journal article·2022-01-17Open access

Spatially mapping thermal transport in graphene by an opto-thermal method

Oliver Braun, Roman Furrer, Pascal Butti, Kishan Thodkar, Ivan Shorubalko, Ilaria Zardo, Michel Calame, Mickael L. Perrin

Abstract

Abstract Mapping the thermal transport properties of materials at the nanoscale is of critical importance for optimizing heat conduction in nanoscale devices. Several methods to determine the thermal conductivity of materials have been developed, most of them yielding an average value across the sample, thereby disregarding the role of local variations. Here, we present a method for the spatially resolved assessment of the thermal conductivity of suspended graphene by using a combination of confocal Raman thermometry and a finite-element calculations-based fitting procedure. We demonstrate the working principle of our method by extracting the two-dimensional thermal conductivity map of one pristine suspended single-layer graphene sheet and one irradiated using helium ions. Our method paves the way for spatially resolving the thermal conductivity of other types of layered materials. This is particularly relevant for the design and engineering of nanoscale thermal circuits (e.g. thermal diodes).
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Research context

OpenAlex topics: Thermal properties of materials · Graphene research and applications · Thermal Radiation and Cooling Technologies

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