journal article·2025-06-05Open access

Electronic structure of a nodal line semimetal candidate TbSbTe

Iftakhar Bin Elius, Jacob F. Casey, Sabin Regmi, Volodymyr Buturlim, Anup Pradhan Sakhya, Milo Sprague, Mazharul Islam Mondal, Nathan Valadez, Arun K. Kumay, Justin Scrivens, Yenugonda Venkateswara, Shovan Dan, Tetiana Romanova, Arjun K Pathak, Krzysztof Gofryk, Andrzej Ptok, Dariusz Kaczorowski, Madhab Neupane

Physical Review Materials· Volume 9· Issue 6

Abstract

The $Ln\mathrm{SbTe}$ ($Ln$ = Lanthanides) family, like isostructural ZrSiS-type compounds, has emerged as a fertile playground for exploring the interaction of electronic correlations and magnetic ordering with the nodal line band topology. Here, we report on a detailed electronic band structure investigation of TbSbTe, corroborated by electrical transport, thermodynamic, and magnetic studies. Temperature-dependent magnetic susceptibility and thermodynamic transport studies indicate the onset of antiferromagnetic ordering below ${T}N\ensuremath{\sim}5.8\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. The electronic band structure study, carried out with high-resolution angle-resolved photoemission spectroscopy measurements aided with density functional theory--based first-principles calculations reveal presence of a nonsymmorphic symmetry-protected Dirac crossing in the $\mathrm{\ensuremath{\Gamma}}$-X high-symmetry (HS) direction, which is part of a nodal line along the X-R HS direction. Another Dirac crossing occurs along the $\mathrm{\ensuremath{\Gamma}}$-X direction at a relatively higher binding energy, which occurs from ${\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\mathcal{C}}}_{2\ensuremath{\nu}}\mathcal{P}$ symmetry which is gapped in the theoretical calculations with the effect of spin-orbit coupling considered. Parallel to this direction, our theoretical calculations and experimental results exhibit strongly momentum-dependent surface bands. In this paper, we open an avenue to further uncover the intricate interplay among symmetry-protected topological band structure, spin-orbit coupling, and magnetism in this material and the $Ln\mathrm{SbTe}$ family, in general.
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Research context

OpenAlex topics: Topological Materials and Phenomena · Advanced Thermoelectric Materials and Devices · Intermetallics and Advanced Alloy Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

University of Central Florida

SUNY Buffalo State, Buffalo

Idaho National Laboratory

Polish Academy of Sciences

Funding

National Science Foundation · Air Force Office of Scientific Research · Directorate for Mathematical and Physical Sciences · Narodowe Centrum Nauki · Idaho National Laboratory · Laboratory Directed Research and Development · U.S. Department of Energy · Advanced Light Source · Lawrence Berkeley National Laboratory

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