journal article·2025-03-28Open access

Metastable photo-induced superconductivity far above Tc

Sambuddha Chattopadhyay, Christian J. Eckhardt, Dante M. Kennes, Michael A. Sentef, Dongbin Shin, Angel Rubio, Andrea Cavalleri, Eugene A. Demler, Marios H. Michael

npj Quantum Materials· Volume 10· Issue 1

Abstract

Abstract Inspired by the striking discovery of metastable superconductivity in K3C60 at 100K, far above T c = 20 K, we discuss possible mechanisms for long-lived, photo-induced superconductivity. Starting from a model of optically-driven Raman phonons coupled to inter-band electronic transitions, we develop a microscopic mechanism for photo-controlling the pairing interaction. Leveraging this mechanism, we first investigate long-lived superconductivity arising from the thermodynamic metastable trapping of the driven phonon. We then propose an alternative route, where the superconducting gap created by an optical drive leads to a dynamical bottleneck in the equilibration of quasi-particles. We conclude by discussing the implications of both scenarios for experiments that can be used to discriminate between them. Our work provides falsifiable explanations for the nanosecond-scale photo-induced superconductivity found in K3C60, while simultaneously offering a theoretical basis for exploring metastable superconductivity in other quantum materials.
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Research context

OpenAlex topics: Physics of Superconductivity and Magnetism · Topological Materials and Phenomena · Atomic and Subatomic Physics Research

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