journal article·2015-11-01Open access

Structural and optical properties of Ca_xBa_1-xNb_2O_6 thin films deposited by radio frequency magnetron sputtering

S. Vigne, N. Hossain, S.M. Humayun Kabir, J. Margot, K. Wu, M. Chaker

Optical Materials Express· Volume 5· Issue 11

Abstract

Highly (001)-oriented Calcium Barium Niobate (CaxBa1-xNb2O6, CBN) thin films were grown on MgO by Radio-Frequency magnetron sputtering. Close-to-bulk film stoichiometry (Ca0.28Ba0.72Nb2O6) is obtained for an O2 fraction of 5% in the deposition chamber. At the annealing temperature of 1000 °C, (001) oriented thin films are achieved with lattice parameter in the c-direction and a chemical composition very close to that of the bulk, and a surface roughness of 2.8 nm RMS. The refractive index of the films is 2.21 at λ = 630 nm and 2.13 at λ = 1550 nm and a strong second harmonic signal can be generated nonlinearly in the films.
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Research context

OpenAlex topics: Ferroelectric and Piezoelectric Materials · Acoustic Wave Resonator Technologies · Photorefractive and Nonlinear Optics

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