journal article·2023-08-11Open access

Collective magnetic Higgs excitation in a pyrochlore ruthenate

Dirk Wulferding, Junkyoung Kim, Mi Kyung Kim, Yang Yang, Jae Hyuck Lee, Dongjoon Song, Dongjin Oh, Heung-Sik Kim, Li Ern Chern, Yong Baek Kim, Minji Noh, Hyunyong Choi, Sungkyun Choi, Natalia B. Perkins, Changyoung Kim, Seung Ryong Park

npj Quantum Materials· Volume 8· Issue 1

Abstract

Abstract The emergence of scalar Higgs-type amplitude modes in systems where symmetry is spontaneously broken has been a highly successful, paradigmatic description of phase transitions, with implications ranging from high-energy particle physics to low-energy condensed matter systems. Here, we uncover two successive high temperature phase transitions in the pyrochlore magnet Nd2Ru2O7 at TN = 147 K and T* = 97 K, that lead to giant phonon instabilities and culminate in the emergence of a highly coherent excitation. This coherent excitation, distinct from other phonons and from conventional magnetic modes, stabilizes at a low energy of 3 meV. We assign it to a collective Higgs-type amplitude mode, that involves bond energy modulations of the Ru4 tetrahedra. Its striking two-fold symmetry, incompatible with the underlying crystal structure, highlights the possibility of multiple entangled broken symmetries.
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Research context

OpenAlex topics: Advanced Condensed Matter Physics · Physics of Superconductivity and Magnetism · Magnetic and transport properties of perovskites and related materials

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