journal article·2023-10-19Open access

Electronic stripe patterns near the fermi level of tetragonal Fe(Se,S)

M. Walker, K. Scott, T. J. Boyle, J. K. Byland, S. Bötzel, Z. Zhao, R. P. Day, S. Zhdanovich, S. Gorovikov, T. M. Pedersen, P. Klavins, A. Damascelli, I. M. Eremin, A. Gozar, V. Taufour, E. H. da Silva Neto

npj Quantum Materials· Volume 8· Issue 1

Abstract

Abstract FeSe1−xSx remains one of the most enigmatic systems of Fe-based superconductors. While much is known about the orthorhombic parent compound, FeSe, the tetragonal samples, FeSe1−xSx with x > 0.17, remain relatively unexplored. Here, we provide an in-depth investigation of the electronic states of tetragonal FeSe0.81S0.19, using scanning tunneling microscopy and spectroscopy (STM/S) measurements, supported by angle-resolved photoemission spectroscopy (ARPES) and theoretical modeling. We analyze modulations of the local density of states (LDOS) near and away from Fe vacancy defects separately and identify quasiparticle interference (QPI) signals originating from multiple regions of the Brillouin zone, including the bands at the zone corners. We also observe that QPI signals coexist with a much stronger LDOS modulation for states near the Fermi level whose period is independent of energy. Our measurements further reveal that this strong pattern appears in the STS measurements as short range stripe patterns that are locally two-fold symmetric. Since these stripe patterns coexist with four-fold symmetric QPI around Fe-vacancies, the origin of their local two-fold symmetry must be distinct from that of nematic states in orthorhombic samples. We explore several aspects related to the stripes, such as the role of S and Fe-vacancy defects, and whether they can be explained by QPI. We consider the possibility that the observed stripe patterns may represent incipient charge order correlations, similar to those observed in the cuprates.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Iron-based superconductors research · Physics of Superconductivity and Magnetism · Rare-earth and actinide compounds

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (37)

Show source-provided references
1. Mizuguchi, Y., Tomioka, F., Tsuda, S., Yamaguchi, T. & Takano, Y. Substitution effects on FeSe superconductor. J. Phys. Soc. Jpn 78, 07 (2009).10.1143/JPSJ.78.074712 ↗
2. Hosoi, S. et al. Nematic quantum critical point without magnetism in FeSe1−xSx superconductors. Proc. Natl. Acad. Sci. USA 113, 8139–8143 (2016).10.1073/pnas.1605806113 ↗
3. Coldea, A. I. Electronic nematic states tuned by isoelectronic substitution in bulk FeSe1−xSx. Front. Phys. 8, 528 (2021).10.3389/fphy.2020.594500 ↗
4. Walmsley, P. et al. Quasiparticle mass enhancement close to the quantum critical point in $${{{{\rm{BaFe}}}}}2{({{{{\rm{As}}}}}1-x{{{{\bf{P}}}}}x)}2$$. Phys. Rev. Lett. 110, 25 (2013).10.1103/PhysRevLett.110.257002 ↗
5. Hanaguri, T. et al. Two distinct superconducting pairing states divided by the nematic end point in FeSe1−xSx. Sci. Adv. 4, 5 (2018).10.1126/sciadv.aar6419 ↗
6. Sato, Y. et al. Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1−xSx. Proc. Natl Acad. Sci. USA 115, 1227–1231 (2018).10.1073/pnas.1717331115 ↗
7. Shibauchi, T., Hanaguri, T. & Matsuda, Y. Exotic superconducting states in FeSe-based materials. J. Phys. Soc. Jpn 89, 10 (2020).10.7566/JPSJ.89.102002 ↗
8. Setty, C., Bhattacharyya, S., Cao, Y., Kreisel, A. & Hirschfeld, P. Topological ultranodal pair states in iron-based superconductors. Nat. Commun. 11, 523 (2020).10.1038/s41467-020-14357-2 ↗
9. Agterberg, D. F., Brydon, P. M. R. & Timm, C. Bogoliubov Fermi surfaces in superconductors with broken time-reversal symmetry. Phys. Rev. Lett. 118, 12 (2017).10.1103/PhysRevLett.118.127001 ↗
10. Moore, S. A. et al. Evolution of the superconducting properties in FeSe1−xSx. Phys. Rev. B 92, 23 (2015).10.1103/PhysRevB.92.235113 ↗
11. Song, C.-L. et al. Suppression of superconductivity by twin boundaries in FeSe. Phys. Rev. Lett. 109, 13 (2012).10.1103/PhysRevLett.109.137004 ↗
12. Watashige, T. et al. Evidence for time-reversal symmetry breaking of the superconducting state near twin-boundary interfaces in FeSe revealed by scanning tunneling spectroscopy. Phys. Rev. X 5, 03 (2015).
13. Cvetkovic, V. & Vafek, O. Space group symmetry, spin-orbit coupling, and the low-energy effective Hamiltonian for iron-based superconductors. Phys. Rev. B 88, 13 (2013).10.1103/PhysRevB.88.134510 ↗
14. Rhodes, L. C., Böker, J., Müller, M. A., Eschrig, M. & Eremin, I. M. Non-local dxy nematicity and the missing electron pocket in FeSe. npj Quantum Mater. 6, 45 (2021).10.1038/s41535-021-00341-6 ↗
15. Arguello, C. J. et al. Quasiparticle interference, quasiparticle interactions, and the origin of the charge density wave in 2H − NbSe2. Phys. Rev. Lett. 114, 03 (2015).10.1103/PhysRevLett.114.037001 ↗
16. da Silva Neto, E. H. et al. Ubiquitous interplay between charge ordering and high-temperature superconductivity in cuprates. Science 343, 393–396 (2014).10.1126/science.1243479 ↗
17. Yim, C. M. et al. Discovery of a strain-stabilised smectic electronic order in LiFeAs. Nat. Commun. 9, 1–7 (2018).10.1038/s41467-018-04909-y ↗
18. Li, W. et al. Stripes developed at the strong limit of nematicity in FeSe film. Nat. Phys. 13, 957–961 (2017).10.1038/nphys4186 ↗
19. Yuan, Y. et al. Incommensurate smectic phase in close proximity to the high-Tc superconductor FeSe/SrTiO3. Nat. Commun. 12, 1–9 (2021).10.1038/s41467-021-22516-2 ↗
20. Zhang, W. et al. Quadrupolar charge dynamics in the nonmagnetic FeSe1−xSx superconductors. Proc. Natl. Acad. Sci. USA 118 (2021).10.1073/pnas.2020585118 ↗
21. Chibani, S. et al. Lattice-shifted nematic quantum critical point in FeSe1−xSx. npj Quantum Mater. 6, 37 (2021).10.1038/s41535-021-00336-3 ↗
22. Hamidian, M. et al. Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state. Nat. Phys. 12, 150–156 (2016).10.1038/nphys3519 ↗
23. Polkovnikov, A., Vojta, M. & Sachdev, S. Pinning of dynamic spin-density-wave fluctuations in cuprate superconductors. Phys. Rev. B 65, 220509 (2002).10.1103/PhysRevB.65.220509 ↗
24. Polkovnikov, A., Sachdev, S. & Vojta, M. Spin collective mode and quasiparticle contributions to STM spectra of d-wave superconductors with pinning. Physica C Supercond 388-389, 19–24 (2003).10.1016/S0921-4534(02)02605-9 ↗
25. Kivelson, S. A. et al. How to detect fluctuating stripes in the high-temperature superconductors. Rev. Mod. Phys. 75, 1201–1241 (2003).10.1103/RevModPhys.75.1201 ↗
26. de’ Medici, L. & Capone, M. Modeling Many-Body Physics with Slave-Spin Mean-Field: Mott and Hund’s Physics in Fe-Superconductors, 115–185 (Springer International Publishing, 2017).10.1007/978-3-319-56117-2_4 ↗
27. Yu, R., Hu, H., Nica, E. M., Zhu, J.-X. & Si, Q. Orbital selectivity in electron correlations and superconducting pairing of iron-based superconductors. Front. Phys. 9, 92 (2021).10.3389/fphy.2021.578347 ↗
28. Yi, M. et al. Observation of temperature-induced crossover to an orbital-selective Mott phase in AxFe2−ySe2 (A = K, Rb) superconductors. Phys. Rev. Lett. 110, 06 (2013).10.1103/PhysRevLett.110.067003 ↗
29. Huang, J. et al. Correlation-driven electronic reconstruction in FeTe1−xSex. Commun. Phys. 5, 29 (2022).10.1038/s42005-022-00805-6 ↗
30. Kostin, A. et al. Imaging orbital-selective quasiparticles in the Hund’s metal state of FeSe. Nat. Mater. 17, 869–874 (2018).10.1038/s41563-018-0151-0 ↗
31. Sprau, P. O. et al. Discovery of orbital-selective Cooper pairing in FeSe. Science 357, 75–80 (2017).10.1126/science.aal1575 ↗
32. Sharma, R. et al. Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination. npj Quantum Mater. 6, 7 (2021).10.1038/s41535-020-00303-4 ↗
33. Villar Arribi, P. & de’ Medici, L. Hund-enhanced electronic compressibility in FeSe and its correlation with Tc. Phys. Rev. Lett. 121, 19 (2018).10.1103/PhysRevLett.121.197001 ↗
34. Reiss, P. et al. Suppression of electronic correlations by chemical pressure from FeSe to FeS. Phys. Rev. B 96, 12 (2017).10.1103/PhysRevB.96.121103 ↗
35. Lahiri, A., Klein, A. & Fernandes, R. M. Defect-induced electronic smectic state at the surface of nematic materials. Phys. Rev. B 106, L14 (2022).10.1103/PhysRevB.106.L140503 ↗
36. Shimojima, T. et al. Discovery of mesoscopic nematicity wave in iron-based superconductors. Science 373, 1122–1125 (2021).10.1126/science.abd6701 ↗
37. Böhmer, A. E., Taufour, V., Straszheim, W. E., Wolf, T. & Canfield, P. C. Variation of transition temperatures and residual resistivity ratio in vapor-grown FeSe. Phys. Rev. B 94, 02 (2016).10.1103/PhysRevB.94.024526 ↗