Improvement of gamma and fast neutron shielding behavior in new ceramic by adding Ho2O3 and Eu2O3: experimental and theoretical studies
Source abstract
Abstract
This study is about improving the shielding performance of new types of ceramics produced by adding Ho2O3 (Holmium(III) Oxide) and Eu2O3 (Europium(III) Oxide) to ceramic bodies against nuclear radiation, namely neutrons and photons. Within the scope of the study, photon intensities (I and I-0) emitted by Barium-133 radioisotope were measured experimentally at different energies (81, 160, 223, 302, 356 and 383 keV). Using the obtained results, mass attenuation coefficient (mu rho), linear attenuation coefficient (mu, cm(-)1), half-value thickness (Delta(0).(5)), mean free path (lambda), effective atomic numbers (Zeff) and electron densities (Nel) were derived. Experimental results were compared with theoretical values obtained from the EpiXS program. Equivalent Absorbed Dose (EAD) values characterizing the experimental shielding properties of fast neutrons were measured using BF3 gas proportional neutron detector and 241Am/Be neutron source. Theoretically fast neutron shielding parameters (Sigma R) were also calculated. It is concluded that doping of ceramic bodies with Ho2O3 and Eu2O3 increases both photon and neutron shielding performance. Experimental results demonstrate the potential of these doped ceramics as effective materials for radiation shielding and the possibility of tailoring their performance by adjusting the doping concentrations. It is thought that the data obtained as a result of this research will be very important for applications in nuclear reactors, medical radiation protection and various high radiation environments.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Radiation Shielding Materials Analysis · Nuclear materials and radiation effects · Nuclear Physics and Applications
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (20)
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1. Alomayrah, N., Al-Buriahi, M.S.: Optical properties, gamma attenuation and fast neutrons moderating performance of V2O5–Bi2O3–B2O3–PbO glasses. J. Aust. Ceram. Soc. (2024). https://doi.org/10.1007/s41779-024-01122-710.1007/s41779-024-01122-7 ↗
2. Alsaif, N.A., Olarinoye, I.O., Rammah, Y.S.: The role of Titania on gamma and neutron attenuation competence of sodium lead borosilicate glasses. J. Aust. Ceram. Soc. 58, 939–947 (2022)10.1007/s41779-022-00749-8 ↗
3. Hannachi, E., Sayyed, M.I., Slimani, Y., Elsafi, M.: Gamma radiation shielding efficiency of some different ceramic composites: A comparative study. Radiat. Phys. Chem. 220, 111695 (2024)10.1016/j.radphyschem.2024.111695 ↗
4. Mhareb, M.H.A.: Optical, Structural, Radiation shielding, and Mechanical properties for borosilicate glass and glass ceramics doped with Gd2O3. Ceram. Int. 49(22), 36950–36961 (2023)10.1016/j.ceramint.2023.09.026 ↗
5. Hannachi, E., Sayyed, M.I., Slimani, Y., Almessiere, M.A., Baykal, A., Elsafi, M.: Structure and radiation-shielding characteristics of BTO/MnZnFeO ceramic composites. J. Phys. Chem. Solids 174, 111132 (2023)10.1016/j.jpcs.2022.111132 ↗
6. Oto, B., Çakar, N., Kavaz, E., Madak, Z.: An experimental study on gamma radiation attenuation effectiveness of magnetite and serpentine doped ceramics. Progress in Nuclear Energy 169, 105079 (2024)10.1016/j.pnucene.2024.105079 ↗
7. Kavaz, E., Oto, B., Durak, H., Madak, Z.: Improving the performance of nuclear protection of Al2Si2O5(OH)4–KAlSi3O8–SiO2 ceramics with cobalt insertion: an experimental study. J. Aust. Ceram. Soc. 56, 1595–1607 (2020)10.1007/s41779-020-00503-y ↗
8. Oto, B., Kavaz, E., Durak, H., Aras, A., Madak, Z.: Effect of addition of molybdenum on photon and fast neutron radiation shielding properties in ceramics. Ceram. Int. 45(17), 23681–23689 (2019)10.1016/j.ceramint.2019.08.082 ↗
9. Alafer, F., Sallam, F.H., Al Meshari, M., Alzamil, Y., Abanomy, A., Alhujaili, S., El-Taher, A.: The influence of thermal treatment on the structural properties and gamma rays shielding of bentonite clay ceramic. Radiat. Phys. Chem. 217, 111531 (2024)10.1016/j.radphyschem.2024.111531 ↗
10. Alhindawy, I.G., Marashdeh, M.W., Aljaafreh, M.J., Al-Hmoud, M., Alanazi, S., Mahmoud, K.: Advanced radiation shielding materials: PbO2-doped zirconi a ceramics synthesized through innovative sol-gel method. Nuclear Engineering and Technology 56(7), 2444–2451 (2024)10.1016/j.net.2024.02.001 ↗
11. Şahin, M.C., Kayhan, M., Kayhan, E.: Assessment of Radiation absorption parameters of lithium disilicate glass-ceramic used in dentistry: experimental and theoretical approaches. J. Aust. Ceram. Soc. 61(2), 361–369 (2025)10.1007/s41779-025-01157-4 ↗
12. Madak, Z., Oto, B., Kavaz, E., Çakar, N.: Improvement of nuclear photon and neutron shielding performance of Tm2O3 and Dy2O3 doped ceramics: An experimental study. Radiat. Phys. Chem. 217, 111516 (2024)10.1016/j.radphyschem.2024.111516 ↗
13. Abdelghany, A.M., El-Batal, H.A., EzzEl-Din, F.M., ElAlialy, N., Okasha, A., Atta, D., Ismai, A.M., Abdelbaky, M., Aboelwafa, M.A., Awad, W.: Structural and gamma-ray attenuation of mixed former lead-free borophosphate glasses. Rad. Phys. Chem. 214, 111276 (2024)10.1016/j.radphyschem.2023.111276 ↗
14. Pulit-Prociak, J., Staroń, A., Prokopowicz, M., Magielska, K., Banach, M.: Analysis of antimicrobial properties of PVA-based coatings with silver and zinc oxide nanoparticles. Journal of Inorganic and Organometallic Polymers and Materials 31, 2306–2318 (2021)10.1007/s10904-020-01838-6 ↗
15. Abdelghany, A.M., Alsaif, N.A., Madshal, M.A., ElBatal, H.A., Rammah, Y.S., Awad, W.: Structural, optical and radiation shielding parameters of sodium aluminium borate glasses modified with chromium oxide. Radiat. Phys. Chem. 207, 110861 (2023)10.1016/j.radphyschem.2023.110861 ↗
16. Manohara, S.R., Hanagodimath, S.M., Gerward, L.: The effective atomic numbers of some biomolecules calculated by two methods: a comparative study. Med. Phys. 36(1), 137–141 (2009)10.1118/1.3030952 ↗
17. Hila, F.C., Amorsolo, A.V., Jr., Javier-Hila, A.M.V., Guillermo, N.R.D.: A simple spreadsheet program for calculating mass attenuation coefficients and shielding parameters based on EPICS2017 and EPDL97 photoatomic libraries. Radiat. Phys. Chem. 177, 109122 (2020)10.1016/j.radphyschem.2020.109122 ↗
18. Hila, F.C., Asuncion-Astronomo, A., Dingle, C.A.M., Jecong, J.F.M., Javier-Hila, A.M.V., Gili, M.B.Z., Amorsolo, A.V., Jr.: EpiXS: A windows-based program for photon attenuation, dosimetry and shielding based on EPICS2017 (ENDF/B-VIII) and EPDL97 (ENDF/B-VI. 8). Radiat. Phys. Chem. 182, 109331 (2021)10.1016/j.radphyschem.2020.109331 ↗
19. Kaplan, M.F.: Concrete radiation shielding. Wiley, New York (1989)
20. Sayyed, M.I.: Half value layer, mean free path and exposure buildup factor for tellurite glasses with different oxide compositions. J. Alloys. Compd. 395, 3191–3197 (2017)10.1016/j.jallcom.2016.11.318 ↗