journal article·2023-05Open access

Constructing a molecular crystal actuator from pamoic acid with multilevel enhanced photoluminescence by cocrystallization

Wenjie Kuang, Yifu Chen, Bo Jing, Guanlun Sun, Songgu Wu, Junbo Gong

Science China Materials· Volume 66· Issue 5

Abstract

高效的光致发光性能促进了晶体材料的发展. 在本文中, 我们通 过引入溶剂分子报道了两例新的双羟萘酸多组分晶体. 通过聚集诱导 发射和共结晶诱导发射增强, 双羟萘酸多组分晶体的绝对量子产率逐 步增强, 最高达52.99%, 据我们所知, 这是目前报道的最大值. 此外, 随 着溶剂分子逃逸, 该系统表现出温度依赖的荧光响应和热诱导的机械 运动, 包括跳跃、摆动、翻转、移动和旋转. 本工作提出的引入共结晶 组分实现材料发光性能逐级提高的方法对设计刺激响应型光学功能材 料具有指导意义.
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Research context

OpenAlex topics: Luminescence and Fluorescent Materials · Nanoplatforms for cancer theranostics · Polydiacetylene-based materials and applications

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References (26)

Show source-provided references
1. Zhang H, Zhao Z, Turley AT, et al. Aggregate science: From structures to properties. Adv Mater, 2020, 32: 200145710.1002/adma.202001457 ↗
2. He Z, Zhao W, Lam JWY, et al. White light emission from a single organic molecule with dual phosphorescence at room temperature. Nat Commun, 2017, 8: 41610.1038/s41467-017-00362-5 ↗
3. Yang J, Zhen X, Wang B, et al. The influence of the molecular packing on the room temperature phosphorescence of purely organic luminogens. Nat Commun, 2018, 9: 84010.1038/s41467-018-03236-6 ↗
4. Yang Y, Wang J, Li D, et al. Tunable photoresponsive behaviors based on triphenylamine derivatives: The pivotal role of π-conjugated structure and corresponding application. Adv Mater, 2021, 33: 210400210.1002/adma.202104002 ↗
5. Sun H, Sun SS, Han FF, et al. Water-stimuli-responsive dynamic fluorescent switch from Kasha’s rule to anti-Kasha’s rule based on a tetraphenylethene substituted Schiff base. Chem Eng J, 2021, 405: 12700010.1016/j.cej.2020.127000 ↗
6. Zhao Y, Ding B, Huang Z, et al. Highly efficient organic long persistent luminescence based on host-guest doping systems. Chem Sci, 2022, 13: 8412–841610.1039/D2SC01622B ↗
7. Song J, Ma L, Sun S, et al. Reversible multilevel stimuli-responsiveness and multicolor room-temperature phosphorescence emission based on a single-component system. Angew Chem Int Ed, 2022, 61: e20220615710.1002/anie.202206157 ↗
8. Ma L, Wang G, Ding B, et al. Dual-responsive thermally activated delayed fluorescence of spiropyran derivatives. CCS Chem, 2021, 4: 2080–208910.31635/ccschem.021.202100992 ↗
9. Chung JW, Yoon SJ, An BK, et al. High-contrast on/off fluorescence switching via reversible E–Z isomerization of diphenylstilbene containing the α-cyanostilbenic moiety. J Phys Chem C, 2013, 117: 11285–1129110.1021/jp401440s ↗
10. Qi Q, Qian J, Tan X, et al. Remarkable turn-on and color-tuned piezochromic luminescence: Mechanically switching intramolecular charge transfer in molecular crystals. Adv Funct Mater, 2015, 25: 4005–401010.1002/adfm.201501224 ↗
11. Yang W, Yang Y, Cao X, et al. On-off switchable thermally activated delayed fluorescence controlled by multiple channels: Understanding the mechanism behind distinctive polymorph-dependent optical properties. Chem Eng J, 2021, 415: 12890910.1016/j.cej.2021.128909 ↗
12. Li S, Lu B, Fang X, et al. Manipulating light-induced dynamic macro-movement and static photonic properties within 1D isostructural hydrogen-bonded molecular cocrystals. Angew Chem Int Ed, 2020, 59: 22623–2263010.1002/anie.202009714 ↗
13. Zhou B, Yan D. Recent advances of dynamic molecular crystals with light-triggered macro-movements. Appl Phys Rev, 2021, 8: 04131010.1063/5.0059919 ↗
14. Alam P, Leung NLC, Cheng Y, et al. Spontaneous and fast molecular motion at room temperature in the solid state. Angew Chem Int Ed, 2019, 58: 4536–454010.1002/anie.201813554 ↗
15. Liu S, Zhou X, Zhang H, et al. Molecular motion in aggregates: Manipulating TICT for boosting photothermal theranostics. J Am Chem Soc, 2019, 141: 5359–536810.1021/jacs.8b13889 ↗
16. Zhao Z, Chen C, Wu W, et al. Highly efficient photothermal nanoagent achieved by harvesting energy via excited-state intramolecular motion within nanoparticles. Nat Commun, 2019, 10: 76810.1038/s41467-019-08722-z ↗
17. Liu G, Liu J, Liu Y, et al. Oriented single-crystal-to-single-crystal phase transition with dramatic changes in the dimensions of crystals. J Am Chem Soc, 2014, 136: 590–59310.1021/ja4102634 ↗
18. Li S, Hao Y, Guo S, et al. Three-primary-color molecular cocrystals showing white-light luminescence, tunable optical waveguide and ultrahigh polarized emission. Sci China Chem, 2022, 65: 408–41710.1007/s11426-021-1130-9 ↗
19. Zhou B, Yan D. Excitation-dependent organic persistent luminescence. Sci China Chem, 2020, 63: 423–42510.1007/s11426-019-9691-2 ↗
20. Huang Y, Zhang Q. Manipulating asymmetric photon transport through electrical control: A new strategy to construct optical diodes or isolators. Sci China Chem, 2018, 61: 1351–135210.1007/s11426-018-9271-5 ↗
21. Zhou B, Zhao Q, Tang L, et al. Tunable room temperature phosphorescence and energy transfer in ratiometric co-crystals. Chem Commun, 2020, 56: 7698–770110.1039/D0CC02730H ↗
22. Ding B, Ma L, Huang Z, et al. Engendering persistent organic room temperature phosphorescence by trace ingredient incorporation. Sci Adv, 2021, 7: eabf966810.1126/sciadv.abf9668 ↗
23. Kuang W, Liu J, Lin X, et al. Insoluble salt of memantine with a unique fluorescence phenomenon. Mol Pharm, 2022, 19: 1389–139910.1021/acs.molpharmaceut.1c00931 ↗
24. Haynes DA, Van de Streek J, Burley JC, et al. Pamoic acid determined from powder diffraction data. Acta Crystlogr E Struct Rep Online, 2006, 62: o1170–o117210.1107/S1600536806005812 ↗
25. Chen Y, Jing B, Chang Z, et al. Desolvation induced crystal jumping: Reversible hydration and dehydration of a spironolactone-saccharin cocrystal with water as the jumping-mate. CrystEngComm, 2021, 23: 6838–684210.1039/D1CE00830G ↗
26. Chen Y, Li J, Gong J. Jumping crystal based on an organic charge transfer complex with reversible on/off switching of luminescence by external thermal stimuli. ACS Mater Lett, 2021, 3: 275–28110.1021/acsmaterialslett.0c00575 ↗