journal article·2023-09-26Open access

Corrosion Behavior in Saline Solution of Electrodeposited Nanocomposite Zn-CeO2 Coatings Deposited onto Low Alloyed Steel

Loïc Exbrayat, Christelle Rébéré, Rémy Milet, Emilie Calvié, Philippe Steyer, Juan Creus

Coatings· Volume 13· Issue 10

Abstract

Zn-CeO2 nanocomposite coatings were deposited onto mild steel substrates by electrodeposition process. Our study highlights the effect of ceria nanoparticles embedded into a metallic matrix on the corrosion behavior in saline environment. The experimental results show that the ceria incorporation and dispersion depend on the particles concentration in the electrolyte. High concentrations of particles favor agglomeration and adsorption of agglomerates on the surface of the zinc coating. A slight improvement of the corrosion resistance compared to pure electrodeposited zinc coatings is observed. The beneficial effect seems to be dependent on the dispersion of the nanoparticles embedded inside the mela matrix. The distribution of nanoparticles seems to be the key-parameter influencing the corrosion behavior, permitting to improve the corrosion behavior during extended immersion test.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Electrodeposition and Electroless Coatings · Corrosion Behavior and Inhibition · ZnO doping and properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

SafranTech, Rue des Jeunes Bois, 78772 Magny Les Hameaux, France

LaSIE UMR 7356 CNRS, La Rochelle Université, Av. Michel Crépeau, 17042 La Rochelle, France

LaSALYS, 1 av. du Champ de Mars, 45100 Orléans, France

Ahlstrom Research Center, 38140 Apprieu, France

MATEIS, INSA Lyon, 21 av. Jean Capelle, 69621 Villeurbanne cedex, France

Funding

Agence Nationale de la Recherche

References (75)

Show source-provided references
1. The role of texture and morphology in optimizing the corrosion resistance of zinc-based electrogalvanized coatings10.1016/S0010-938X(97)00148-0 ↗
2. Landner, L., and Reuther, R. (2004). Metals in Society and in the Environment: A Critical Review of Current Knowledge on Fluxes, Speciation, Bioavailability and Risk for Adverse Effects of Copper, Chromium, Nickel and Zinc, Springer.
3. The european union risk assessment on zinc and zinc compounds: The process and the facts10.1002/ieam.5630010401 ↗
4. Corrosion behavior of zinc-nickel coatings, electrodeposited on steel10.1016/S0257-8972(99)00455-7 ↗
5. Alternative technologies and coatings for electroplated cadmium and hard chromium10.5589/q11-001 ↗
6. Properties of Zn-Ni alloy deposits from ammonium baths10.1007/BF00249889 ↗
7. Electrodeposition of Zn-Mn alloys at low current densities10.1149/1.1512668 ↗
8. Electrodeposition of Zn-Mn alloys on steel using an alkaline pyrophosphate-based electrolytic bath10.1016/j.surfcoat.2004.11.020 ↗
9. Zn-Fe electrodeposition from chloride bath: Influence of deposition parameters on coatings morphology and structure10.1002/maco.201106290 ↗
10. Optimization of the morphology, structure and properties of high iron content Zn-Fe coatings by pulse electrodeposition10.1016/j.matchemphys.2021.124366 ↗
11. Electrodeposition of composite coatings containing nanoparticles in a metal deposit10.1016/j.surfcoat.2005.11.123 ↗
12. Ahmadkhaniha, D., and Zanella, C. (2019). The effects of additives, particles load and current density on codeposition of SiC particles in NiP nanocomposite coatings. Coatings, 9.10.3390/coatings9090554 ↗
13. Studies on the Stability of Zn and Zn – TiO2 Nanocomposite Coatings Prepared by Pulse Reverse Current10.1149/1.3531949 ↗
14. Zn composite corrosion resistance coatings: What works and what does not work?10.1016/j.jlp.2020.104376 ↗
15. Electrodeposition of zinc and composite zinc–yttria stabilized zirconia coatings10.1016/j.jmatprotec.2008.06.031 ↗
16. Surface characterization, mechanical properties and corrosion behaviour of ternary based Zn-ZnO-SiO2 composite coating of mild steel10.1016/j.jallcom.2015.09.090 ↗
17. Enhanced Hardness and Corrosion Resistance of Zn/SiO2 Films by Electrodeposition10.1149/2.0821509jes ↗
18. Morphology Control of Zn-SiO2 Composite Films Electrodeposited from Aqueous Solution Containing Quaternary Ammonium Cations10.1088/1742-6596/417/1/012006 ↗
19. Zn–ZrO2 nanocomposite coatings: Electrodeposition and evaluation of corrosion resistance10.1016/j.apsusc.2011.05.067 ↗
20. Effect of current density on corrosion and mechanical properties of Zn-SiC composite coating10.1016/j.matpr.2019.06.348 ↗
21. Studies on electrodeposition of Zn–MoS2 nanocomposite coatings on mild steel and its properties10.1007/s10008-011-1475-8 ↗
22. Electrogalvanization using Zn-graphene oxide composite coatings with enhance corrosion resistance performance10.1007/s11998-020-00439-9 ↗
23. Electrodeposition and the properties of a Zn-cotton nanocrystal composite coating10.1016/j.jmrt.2022.01.016 ↗
24. Electrolytic zinc composite coatings: Ultrasound assisted deposition for morphological and composition modification10.1149/09210.0025ecst ↗
25. Praveen Kumar, C.M., Gowdru Chandrashekarppa, M.P., Mahabaleshwar Kulkarni, R., Yurievich Pimenov, D., and Giasin, K. (2021). The effect of Zn and Zn-WO3 composites nanocoatings deposition on hardness and corrosion resistance n steel substrate. Materials, 14.10.3390/ma14092253 ↗
26. Corrosion behaviour of Zn-Ni alloy and Zn-Ni nano-TiO2 composite coatings electrodeposited from ammonium citrate baths10.1016/j.psep.2020.05.048 ↗
27. Electrodeposited Ni-Co alloy-particle composite coatings: A comprehensive review10.1016/j.surfcoat.2019.125153 ↗
28. The effect of the ultrasound agitation and source of ceria particles on the morphology and structure of the Zn-Co-CeO2 composite coatings10.1016/j.jmrt.2021.05.064 ↗
29. Ridosic, M., Bucko, M., Salicio-Paz, A., Garcia-Lecina, E., Zivkovic, L.S., and Bajat, J.B. (2021). Ceria particles as efficient dopant in the electrodeposition of Zn-Co-CeO2 composite coatings with enhanced corrosion resistance. The effect of current density and particle concentration. Molecules, 26.10.3390/molecules26154578 ↗
30. Synthesis of Ni-Co-ZrO2 nanocomposites doped with ceria particles via electrodeposition as highly protective coating10.1016/j.jallcom.2019.153158 ↗
31. Electrolytic co-deposition of silicate and mica particles with zinc10.1007/s10008-004-0572-3 ↗
32. Initial corrosion behavior of composite coatings obtained by co-electrodeposition of zinc with nanoparticles of Ti and Ce oxides10.1007/s10008-012-1901-6 ↗
33. (2019). Standard Practice for Operating Salt Spray (Fog) Apparatus (Standard No. ASTM B117).
34. Electrochemical studies on Zn/nano-CeO2 electrodeposited composite coatings10.1016/j.surfcoat.2012.08.004 ↗
35. Electrodeposition of zinc–ceria nanocomposite coatings in alkaline bath10.1007/s10008-013-2264-3 ↗
36. Electrodeposition on Ni-SiC nanocomposite coatings and evaluation of the wear and corrosion resistance and electroplating characteristics10.1016/j.colsurfa.2007.07.027 ↗
37. Abdeen, D.H., El Hachach, M., Koc, M., and Atieh, M.A. (2019). A review on the corrosion behaviour of nanocoatings on metallic substrates. Materials, 12.10.3390/ma12020210 ↗
38. Role of Ceria Nanoparticles on the Electrodeposited Zinc Coating’s Growth: Interest of a TEM-Scale Investigation10.1149/2.0011410eel ↗
39. Validation of corrosion rates measured by the Tafel extrapolation method10.1016/j.corsci.2005.05.046 ↗
40. The Analysis of electrodes Impedances Complicated by the Presence of a Constant Phase element10.1016/S0022-0728(84)80324-1 ↗
41. Concerning the conversion of the constant phase element parameter Y0 into a capacitance10.5006/1.3280607 ↗
42. Structural factor of Zn alloy electrodeposit corrosion10.1016/S0169-4332(99)00334-7 ↗
43. An investigation on the role of texture and surface morphology in the corrosion resistance of zinc electrodeposits10.1016/j.corsci.2011.04.007 ↗
44. Synergistic effects of additives on morphology, texture and discharge mechanism of zinc during electrodeposition10.1016/j.jelechem.2011.10.001 ↗
45. Electrodeposition of Zinc from acid based solutions: A review and experimental study10.3923/ajaps.2012.314.326 ↗
46. Electrodeposition of Zinc-SiO2 Composite10.1149/1.1393577 ↗
47. Electrochemical polarization I. A theoretical analysis of the shape of polarization curves10.1149/1.2428496 ↗
48. Initial formation of corrosion products on pure zinc in saline solution10.1016/j.bioactmat.2018.08.003 ↗
49. Dramatic reduction of the oxygen vacancy formation energy in ceria particles: A possible key to their remarkable reactivity at the nanoscale10.1039/c0jm01908a ↗
50. Size-dependent oxygen storage ability of nano-sized ceria10.1039/c3cp51959g ↗
51. CeO2 modified SiO2 acted as additive in electrodeposition of Zn-Ni alloy coating with enhanced corrosion resistance10.1016/j.jallcom.2017.11.031 ↗
52. Understanding of the oxygen activation on ceria-and ceria/alumina-supported gold catalysts: A study combining 18O/16O isotopic exchange and EPR spectroscopy10.1007/s13404-013-0103-z ↗
53. Effect of nano-zirconia on electrochemical performance, corrosion behavior and microstructure of Al-Mg-Sn-Ga anode for aluminium batteries10.1016/j.jallcom.2019.04.110 ↗
54. Electrodeposited Zn–TiO2 nanocomposite coatings and their corrosion behavior10.1007/s10800-010-0130-x ↗
55. Structure—Activity Map of Ceria Nanoparticles, Nanocubes, and Mesoporous Architectures10.1021/acs.chemmater.6b02536 ↗
56. Modeling ceria-based nanomaterials for catalysis and related applications10.1007/s10562-016-1799-1 ↗
57. EIS study of the corrosion behavior of zinc-based coatings on steel in quiescent 3% NaCl solution. Part 1: Directly exposed coatings10.1016/j.corsci.2003.09.032 ↗
58. Electrochemical corrosion monitoring of galvanized steel under cyclic wet-dry conditions10.1016/S0010-938X(99)00057-8 ↗
59. Characterization of corrosion resistance of electrodeposited Zn–Ni Zn and Cd coatings10.1016/j.electacta.2013.05.010 ↗
60. Effect of crystallographic orientation on the tribological behavior of electrodeposited Zn coatings10.1039/C5RA15490A ↗
61. Preparation and corrosion resistance of pulse electrodeposited Zn and Zn-SiC nanocomposite coatings10.1016/j.apsusc.2013.12.143 ↗
62. Poupard, S., Pedraza, F., and Creus, J. (2009). Diffusion of a Corroding Electrolyte through Defective Electroplated Ceria Based Coatings. Defect and Diffusion Forum, Trans Tech Publications.10.4028/www.scientific.net/DDF.289-292.235 ↗
63. Surface study of cerium oxide based coatings obtained by cathodic electrodeposition on zinc10.1016/j.apsusc.2011.02.033 ↗
64. The characterization of electrodeposited Zn-SiO2 composites before and after corrosion test10.1016/0010-938X(94)90011-6 ↗
65. Comparative EIS study of pretreatment performance in coated metals10.1016/S0300-9440(96)00691-1 ↗
66. Electrochemical impedance spectroscopy (EIS) of corrosion processes on inhomogeneous surfaces10.1016/0013-4686(90)80004-8 ↗
67. Corrosion inhibition of steel in sodium chloride solution by undoped polyaniline epoxy blend coating10.1016/j.porgcoat.2008.07.018 ↗
68. Electrochemical Impedance Spectroscopy on 3-D Inhomogeneous Surfaces: Corrosion in Neutral Aerated Solutions10.1149/1.2095610 ↗
69. An electrochemical impedance spectroscopy study of the corrosion behavior of PVD coated steels in 0.5 M NaCl aqueous solution: Part I. Establishment of equivalent circuits for EIS data modelling10.1016/S0010-938X(02)00213-5 ↗
70. Corrosion behavior in saline solution of pulsed electrodeposited zinc-nickel-ceria nanocomposite coatings10.1002/maco.201709419 ↗
71. Corrosion resistance and microstructure of electrodeposited Zn and Zn alloy coatings10.1016/S0257-8972(96)03125-8 ↗
72. Corrosion resistance of electroplated zinc alloy coatings10.1080/00202967.1989.11870845 ↗
73. Formation of the main atmospheric zinc end products: NaZn4Cl(OH)6SO4. 6H2O, Zn4SO4(OH)6. nH2O and Zn4Cl2 (OH) 4SO4. 5H2O in [Cl−] [SO2−4] [HCO−3] [H2O2] electrolytes10.1016/S0010-938X(98)00176-0 ↗
74. The effect of an artificially synthesized simonkolleite layer on the corrosion of electrogalvanized steel10.1016/j.corsci.2012.10.024 ↗
75. Electrochemical codeposition of PMMA particles with zinc10.1016/j.surfcoat.2010.06.011 ↗