Magnetoelectric effects in a heterostructure of magnetostrictive fiber composite and piezopolymer film

Abstract Magnetoelectric (ME) effects in composite heterostructures comprising ferromagnetic (FM) and piezoelectric (PE) layers realize mutual transformation of magnetic and electric fields and form the basis for the development of highly sensitive magnetic field sensors, electrically tuned electronic components, and energy harvesting devices. ME effects result from a combination of magnetostriction of the FM layer and piezoelectricity in the PE layer due to mechanical coupling between the layers. In this work ME effects are studied in a flexible heterostructure containing a magnetostrictive fiber composite (MFC) and a piezopolymer layer. MFC is a set of microwires made of amorphous FeCoSiB alloy with high magnetostriction and arranged in a plane parallel to each other in a polymer matrix. MFC exhibits strong in-plane anisotropy of magnetization and magnetostriction resulting from demagnetization effects in microwires. Anisotropy leads to the dependence of the linear and nonlinear ME effects characteristics on the orientation of dc magnetic field in the plane of the heterostructure. For the fabricated heterostructure at the resonance frequency of bending vibrations, a linear ME coefficient of 24 V (Oe∙cm)⁻¹ was obtained, and the efficiency of nonlinear generation of the second voltage harmonic reached 1.6 V (Oe²∙cm)⁻¹. ME effects in MFC heterostructures can be used to create magnetic field sensors and electronic devices that are sensitive to the field orientation.