journal article·2024-05

Nano-structure and hydrophobicity co-determined barrier properties of corrosion protective ZnAl-LDH film in atmospheric environment

Han Zhang, Wen Sun, Lida Wang, Yixuan Feng, Shiheng Ma, Liqiu Zhao, Guichang Liu

Corrosion Science· Volume 232
Publisher page

Abstract

Salt spray is prone to convert superhydrophobic surface from Cassie-Baxter state to Wenzel state, which accelerates the metallic corrosion. Herein, corrosion process of superhydrophobic coatings were investigated by in-situ growth of LDH lamellae with different platelet spacing and modification of stearic acid. The corrosion protection mechanism of the superhydrophobic coating divided into two stages: the well-known air film blocking effect and the hydrophobicity-depended barrier performance, which is a new focus. Through investigating the influences of the nano-structure on corrosion protection via experiments and simulation, a new mechanism on corrosion protection failure of superhydrophobic surfaces in atmospheric environment is proposed.
Source: expertdata · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Surface Modification and Superhydrophobicity · Aerogels and thermal insulation · High voltage insulation and dielectric phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (45)

Show source-provided references
1. Design of robust superhydrophobic surfaces10.1038/s41586-020-2331-8 ↗
2. Comparison of barrier properties for a superhydrophobic epoxy coating under different simulated corrosion environments10.1016/j.corsci.2015.11.023 ↗
3. Advantage of super-hydrophobic surface as a barrier against atmospheric corrosion induced by salt deliquescence10.1016/j.corsci.2014.09.001 ↗
4. Long-lived superhydrophobic surfaces10.1039/c2ta01073a ↗
5. The lowest surface free energy based on −CF3 alignment10.1021/la981727s ↗
6. Surface characteristics and wettability of superhydrophobic silanized inorganic glass coating surfaces textured with a picosecond laser10.1016/j.apsusc.2020.147808 ↗
7. Durable superhydrophobic surface prepared by designing "micro-eggshell" and "web-like" structures10.1016/j.cej.2019.123741 ↗
8. Aerosol size distribution transformation in fog10.1016/1352-2310(94)90238-0 ↗
9. Chemical modification of hydrotalcite coating for enhanced corrosion resistance10.1016/j.corsci.2015.01.033 ↗
10. Enhanced corrosion resistance of superhydrophobic layered double hydroxide films with long-term stability on Al substrate10.1021/acsami.8b02280 ↗
11. Corrosion resistance of superhydrophobic Mg-Al layered double hydroxide coatings on aluminum alloys10.1007/s40195-015-0335-4 ↗
12. Corrosion resistance of superhydrophobic layered double hydroxide films on aluminum10.1002/anie.200704694 ↗
13. A facile approach to superhydrophobic LiAl-layered double hydroxide film on Al-Li alloy substrate10.1007/s11998-015-9660-9 ↗
14. A mechanically and chemically stable superhydrophobic coating for preventing marine atmospheric corrosion10.1016/j.surfin.2021.101537 ↗
15. A novel two-component self-healing coating comprising vinyl ester resin-filled microcapsules with prolonged anticorrosion performance10.1016/j.porgcoat.2021.106220 ↗
16. Structural arrangement and properties of layered double hydroxide drug nanocarrier intercalated by sulindac and mefenamic acid solved by molecular simulation methods10.1016/j.clay.2020.105560 ↗
17. Fabrication of inhibitor anion-intercalated layered double hydroxide host films on aluminum alloy 2024 and their anticorrosion properties10.1007/s11998-014-9644-1 ↗
18. Preventing the Cassie−Wenzel transition using surfaces with noncommunicating roughness elements10.1021/la803691m ↗
19. Layered double hydroxide interfaced stearic acid - cellulose fibres: a new class of super-hydrophobic hybrid materials10.1016/j.colsurfa.2017.03.025 ↗
20. Comparison and characterization of chemical surfactants and bio-surfactants intercalated with layered double hydroxides (LDHs) for removing naphthalene from contaminated aqueous solutions10.1016/j.colsurfa.2010.06.009 ↗
21. Nitrate-intercalated layered double hydroxides structure model, order, and disorder10.1002/ejic.201201405 ↗
22. One-pot microwave-assisted synthesis of graphene/layered double hydroxide (LDH) nanohybrids10.1007/s40820-015-0047-3 ↗
23. Enhanced corrosion protection by Al surface immobilization of in-situ grown layered double hydroxide films co-intercalated with inhibitors and low surface energy species10.1016/j.corsci.2019.108340 ↗
24. Oriented CuZnAl ternary layered double hydroxide films: in situ hydrothermal growth and anticorrosion properties10.1021/ie403299u ↗
25. Layered double hydroxide interfaced stearic acid – cellulose fibres: a new class of super-hydrophobic hybrid materials10.1016/j.colsurfa.2017.03.025 ↗
26. Spectroscopic, microscopic, X-ray diffraction and thermal stability studies of stearic acid modified hydrotalcite formed through memory effect10.1002/masy.202000277 ↗
27. Superior adsorptive removal of eco-toxic drug diclofenac sodium by Zn–Al LDH⋅xBi2O3 layer double hydroxide composites10.1016/j.clay.2021.106119 ↗
28. Facile fabrication of superhydrophobic surface with micro/nanoscale binary structures on aluminum substrate10.1016/j.apsusc.2011.01.114 ↗
29. A novel approach to fabricate protective layered double hydroxide films on the surface of anodized Mg-Al alloy10.1002/admi.201700163 ↗
30. Inhibiting the corrosion-promotion activity of graphene10.1021/cm5043099 ↗
31. S. Dasgupta, Controlled release of ibuprofen using Mg Al LDH nano carrier, in: Proceedings of the International Conference on Materials, Alloys and Experimental Mechanics (Icmaem-2017), vol. 225, 2017, 012005.10.1088/1757-899X/225/1/012005 ↗
32. Mechanically robust superhydrophobic steel surface with anti-icing, UV-durability, and corrosion resistance properties10.1021/acsami.5b00558 ↗
33. Chemically stable and mechanically durable superamphiphobic aluminum surface with a micro/nanoscale binary structure10.1021/am503441x ↗
34. Fabrication of superhydrophobic marigold shape LDH films on stainless steel meshes via in-situ growth for enhanced anti-corrosion and high efficiency oil-water separation10.1016/j.clay.2019.105292 ↗
35. Superhydrophobic double layered MgAl-LDH/epoxy composite coatings for enhanced anticorrosion performance of magnesium alloys
36. A protective superhydrophobic Mg–Zn–Al LDH film on surface-alloyed magnesium10.1016/j.jallcom.2020.157550 ↗
37. Fabrication of durability superhydrophobic LDH coating on zinc sheet surface via NH4F-assisted in-situ growth and post-modification for enhancing anti-corrosion and anti-icing10.1016/j.clay.2019.105182 ↗
38. Fast healable superhydrophobic material10.1021/acsami.9b07563 ↗
39. Super-hydrophobic film fabricated on aluminium surface as a barrier to atmospheric corrosion in a marine environment10.1016/j.corsci.2014.11.029 ↗
40. Fabrication of host–guest UV-blocking materials by intercalation of fluorescent anions into layered double hydroxides10.1039/C5RA00589B ↗
41. UV blocking by Mg–Zn–Al layered double hydroxides for the protection of asphalt road surfaces10.1021/ie403901n ↗
42. The microstructure evolution and electrochemical corrosion behavior of 7A46 aluminum alloy in different quenching conditions10.3390/ma15020477 ↗
43. Pitting corrosion of aluminum10.1016/S0010-938X(99)00012-8 ↗
44. Effects of pH and chloride concentration on pitting corrosion of AA6061 aluminum alloy10.1016/j.corsci.2008.03.006 ↗
45. A chemically robust and self-healing superhydrophobic polybenzoxazine coating without fluorocarbon resin modification: fabrication and failure mechanism