Contribution of Magnetization Mechanisms in MnZn Ferrites with Different Grain Sizes and Sintering Densification
Source abstract
Abstract
This study investigates the magnetization mechanisms in MnZn ferrites, which are key materials in high-frequency power electronics, to understand their behavior under various sintering conditions. Employing X-ray diffraction and scanning electron microscopy, we analyzed the microstructure and phase purity of ferrites sintered at different temperatures. Our findings confirm consistent spinel structures and highlight significant grain-growth and densification variabilities. Magnetic properties, particularly the saturation magnetization (Ms) and initial permeability (μi), were explored, revealing their direct correlation with the sintering process. The decomposition of magnetic spectra into domain-wall-motion and spin-rotation components offered insights into the dominant magnetization mechanisms, with the domain wall movement becoming increasingly significant at higher sintering temperatures. The samples sintered at 1310 °C showcased superior permeability and the least loss in our investigations. This research underscores the impact of sintering conditions on the magnetic behavior of MnZn ferrites, providing valuable guidelines for optimizing their magnetic performance in advanced electronic applications and contributing to the material science field’s understanding of the interplay between sintering, microstructures, and magnetic properties.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Magnetic Properties and Synthesis of Ferrites · Magnetic Properties and Applications · Magnetic Properties of Alloys
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Hubei Key Laboratory of Low Dimensional Optoelectronic Materials and Devices, Hubei University of Arts and Science, Xiangyang 441053, China
School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 610054, China
Hubei Huaci Electronic Technology Co., Ltd., Xiangyang 441053, China
Funding
Research and Development Projects in Xiangyang City
References (41)
Show source-provided references
1. Magnetic Nanoferrites for RF CMOS: Enabling 5G and Beyond10.1149/2.F08174if ↗
2. A Compact 5G Antenna Printed on Manganese Zinc Ferrite Substrate Material10.1587/elex.13.20160377 ↗
3. Design of a Wide-Input-Voltage PCB-Embedded Transformer Based Active-Clamp Flyback Converter Considering Permeability Degradation10.1109/TPEL.2021.3064536 ↗
4. Optimized Kilowatt-Range Boost Converter Based on Impulse Rectification with 52 kW/l and 98.6% Efficiency10.1109/TPEL.2020.3045062 ↗
5. Review of Integrated Magnetics for Power Supply on Chip (PwrSoC)10.1109/TPEL.2012.2198891 ↗
6. A Novel Method to Predict the Real Operation of Ferrite Inductors with Moderate Saturation in Switching Power Supply Applications10.1109/TPEL.2015.2438952 ↗
7. Iron-Based Soft Magnetic Composites with Mn–Zn Ferrite Nanoparticles Coating Obtained by Sol–Gel Method10.1016/j.jmmm.2012.06.042 ↗
8. Synthesis and the Physical Properties of MnZn Ferrite and NiMnZn Ferrite–Polyaniline Nanocomposite Particles10.1039/B408165J ↗
9. Development of High-Temperature High-Permeability MnZn Power Ferrites for MHz Application by Nb2O5 and TiO2 Co-Doping10.1016/j.ceramint.2019.12.140 ↗
10. High Permeability–High Frequency Stable MnZn Ferrites10.1016/j.jmmm.2012.04.011 ↗
11. High Permeability of Low Loss Mn–Zn Ferrite Obtained by Sintering Nanoparticle Mn–Zn Ferrite10.1016/j.jmmm.2006.01.018 ↗
12. Influence of V2O5 Addition on the Grain Growth and Magnetic Properties of Mn–Zn High Permeability Ferrites10.1016/j.jmmm.2006.05.023 ↗
13. Effects of Calcining and Sintering Parameters on the Magnetic Properties of High-Permeability MnZn Ferrites10.1109/TMAG.2005.855327 ↗
14. Active Power Device Selection in High- and Very-High-Frequency Power Converters10.1109/TPEL.2018.2874420 ↗
15. Steinmetz Law for Ac Magnetized Iron-Phenolformaldehyde Resin Soft Magnetic Composites10.1016/j.jmmm.2016.10.060 ↗
16. Ying, Y., Hu, L., Li, Z., Zheng, J., Yu, J., Li, W., Qiao, L., Cai, W., Li, J., and Bao, D. (2023). Preparation of Densified Fine-Grain High-Frequency MnZn Ferrite Using the Cold Sintering Process. Materials, 16.10.3390/ma16093454 ↗
17. A Comprehensive Study on MnZn Ferrite Materials with High Saturation Magnetic Induction Intensity and High Permeability for Magnetic Field Energy Harvesting10.1016/j.jmmm.2023.171635 ↗
18. Effect of Compressive Stress on Power Loss of Mn–Zn Ferrite for High-Frequency Applications10.1016/j.ceramint.2022.03.042 ↗
19. Calcination Induced Phase Transformation in MnZn Ferrite Powders10.1016/j.jallcom.2019.152307 ↗
20. Mechanistic Insights into the Sol-Gel Synthesis of Complex (Quaternary) Co–Mn–Zn-Spinel Ferrites: An Annealing Dependent Study10.1016/j.ceramint.2020.04.031 ↗
21. Microstructure and Magnetic Properties of Sn-Substituted MnZn Ferrites10.1016/j.jmmm.2009.04.053 ↗
22. The Improved Saturation Magnetization and Initial Permeability in Mn–NiZn Ferrites after Cooling in Vacuum10.1007/s00339-022-05422-2 ↗
23. Hysteresis Losses of Minor Loops versus Temperature in MnZn Ferrite10.1109/TMAG.2012.2219877 ↗
24. Complex Additive Systems for Mn-Zn Ferrites with Low Power Loss10.1063/1.4918692 ↗
25. Cation Distribution and Temperature Dependence of Brillouin Function for Nickel-Substituted Manganese–Zinc Ferrites10.1109/TMAG.2015.2446754 ↗
26. Enhanced Magnetic Domain Relaxation Frequency and Low Power Losses in Zn2+ Substituted Manganese Ferrites Potential for High Frequency Applications10.1016/j.jmmm.2016.07.011 ↗
27. Thermomagnetization Characteristics and Ferromagnetic Resonance Linewidth Broadening Mechanism for Ca-Sn Co-Substituted YIG Ferrites10.1016/j.ceramint.2018.03.249 ↗
28. Barium Hexaferrites with Narrow Ferrimagnetic Resonance Linewidth Tailored by Site-Controlled Cu Doping10.1111/jace.18702 ↗
29. Structural and Mössbauer Spectral Studies of Nanosized Aluminum Doped Manganese Zinc Ferrites
30. Cation Distribution in Ni-Substituted Mn-Ferrites by Mössbauer Technique10.1023/B:JRNC.0000011746.68066.f5 ↗
31. Effects of Magnetic Domain Morphology on the Magnetic Spectrum and High-Frequency Core Losses of MnZn Ferrites10.1111/jace.19519 ↗
32. Excellent Tunable DC Bias Superposition Characteristics for Manganese–Zinc Ferrites10.1109/TPEL.2019.2921868 ↗
33. The Influence of Remanence on Magnetostrictive Vibration and Hysteresis in Mn-Zn Ferrite Cores10.1109/TMAG.2011.2174251 ↗
34. Emerging Magnetodielectric Materials for 5G Communications: 18H Hexaferrites10.1016/j.actamat.2022.117854 ↗
35. Suppressed Domain Wall Damping in Planar BaM Hexaferrites for Miniaturization of Microwave Devices10.1016/j.jmmm.2020.167172 ↗
36. Domain Structure of Polycrystalline MnZn Ferrites10.1016/S0921-5107(00)00585-7 ↗
37. Bounds on the Dynamic Properties of Magnetic Materials10.1103/PhysRevB.62.11324 ↗
38. Mechanisms and Kinetics of the Migration of Grain Boundaries Containing Extended Defects10.1103/PhysRevB.92.174115 ↗
39. Excessive Grain Boundary Conductivity of Spin-Spray Deposited Ferrite/Non-Magnetic Multilayer10.1063/1.3676242 ↗
40. Temperature Dependence of Core Loss in Co-Substituted MnZn Ferrites10.1063/1.1557952 ↗
41. Frequency Dispersion of Complex Permeability in Mn–Zn and Ni–Zn Spinel Ferrites and Their Composite Materials10.1063/1.1542651 ↗