journal article·2021

Signatures of continuous hexatic–liquid transition in two-dimensional melting

Jialing Guo, Yunhuan Nie, Ning Xu

Soft Matter· Volume 17· Issue 12
Publisher page

Abstract

Recent studies have shown that the melting of two-dimensional crystals can be either continuous or discontinuous, relying on multiple parameters such as particle stiffness, density, and particle size dispersity. However, what determines the continuity or discontinuity of the two-dimensional melting remains elusive. Here we study the two-dimensional melting of binary mixtures of soft-core particles. The two particle species are different in either particle size or particle stiffness. Starting with the mono-component systems which exhibit discontinuous hexatic-liquid transition, we gradually increase the particle size or stiffness dispersity and find that the hexatic-liquid coexistent region shrinks and eventually vanishes above a critical dispersity. Therefore, the growth of disorder caused by the particle size or stiffness dispersity leads to the discontinuous-continuous transition of the two-dimensional melting. We further find that as long as the melting is continuous the defect concentrations on the boundary between hexatic and liquid phases remain almost constant, accompanied by an almost constant correlation length. These characteristic defect concentrations and correlation length are universal and independent of particle interactions, temperature, and type of particle dispersity, which act as signatures of the continuous two-dimensional melting.
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Research context

OpenAlex topics: Material Dynamics and Properties · Theoretical and Computational Physics · Pickering emulsions and particle stabilization

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Hefei National Laboratory for Physical Sciences at the Microscale

CAS Key Laboratory of Microscale Magnetic Resonance and Department of Physics

University of Science and Technology of China

Hefei 230026

People's Republic of China

Funding

National Natural Science Foundation of China

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