journal article·2022-08

CoN4 active sites in a graphene matrix for the highly efficient electrocatalysis of CO2 reduction

Hui-nian Zhang, Hui-qi Wang, Su-ping Jia, Qing Chang, Ning Li, Ying Li, Xiao-lin Shi, Zi-yuan Li, Sheng-liang Hu

New Carbon Materials· Volume 37· Issue 4
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Abstract

Developing highly selective, economical and stable catalysts for the electrochemical conversion of CO2 into value-added carbon products to mitigate both CO2 emission and the energy crisis is challenging. We report an efficient and robust electrocatalyst for the CO2 reduction reaction (CO2RR) by embedding CoN4 active sites in a graphene matrix. These highly dispersed CoN4 sites show an extraordinary CO2RR activity, with a high CO Faradaic efficiency of nearly 95% at −0.76 V (vs. RHE) and remarkable durability. The corresponding overpotential is 0.65 V. Our finding could pave the way for the design at the atomic scale of highly efficient electrocatalysts for the CO2RR.
Source: expertdata · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: CO2 Reduction Techniques and Catalysts · Electrocatalysts for Energy Conversion · Advanced Photocatalysis Techniques

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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