 860510.1063/1.478857 ↗
28. Winkler · Comput. Phys. Commun. · 2005 · 169 · 32610.1016/j.cpc.2005.03.073 ↗
29. Lamura · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2001 · 64 · 06180110.1103/PhysRevE.64.061801 ↗
30. Reyes-Arango · Phys. A · 2020 · 547 · 12386210.1016/j.physa.2019.123862 ↗
31. Shendruk · Anal. Chem. · 2013 · 85 · 598110.1021/ac400802g ↗
32. Zantop · J. Chem. Phys. · 2021 · 155 · 13490410.1063/5.0064558 ↗
33. Zöttl · Eur. Phys. J. E: Soft Matter Biol. Phys. · 2018 · 41 · 6110.1140/epje/i2018-11670-3 ↗
34. Sengupta · Liq. Cryst. Today · 2015 · 24 · 7010.1080/1358314X.2015.1039196 ↗
35. Čopar · Crystals · 2021 · 11 · 95610.3390/cryst11080956 ↗
36. Luo · Nat. Commun. · 2018 · 9 · 384110.1038/s41467-018-06054-y ↗
37. Noguchi · EPL · 2007 · 78 · 1000510.1209/0295-5075/78/10005 ↗
38. Götze · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2007 · 76 · 04670510.1103/PhysRevE.76.046705 ↗
39. Ihle · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2001 · 63 · 02020110.1103/PhysRevE.63.020201 ↗
40. G.Gompper , T.Ihle , D. M.Kroll and R. G.Winkler , in Multi-Particle Collision Dynamics: A Particle-Based Mesoscale Simulation Approach to the Hydrodynamics of Complex Fluids , ed. C. Holm and K. Kremer , Springer Berlin Heidelberg , Berlin, Heidelberg , 2009 , pp. 1–87
41. Híjar · Fluct. Noise Lett. · 2019 · 18 · 195001110.1142/S0219477519500111 ↗
42. Híjar · Soft Matter · 2024 · 20 · 375510.1039/D3SM01684F ↗
43. Armendáriz · Int. J. Mod. Phys. B · 2021 · 35 · 215012410.1142/S0217979221501241 ↗
44. Armendáriz · Materials · 2021 · 14 · 288610.3390/ma14112886 ↗
45. Duarte Alaniz · Phys. A · 2023 · 609 · 12829810.1016/j.physa.2022.128298 ↗
46. Lamura · Eur. Phys. J. E: Soft Matter Biol. Phys. · 2002 · 9 · 47710.1140/epje/i2002-10107-0 ↗
47. Cui · Mol. Cryst. Liq. Cryst. Sci. Technol., Sect. A · 1999 · 331 · 4910.1080/10587259908047499 ↗
48. Ž.Kos , J.Aplinc , U.Mur and M.Ravnik , in Mesoscopic Approach to Nematic Fluids , ed. F. Toschi and M. Sega , Springer International Publishing , Cham , 2019 , pp. 51–93
49. N. D.Mermin , Boojums All the Way Through , Cambridge University Press , 199010.1017/CBO9780511608216 ↗
50. Liu · Proc. Natl. Acad. Sci. U. S. A. · 2013 · 110 · 923110.1073/pnas.1301464110 ↗
51. Tasinkevych · New J. Phys. · 2012 · 14 · 07303010.1088/1367-2630/14/7/073030 ↗
52. Poulin · Science · 1997 · 275 · 177010.1126/science.275.5307.1770 ↗
53. Fukuda · Eur. Phys. J. E: Soft Matter Biol. Phys. · 2004 · 13 · 8710.1140/epje/e2004-00043-2 ↗
54. Wang · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2017 · 96 · 04270210.1103/PhysRevE.96.042702 ↗
55. Andrienko · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2001 · 63 · 04170110.1103/PhysRevE.63.041701 ↗
56. Ruhwandl · Phys. Rev. E: Stat. Phys., Plasmas, Fluids, Relat. Interdiscip. Top. · 1997 · 56 · 556110.1103/PhysRevE.56.5561 ↗
57. Friedel · CR Acad. Sci. Paris B · 1969 · 268 · 257
58. Velez · Soft Matter · 2021 · 17 · 384810.1039/D0SM02040K ↗
59. Duclos · Science · 2020 · 367 · 112010.1126/science.aaz4547 ↗
60. Shendruk · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2018 · 98 · 01060110.1103/PhysRevE.98.010601 ↗
61. Negro · Research Square · 202410.21203/rs.3.rs-3945915/v1 ↗
62. Lubensky · Phys. Rev. E: Stat. Phys., Plasmas, Fluids, Relat. Interdiscip. Top. · 1998 · 57 · 61010.1103/PhysRevE.57.610 ↗
63. Chernyshuk · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2011 · 84 · 01170710.1103/PhysRevE.84.011707 ↗
64. Pergamenshchik · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2009 · 79 · 02170410.1103/PhysRevE.79.021704 ↗
65. Dolganov · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2006 · 73 · 04170610.1103/PhysRevE.73.041706 ↗
66. Müller · Sci. Rep. · 2020 · 10 · 1271810.1038/s41598-020-69544-4 ↗
67. Noël · Phys. Rev. Lett. · 2006 · 96 · 21780110.1103/PhysRevLett.96.217801 ↗
68. Takahashi · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2008 · 77 · 02070310.1103/PhysRevE.77.020703 ↗
69. Muševič · Materials · 2018 · 11 · 2410.3390/ma11010024 ↗
70. Silvestre · J. Phys.: Condens. Matter · 2004 · 16 · S1921
71. Škarabot · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2008 · 77 · 03170510.1103/PhysRevE.77.031705 ↗
72. Alexander · Liq. Cryst. Rev. · 2022 · 10 · 9110.1080/21680396.2022.2067257 ↗
73. Guzmán · Phys. Rev. Lett. · 2003 · 91 · 23550710.1103/PhysRevLett.91.235507 ↗
74. Araki · Phys. Rev. Lett. · 2006 · 97 · 12780110.1103/PhysRevLett.97.127801 ↗
75. Ravnik · Phys. Rev. Lett. · 2007 · 99 · 24780110.1103/PhysRevLett.99.247801 ↗
76. Tkalec · Phys. Rev. Lett. · 2009 · 103 · 12780110.1103/PhysRevLett.103.127801 ↗
77. Schimming · Soft Matter · 2022 · 18 · 223410.1039/D1SM01584B ↗
78. Tkalec · Soft Matter · 2013 · 9 · 814010.1039/c3sm50713k ↗
79. Čopar · Proc. R. Soc. A · 2013 · 469 · 2013020410.1098/rspa.2013.0204 ↗
80. Jänich · Acta Appl. Math. · 1987 · 8 · 6510.1007/BF00046687 ↗
81. Jampani · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2011 · 84 · 03170310.1103/PhysRevE.84.031703 ↗
82. Tkalec · Science · 2011 · 333 · 6210.1126/science.1205705 ↗
83. Machon · Liq. Cryst. Today · 2019 · 28 · 5810.1080/1358314X.2019.1681113 ↗
84. P.-G.De Gennes and J.Prost , The Physics of Liquid Crystals , Oxford University Press , 199310.1093/oso/9780198520245.001.0001 ↗
85. Kamien · Rev. Mod. Phys. · 2002 · 74 · 95310.1103/RevModPhys.74.953 ↗