journal article·2022-01-21Open access

f-electron hybridised Fermi surface in magnetic field-induced metallic YbB12

H. Liu, A. J. Hickey, M. Hartstein, A. J. Davies, A. G. Eaton, T. Elvin, E. Polyakov, T. H. Vu, V. Wichitwechkarn, T. Förster, J. Wosnitza, T. P. Murphy, N. Shitsevalova, M. D. Johannes, M. Ciomaga Hatnean, G. Balakrishnan, G. G. Lonzarich, Suchitra E. Sebastian

npj Quantum Materials· Volume 7· Issue 1

Abstract

Abstract The nature of the Fermi surface observed in the recently discovered family of unconventional insulators starting with SmB6 is a subject of intense inquiry. Here we shed light on this question by accessing quantum oscillations in the high magnetic field-induced metallic regime above ≈47 T in YbB12, which we compare with the unconventional insulating regime. In the field-induced metallic regime, we find prominent quantum oscillations in the electrical resistivity characterised by multiple frequencies and heavy effective masses. The close similarity in Lifshitz-Kosevich low-temperature growth of quantum oscillation amplitude in insulating YbB12 to field-induced metallic YbB12, points to an origin of quantum oscillations in insulating YbB12 from in-gap neutral low energy excitations. Higher frequency Fermi surface sheets of heavy quasiparticle effective mass emerge in the field-induced metallic regime of YbB12 in addition to multiple heavy Fermi surface sheets observed in both insulating and metallic regimes. f-electron hybridisation is thus observed to persist from the unconventional insulating to the field-induced metallic regime of YbB12, in contrast to the unhybridised conduction electron Fermi surface observed in unconventional insulating SmB6. Our findings thus require an alternative model for YbB12, of neutral in-gap low energy excitations, wherein the f-electron hybridisation is retained.
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Research context

OpenAlex topics: Rare-earth and actinide compounds · Iron-based superconductors research · High-pressure geophysics and materials

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References (36)

Show source-provided references
1. Tan, B. S. et al. Unconventional Fermi surface in an insulating state. Science. 349, 287–290 (2015).10.1126/science.aaa7974 ↗
2. Hartstein, M. et al. Fermi surface in the absence of a Fermi liquid in the Kondo insulator SmB6. Nat. Phys. 14, 166–172 (2018).10.1038/nphys4295 ↗
3. Li, G. et al. Two-dimensional Fermi surfaces in Kondo insulator SmB6. Science. 346, 1208–1212 (2014).10.1126/science.1250366 ↗
4. Liu, H. et al. Fermi surfaces in Kondo insulators. J. Phys. Condens. Matter 30, 16LT01 (2018).10.1088/1361-648X/aaa522 ↗
5. Xiang, Z. et al. Quantum oscillations of electrical resistivity in an insulator. Science 362, 65–69 (2018).10.1126/science.aap9607 ↗
6. Wang, P. et al. Landau quantization and highly mobile fermions in an insulator. Nature 589, 225–229 (2021).10.1038/s41586-020-03084-9 ↗
7. Hartstein, M. et al. Intrinsic bulk quantum oscillations in a bulk unconventional insulator SmB6. iScience 23, 101632 (2020).10.1016/j.isci.2020.101632 ↗
8. Sugiyama, K., Iga, F., Kasaya, M., Kasuya, T. & Date, M. Field-induced metallic state in YbB12 under high magnetic field. J. Phys. Soc. Japan 57, 3946–3953 (1988).10.1143/JPSJ.57.3946 ↗
9. Iga, F. et al. Anisotropic magnetoresistance and collapse of the energy gap in Yb1−xLuxB12. J. Phys. Conf. Ser. 200, 012064 (2010).10.1088/1742-6596/200/1/012064 ↗
10. Terashima, T. T. et al. Magnetic-field-induced Kondo metal realized in YbB12. Phys. Rev. Lett. 120, 257206 (2018).10.1103/PhysRevLett.120.257206 ↗
11. Miyake, K. de Haas-van Alphen oscillations in superconducting states as a probe of gap anisotropy. Physica B Condens. Matter 186-188, 115–117 (1993).10.1016/0921-4526(93)90509-5 ↗
12. Knolle, J. & Cooper, N. R. Quantum oscillations without a Fermi surface and the anomalous de Haas-van Alphen effect. Phys. Rev. Lett. 115, 146401 (2015).10.1103/PhysRevLett.115.146401 ↗
13. Riseborough, P. S. & Fisk, Z. Critical examination of quantum oscillations in SmB6. Phys. Rev. B 96, 195122 (2017).10.1103/PhysRevB.96.195122 ↗
14. Peters, R., Yoshida, T. & Kawakami, N. Quantum oscillations in strongly correlated topological Kondo insulators. Phys. Rev. B 100, 085124 (2019).10.1103/PhysRevB.100.085124 ↗
15. Zhang, L., Song, X. Y. & Wang, F. Quantum oscillation in narrow-gap topological insulators. Phys. Rev. Lett. 116, 046404 (2016).10.1103/PhysRevLett.116.046404 ↗
16. Lee, P. A. Quantum oscillations in the activated conductivity in excitonic insulators: possible application to monolayer WTe2. Phys. Rev. B 103, L041101 (2021).10.1103/PhysRevB.103.L041101 ↗
17. Liu, J. & Balents, L. Correlation effects and quantum oscillations in topological nodal-loop semimetals. Phys. Rev. B 95, 075426 (2017).10.1103/PhysRevB.95.075426 ↗
18. Bulaevskii, L. N., Batista, C. D., Mostovoy, M. V. & Khomskii, D. I. Electronic orbital currents and polarization in Mott insulators. Phys. Rev. B 78, 024402 (2008).10.1103/PhysRevB.78.024402 ↗
19. Motrunich, O. I. Orbital magnetic field effects in spin liquid with spinon Fermi sea: possible application to κ-(ET)2Cu2(CN)3. Phys. Rev. B 73, 155115 (2006).10.1103/PhysRevB.73.155115 ↗
20. Baskaran, G. Majorana Fermi sea in insulating SmB6: a proposal and a theory of quantum oscillations in Kondo insulators. Preprint at [https://arxiv.org/abs/1507.03477] (2015).
21. Erten, O., Chang, P. Y., Coleman, P. & Tsvelik, A. M. Skyrme insulators: insulators at the brink of superconductivity. Phys. Rev. Lett. 119, 057603 (2017).10.1103/PhysRevLett.119.057603 ↗
22. Varma, C. M. Majoranas in mixed-valence insulators. Phys. Rev. B 102, 155145 (2020).10.1103/PhysRevB.102.155145 ↗
23. Chowdhury, D., Sodemann, I. & Senthil, T. Mixed-valence insulators with neutral Fermi surfaces. Nat. Commun. 9, 1766 (2018).10.1038/s41467-018-04163-2 ↗
24. Settai, R. et al. Quasi-two-dimensional Fermi surfaces and the de Haas-van Alphen oscillation in both the normal and superconducting mixed states of CeCoIn5. J. Phys. Condens. Matter 13, L627–L634 (2001).10.1088/0953-8984/13/27/103 ↗
25. Hedo, M. et al. Magnetoresistance and de Haas-van Alphen oscillation in normal and superconducting CeRu2. Philos. Mag. B 77, 975–1000 (1998).10.1080/13642819808206399 ↗
26. Inada, Y. et al. Fermi surface and de Haas-van Alphen oscillation in both the normal and superconducting mixed states of UPd2Al3. J. Phys. Soc. Japan 68, 3643–3654 (1999).10.1143/JPSJ.68.3643 ↗
27. Ohkuni, H. et al. Fermi surface properties and de Haas-van Alphen oscillation in both the normal and superconducting mixed states of URu2Si2. Philos. Mag. B 79, 1045–1077 (1999).
28. Clayton, N. J. et al. Superconducting fluctuations and the reduced dimensionality of the organic superconductor κ-(BEDT-TTF)2Cu(NCS)2 as observed through measurements of the de Haas-van Alphen effect. Phys. Rev. B 65, 064515 (2002).10.1103/PhysRevB.65.064515 ↗
29. Werheit, H. et al. Raman scattering and isotopic phonon effects in dodecaborides. J. Phys. Condens. Matter 23, 065403 (2011).10.1088/0953-8984/23/6/065403 ↗
30. Iga, F., Shimizu, N. & Takabatake, T. Single crystal growth and physical properties of Kondo insulator YbB12. J. Magn. Magn. Mater. 177-181, 337–338 (1998).10.1016/S0304-8853(97)00493-9 ↗
31. Altarawneh, M. M., Mielke, C. H. & Brooks, J. S. Proximity detector circuits : an alternative to tunnel diode oscillators for contactless measurements in pulsed magnetic field environments. Rev. Sci. Instrum. 80, 066104 (2009).10.1063/1.3152219 ↗
32. Blaha, P., Schwarz, K., Madsen, G., Kvasnicka, D. & Luitz, J. WIEN2k: an augmented plane wave + local orbitals program for calculating crystal properties. (Vienna University of Technology Institute of Materials Chemistry, Vienna, 2001).
33. Tran, F. & Blaha, P. Accurate band gaps of semiconductors and insulators with a semilocal exchange-correlation potential. Phys. Rev. Lett. 102, 226401 (2009).10.1103/PhysRevLett.102.226401 ↗
34. Anisimov, V. I., Zaanen, J. & Andersen, O. K. Band theory and Mott insulators: Hubbard U instead of Stoner I. Phys. Rev. B 44, 943 (1991).10.1103/PhysRevB.44.943 ↗
35. Shoenberg, D. Magnetic oscillations in metals (Cambridge University Press, Cambridge, UK, 1984).10.1017/CBO9780511897870 ↗
36. Chang, T. R. et al. Two distinct topological phases in the mixed-valence compound YbB6 and its differences from SmB6. Phys. Rev. B 91, 155151 (2015).10.1103/PhysRevB.91.155151 ↗