journal article·2020-07-09Open access

Spin dynamics and a nearly continuous magnetic phase transition in an entropy-stabilized oxide antiferromagnet

Benjamin A. Frandsen, K. Alec Petersen, Nicolas A. Ducharme, Alexander G. Shaw, Ethan J. Gibson, Barry Winn, Jiaqiang Yan, Junjie Zhang, Michael E. Manley, Raphaël P. Hermann

Physical Review Materials· Volume 4· Issue 7

Abstract

Studying magnetism in entropy-stabilized oxides (ESOs) is an exciting new research avenue following the recent discovery of antiferromagnetic order in (Mg${}0.2$Co${}0.2$Ni${}0.2$Cu${}0.2$Zn${}0.2$)O (MgO-ESO). Muon spin relaxation and neutron scattering experiments reveal a continuous transition that occurs across a broad distribution of antiferromagnetic ordering temperatures throughout the MgO-ESO sample. The ground state exhibits a magnon gap and significant quasielastic neutron scattering, suggesting unusual intrinsic magnetic fluctuations. These results resolve several open questions about magnetic order in MgO-ESO and pave the way for future investigations of magnetic ESOs.
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Research context

OpenAlex topics: Magnetic and transport properties of perovskites and related materials · High-pressure geophysics and materials · Advanced Condensed Matter Physics

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