journal article·2023-05Open access

Resistance of slurry aluminide coatings on pure nickel under different sulphidizing/Hot corrosion conditions at 700 °C

Benjamin Grégoire, Xabier Montero, Mathias C. Galetz, Gilles Bonnet, Fernando Pedraza

Corrosion Science· Volume 216

Abstract

A water-based slurry aluminide coating was elaborated on high-purity nickel and tested in synthetic air, synthetic air + 0.5 % SO 2/SO 3 and synthetic air + 0.5 % SO 2/SO 3 with sodium sulphate (Na 2SO 4 ) deposit at 700 °C. The developed coating considerably increased the oxidation-sulphidation resistance of nickel in the absence of salt through the formation of thin and adherent alumina scales. In contrast, the presence of sodium sulphate decreased the corrosion resistance. Microstructural investigations indicated that aluminium depletion and the related formation of Ni-rich oxides is mainly responsible for the onset of the corrosion attack following sulphation reaction and fluxing mechanisms.
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Research context

OpenAlex topics: High-Temperature Coating Behaviors · Advanced ceramic materials synthesis · Intermetallics and Advanced Alloy Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (55)

Show source-provided references
1. Hot corrosion of metals and alloys10.1007/s11085-011-9254-6 ↗
2. Young · 2008
3. High-temperature corrosion of superalloys10.1080/02670836.1987.11782259 ↗
4. Common failures in gas turbine blades10.1016/j.engfailanal.2004.07.004 ↗
5. A review on atom probe and correlative microscopy studies of corrosion in nickel-based superalloys10.1557/s43577-022-00366-7 ↗
6. “Saüren” und “Basen” im schmelzfluss: die bestimmung der sauerstoffionen-konzentration
7. The acidic and basic properties of oxides10.3891/acta.chem.scand.01-0592 ↗
8. Synergistic dissolution of oxides in molten sodium sulfate10.1149/1.2086647 ↗
9. Analysis of combined static load and low temperature hot corrosion induced cracking in CMSX-4 at 550 °C10.1016/j.corsci.2019.108293 ↗
10. On the effect of environmental exposure on dwell fatigue performance of a fine-grained nickel-based superalloy10.1007/s11661-018-4752-7 ↗
11. On the hot corrosion of nickel at 700 °C10.1007/s11085-015-9588-6 ↗
12. Mechanisms of hot corrosion of pure nickel at 700 °C: influence of testing conditions10.1016/j.corsci.2018.06.009 ↗
13. Correlations between the kinetics and the mechanisms of hot corrosion of pure nickel at 700 °C10.1016/j.corsci.2019.04.022 ↗
14. A new solid-state mode of hot corrosion at temperatures below 700 °C10.1002/maco.201810751 ↗
15. The influence of iron and cobalt on the Type II hot corrosion behavior of NiCr model alloys10.1002/maco.201911376 ↗
16. Compositional factors affecting protective alumina formation under type II hot corrosion conditions10.1007/s11085-013-9410-2 ↗
17. Reaction morphologies developed by nickel aluminides in type II hot corrosion conditions: the effect of chromium10.1016/j.corsci.2015.08.029 ↗
18. Influence of gaseous atmosphere on electrochemical behavior of nickel alloys in LiCl-KCl-Na2SO4 at 700 °C10.1016/j.corsci.2018.05.039 ↗
19. M. Zahiri Azar, Early Stage Hot Corrosion Behavior of Pt/Cr-Modified β-NiAl Alloys at 700 °C (Electronic Thesis or Dissertation), Case Western Reserve University, 2015. Retrieved from 〈https://etd.ohiolink.edu〉.
20. Initial stages of Na2SO4-induced degradation of β-Ni-36Al at 700 °C: i-intrinsic behavior10.1007/s11085-017-9760-2 ↗
21. Sodium sulfate–diatomite composite materials for high temperature thermal energy storage10.1016/j.powtec.2014.08.075 ↗
22. Preparation and characterization of sodium sulfate/silica composite as a shape-stabilized phase change material by sol-gel method10.1016/S1004-9541(14)60047-1 ↗
23. Designing oxidation-resistant coatings10.1007/s11837-000-0112-2 ↗
24. Microstructural and microchemical development of simple and Pt-modified aluminide diffusion coatings during long term oxidation at 1050 °C10.1016/S0257-8972(03)00767-9 ↗
25. Environmental resistance of pure and alloyed γ’-Ni3Al and β-NiAl10.5006/0010-9312-32.12.476 ↗
26. The influence of reducing conditions on the sodium sulfate-induced corrosion of pure and alloyed β-NiAl10.1016/0010-938X(85)90040-X ↗
27. Mécanismes de corrosion à chaud de revêtements d’aluminures type Ni-Al en conditions aéronautiques10.1016/0025-5416(87)90396-X ↗
28. Mechanisms of formation of slurry aluminide coatings from Al and Cr microparticles10.1016/j.surfcoat.2018.11.077 ↗
29. I.S.O. International Standard, Corrosion of metals and alloys – test method for high temperature corrosion testing of metallic materials by application of a deposit of salt, ash, or other substances, 2015, 17224.
30. I.S.O. International Standard, Corrosion of metals and alloys – test method for high temperature corrosion testing of metallic materials by immersing in molten salt or other liquids under static conditions, 2015, 17245.
31. Reinterpretation of type II hot corrosion of Co-base alloys incorporating synergistic fluxing10.1007/s11085-018-9853-6 ↗
32. The effect of manganese and silicon additions on the corrosion resistance of a polycrystalline nickel-based superalloy10.1016/j.corsci.2020.109042 ↗
33. Long-term exposure of austenitic steels and nickel-based alloys in lignite-biomass cofiring10.1002/maco.201911109 ↗
34. Corrosion mechanisms of ferritic-martensitic P91 steel and Inconel 600 nickel-based alloy in molten chlorides. Part I: NaCl-KCl binary system10.1016/j.solmat.2020.110659 ↗
35. Microstructural study of the theta-alpha transformation in alumina scales formed on nickel-aluminides10.1179/mht.2000.011 ↗
36. An X-ray analysis of the nickel-aluminium system
37. Optical constants of β-phase NiAl10.1063/1.1710060 ↗
38. Peña-Álvareza · RSC Adv. · 2016 · 6 · 4954310.1039/C5RA27162B ↗
39. Effect of water drops on the oxidation mechanisms of a ceria coated nickel-based superalloy10.1016/j.corsci.2012.11.010 ↗
40. Novel strategies for evaluating the degradation of protective coatings on superalloys10.1016/S1466-6049(99)00047-1 ↗
41. γ-Al2O3 thin film formation via oxidation of β-NiAl(110)10.1016/j.actamat.2011.05.064 ↗
42. The formation of aluminium oxide scales on high-temperature alloys10.1007/BF00666913 ↗
43. The oxidation behaviour of NiAl – I. Phase transformations in the alumina scale during oxidation of NiAl and NiAl-Cr alloys10.1016/0010-938X(92)90002-K ↗
44. Oxidation of NiAl and FeAl10.1016/S0966-9795(99)00037-0 ↗
45. The oxidation of NiAl – III. Internal and intergranular oxidation10.1016/0010-938X(94)90107-4 ↗
46. Corrosion behavior of stainless and low-chromium steels and IN625 in molten nitrate salts at 600 °C10.1016/j.solmat.2015.08.011 ↗
47. Catalytic reduction of sodium sulfate10.1021/ie50452a019 ↗
48. Sulfate-induced hot corrosion of nickel10.1007/BF00656835 ↗
49. A.K. Misra, D.P. Whittle, W.L. Worrell, Thermodynamics of Low-temperature (700–850 °C) Hot Corrosion, University of North Texas Libraries, UNT Digital Library, Berkeley, California, 1980. 〈(https://digital.library.unt.edu/ark:/67531/metadc838340/〉: Accessed 5 March 2021).
50. Accelerated oxidation, internal oxidation, intergranular oxidation, and pesting of intermetallic compounds10.1007/BF01046726 ↗
51. The influence of sulfides on the oxidation behavior of nickel-base alloys10.1007/BF03037874 ↗
52. Type-I hot corrosion of Ni-base superalloy CM247LC in presence of molten Na2SO4 film10.1007/s11661-020-06068-6 ↗
53. The oxidation of NiAl10.1002/maco.19960471203 ↗
54. Hot corrosion of materials: fundamental studies10.1007/BF03222665 ↗
55. The corrosion of Ni in O2 + SO2 atmospheres in the temperature range 500–750 °C10.1016/S0010-938X(69)80047-8 ↗