journal article·2025-10-26Open access

Microfluidic Edible Coatings: Multiphase VOF Modeling, Physicochemical Properties, Image Analysis, and Applications in Fried Foods

Cristian Aarón Dávalos-Saucedo, Giovanna Rossi-Márquez, Sergio Rodríguez-Miranda, Carlos E. Castañeda

Coatings· Volume 15· Issue 11

Abstract

Edible coatings are widely used to modulate oil uptake and moisture in fried foods. In this study, we evaluated a microfluid-assisted flow-blurring spray against conventional application by dipping/spraying, focusing on the coating efficiency and preliminary implications for sustainable process. This study combines benchtop experiments with a near-nozzle numerical analysis where the gas–liquid interface and primary breakup are modeled using the Volume of Fluid (VOF) approach implemented in OpenFOAM, configured for a flow-blurring geometry to generate whey protein isolate (WPI) coatings. Viscosity, density, solid content, and contact angle were validated experimentally and used in the simulation setup. An image-based droplet pipeline quantified spray characteristics, yielding a volumetric median diameter D50 = 83.69 µm and confirming process uniformity. Contact angles showed marked substrate dependence: hydrophilic surfaces, 68°–85°; hydrophobic surfaces, 95°–110°. For turkey sausages, sessile-drop contact angles were not determinable (N.D.) due to wicking/roughness; wettability was therefore assessed on smooth surrogates and via performance metrics. Fit-for-purpose simulation procedures are outlined. Microfluidic application (WPI-McF) lowered oil uptake versus uncoated controls. Together, robust modeling, targeted image analytics, and high-precision microfluidics enable rational tuning of coating microstructure and barrier performance, offering a scalable pathway to reduce lipid content and enhance fried food quality.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Microencapsulation and Drying Processes · Surface Modification and Superhydrophobicity · Fluid Dynamics and Heat Transfer

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Tecnológico Nacional de México, Instituto Tecnológico “José Mario Molina Pasquel y Henríquez”, Unidad Académica Lagos de Moreno, Lagos de Moreno C.P. 47480, Jalisco, México

Centro Universitario de los Lagos, Universidad de Guadalajara, Lagos de Moreno C.P. 47460, Jalisco, Mexico

References (55)

Show source-provided references
1. Rossi-Márquez, G., Dávalos-Saucedo, C.A., and Di Pierro, P. (2023). Edible Films and Coatings Applied in the Food Industry. Coatings, 13.10.3390/coatings13040670 ↗
2. Advances in Edible Coatings for Fresh Fruits and Vegetables: A Review10.1080/10408398.2010.541568 ↗
3. Optimization of Deep-Fat Frying Operations10.1016/0924-2244(91)90659-7 ↗
4. A Review of Factors Affecting Fat Absorption in Hot Chips10.1080/20014091091788 ↗
5. Oil Uptake during Deep-Fat Frying: Factors and Mechanism
6. Edible Films and Coatings: Structures, Active Functions and Trends in Their Use10.1016/j.tifs.2011.02.004 ↗
7. Talens, P., Pérez-Masia, R., Jiménez, A., Fabra, M.J., and Chiralt, A. (2010, January 25–29). Use of Edible Films to Control Moisture Migration in Multicomponent Food Systems. Proceedings of the International Conference of Food Innovation (FoodInnova 2010), Valencia, Spain.
8. Application of Transglutaminase-Crosslinked Whey Protein/Pectin Films as Water Barrier Coatings in Fried and Baked Foods10.1007/s11947-012-1045-9 ↗
9. Functional Materials for Health Care and Pharmacy from Microfluidic Principles and Flow Focusing10.1016/j.addr.2013.08.003 ↗
10. Microfluidic Emulsification in Food Processing10.1016/j.jfoodeng.2014.09.021 ↗
11. Computational Fluid Dynamics (CFD)—An Effective and Efficient Design and Analysis Tool for the Food Industry: A Review10.1016/j.tifs.2006.05.004 ↗
12. A Coupled VOF/Embedded Boundary Method to Model Two-Phase Flows on Arbitrary Solid Surfaces10.1016/j.compfluid.2024.106317 ↗
13. Applications of Microfluidic Devices in Food Engineering10.1007/s11483-007-9043-6 ↗
14. Association of Official Analytical Chemists (1990). AOAC Method 950.46. Official Methods of Analysis, AOAC International.
15. NIH Image to ImageJ: 25 Years of Image Analysis10.1038/nmeth.2089 ↗
16. A Snake-Based Approach to Accurate Determination of Both Contact Points and Contact Angles10.1016/j.colsurfa.2006.03.008 ↗
17. Study on Imaging Method for Measuring Droplet Size in Large Sprays10.1016/j.partic.2014.12.003 ↗
18. Image Illumination Adaptive Correction Algorithm Based on a Combined Model of Bottom-Hat and Improved Gamma Transformation10.1007/s13369-022-07368-2 ↗
19. A Threshold Selection Method from Gray-Level Histograms10.1109/TSMC.1979.4310076 ↗
20. Automatic Thresholding for Defect Detection10.1016/j.patrec.2006.03.009 ↗
22. Gaussian-Based Edge-Detection Methods-a Survey10.1109/TSMCC.2002.804448 ↗
23. Dhar, R., Gupta, R., and Baishnab, K.L. (2014, January 6–8). An Analysis of CANNY and LAPLACIAN of GAUSSIAN Image Filters in Regard to Evaluating Retinal Image. Proceedings of the 2014 International Conference on Green Computing Communication and Electrical Engineering (ICGCCEE), Coimbatore, India.10.1109/ICGCCEE.2014.6922270 ↗
24. Twisted Fiber Microfluidics: A Cutting-Edge Approach to 3D Spiral Devices10.1038/s41378-023-00642-9 ↗
25. Azzini, F., Pulvirenti, B., Rossi, M., and Morini, G.L. (2024). Squeezing Droplet Formation in a Flow-Focusing Micro Cross-Junction. Micromachines, 15.10.20944/preprints202401.1676.v1 ↗
26. Pinch-off Dynamics of Droplet Formation in Microchannel Flow10.1016/j.ces.2023.119296 ↗
27. Okagaki, Y., Yonomoto, T., Ishigaki, M., and Hirose, Y. (2021). Numerical Study on an Interface Compression Method for the Volume of Fluid Approach. Fluids, 6.10.3390/fluids6020080 ↗
28. Breakup of Planar Liquid Sheets Injected at High Speed in a Quiescent Gas Environment10.1017/jfm.2023.843 ↗
29. A Hybrid Continuum Surface Tension Force for the Three-Phase VOF Method10.1016/j.jcp.2024.112872 ↗
30. On Wind–Wave Interaction Phenomena at Low Reynolds Numbers10.1017/jfm.2023.4 ↗
31. The IAPWS Formulation 1995 for the Thermodynamic Properties of Ordinary Water Substance for General and Scientific Use10.1063/1.1461829 ↗
32. New International Formulation for the Viscosity of H2O10.1063/1.3088050 ↗
33. Petrova, T., and Dooley, R.B. (2014, January 22–27). Revised Release on Surface Tension of Ordinary Water Substance. Proceedings of the International Association for the Properties of Water and Steam, Moscow, Russia.
34. Numerical Investigation of Droplet Generation Within a Microfluidic T-Junction With Semicylindrical Obstacle10.1115/1.4055177 ↗
35. Modeling of Two-Phase Flows at Low Capillary Number with VoF Method10.1016/j.compfluid.2022.105772 ↗
36. Laín, S., Lozano-Parada, J.H., and Guzmán, J. (2022). Computational Characterization of Turbulent Flow in a Microfluidic Actuator. Appl. Sci., 12.10.3390/app12073589 ↗
37. On Floating Point Precision in Computational Fluid Dynamics Using OpenFOAM10.1016/j.future.2023.10.006 ↗
38. Towards a Platform-Portable Linear Algebra Backend for OpenFOAM10.1007/s11012-024-01806-1 ↗
39. Piscaglia, F., and Ghioldi, F. (2023). GPU Acceleration of CFD Simulations in OpenFOAM. Aerospace, 10.10.3390/aerospace10090792 ↗
40. Effects of Microbial Polysaccharides on the Oil Absorption and Quality Characteristics of a Deep-Fried Snack Namkeen10.1002/ejlt.202000404 ↗
41. Edge Detection Techniques For Image Segmentation
42. Schlieren Image Velocimetry of Swirl Sprays10.1007/s10494-022-00385-z ↗
43. Athanasopoulou, E., Bigi, F., Maurizzi, E., Karellou, E.I.E., Pappas, C.S., Quartieri, A., and Tsironi, T. (2024). Synthesis and Characterization of Polysaccharide- and Protein-Based Edible Films and Application as Packaging Materials for Fresh Fish Fillets. Sci. Rep., 14.10.1038/s41598-024-51163-y ↗
44. Yashwant, A.S., Kashyap, P., and Goksen, G. (2023). Recent Advances in the Improvement of Protein-Based Edible Films through Non-Thermal and Thermal Techniques. Food Biosci., 55.10.1016/j.fbio.2023.103032 ↗
45. Large Area Optical Mapping of Surface Contact Angle10.1364/OE.25.021127 ↗
46. Lößlein, S.M., Merz, R., Müller, D.W., Kopnarski, M., and Mücklich, F. (2022). An In-Depth Evaluation of Sample and Measurement Induced Influences on Static Contact Angle Measurements. Sci. Rep., 12.10.1038/s41598-022-23341-3 ↗
47. Ponomar, M., Krasnyuk, E., Butylskii, D., Nikonenko, V., Wang, Y., Jiang, C., Xu, T., and Pismenskaya, N. (2022). Sessile Drop Method: Critical Analysis and Optimization for Measuring the Contact Angle of an Ion-Exchange Membrane Surface. Membranes, 12.10.3390/membranes12080765 ↗
48. An Experimental Investigation of Oil-Water Flow in a Serpentine Channel10.1016/j.ijmultiphaseflow.2020.103327 ↗
49. Contact Angle Measurements: From Existing Methods to an Open-Source Tool10.1016/j.cis.2021.102470 ↗
50. A Computational Study of a Two-Fluid Atomizing Coaxial Jet: Validation against Experimental Back-Lit Imaging and Radiography and the Influence of Gas Velocity and Contact Line Model10.1016/j.ijmultiphaseflow.2023.104520 ↗
51. A comparative study of direct numerical simulation and experimental results on a prefilming airblast atomization configuration10.1615/AtomizSpr.2021037399 ↗
52. Air-Blast Atomization of a Liquid Film10.1017/jfm.2024.279 ↗
53. Chen, S., Zhang, Y., Wu, Z., Fang, G., Chen, Y., and Duan, J. (2025). Near-Nozzle Atomization Characteristics in Air-Assisted Spraying: Integrated VOF-DPM Modeling and Experimental Validation. Coatings, 15.10.3390/coatings15080939 ↗
54. A Computational Methodology to Account for the Liquid Film Thickness Evolution in Direct Numerical Simulation of Prefilming Airblast Atomization10.1016/j.ijmultiphaseflow.2023.104403 ↗
55. Numerical Analysis of the Airflow Field and Experiments of Fiber Motion for Solution Blowing10.1021/acsomega.3c09876 ↗