journal article·2021-05

One-step laser induced conversion of a gelatin-coated polyimide film into graphene: Tunable morphology, surface wettability and microsupercapacitor applications

WenTao Wang, LongSheng Lu, YingXi Xie, ZeHong Li, WeiBin Wu, RongXuan Liang, Yong Tang

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Abstract

Latest advances have witnessed the laser induction process on polyimide (PI) films for the formation of porous graphene. Herein, a fully converted graphene film was prepared by Nd:YAG laser scribing a gelatin coated PI film. It was found that the gelatin played the role of “shield” well in absorbing intense laser impact and benefit for the surface morphology modulation. Laser treatment lower than a critical fluence point of ~4.00 J mm−2 contributed to a crater-like surface morphology due to the dispersed nature of Nd:YAG laser beam. By tuning laser fluence above the threshold, carbonized surface turned into continuous morphology. A fluid dynamics process accompanied by outgassing occurred during the carbonization, and the surface morphology gradually varied from stretched droplets to porous strips and finally to amorphous porous structures. The morphology evolution in combination with surface chemistry is responsible for the significant wettability transition from superhydrophobic to superhydrophilic, and a Janus superhydrophobic/superhydrophilic surface wettability was achieved under a laser fluence of ~8.00 J mm−2. Eventually, microsupercapacitors (MSCs) were fabricated to show the great potential of our prepared graphene in flexible electronics.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Supercapacitor Materials and Fabrication · Graphene research and applications · Advanced Sensor and Energy Harvesting Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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