journal article·2024-03-29Open access

Machine Learning-Based Predictions of Porosity during Cold Spray Deposition of High Entropy Alloy Coatings

Deepak Sharma, Dibakor Boruah, Ali Alperen Bakir, Ahamed Ameen, Shiladitya Paul

Coatings· Volume 14· Issue 4

Abstract

Porosity poses a challenge to the mechanical properties of cold sprayed coatings, especially when it is open or surface-connected, limiting the coatings’ capabilities to act as a barrier. The porosity formation is dependent on the feedstock powder characteristics and the cold spray process parameters. We present a machine learning-based approach to predict porosity based on the above-mentioned factors. Nine different machine learning models based on linear regression (LR), decision trees, random forests, gradient boosting, support vector machine (SVM), and neural networks were explored. Considering the excellent properties of high entropy alloys, Cantor alloy was taken as the consumable. Our dataset, derived from the literature and experiments, identified SVM with a linear kernel and LR as the top-performing models based on the Pearson correlation coefficient (PCC) and root mean square error, where the PCC values exceeded 0.8. The SHapley Additive exPlanations method helped in identifying that the type of gas and powder are the top two factors in pore formation.
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Research context

OpenAlex topics: High-Temperature Coating Behaviors · High Entropy Alloys Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Materials Innovation Centre, School of Engineering, University of Leicester, Leicester LE1 7RH, UK

Materials Performance and Integrity Technology Group, TWI Ltd., Cambridge CB21 6AL, UK

Funding

European Union’s Horizon 2020 research and innovation programme

References (39)

Show source-provided references
1. Cold spraying—A materials perspective10.1016/j.actamat.2016.06.034 ↗
2. The effect of annealing on trapped copper oxides in particle-particle interfaces of cold-sprayed Cu coatings10.1016/j.scriptamat.2021.114333 ↗
3. Cold Spray Additive Manufacturing: Microstructure Evolution and Bonding Features10.1021/accountsmr.1c00138 ↗
4. Cold-sprayed coatings: Microstructure, mechanical properties, and wear behaviour10.1016/j.pmatsci.2021.100839 ↗
5. Adiabatic shear instability is not necessary for adhesion in cold spray10.1016/j.actamat.2018.07.065 ↗
6. A numerical study of pore formation mechanisms in aluminium cold spray coatings
7. Investigating the Effect of Porosity on Corrosion Resistance and Hardness of WC-Co Coatings on Metal Substrates
8. A study of the parameters affecting the particle velocity in cold-spray: Theoretical results and comparison with experimental data
9. Influence of feedstock powder and cold spray processing parameters on microstructure and mechanical properties of Ti-6Al-4V cold spray depositions10.1016/j.surfcoat.2017.12.014 ↗
10. A critical review of high entropy alloys and related concepts10.1016/j.actamat.2016.08.081 ↗
11. Mechanical properties of Cantor alloys driven by additional elements: A review10.1016/j.jmrt.2021.09.019 ↗
12. Nanostructured nitride films of multi-element high-entropy alloys by reactive DC sputtering10.1016/j.surfcoat.2004.08.023 ↗
13. Microstructural development in equiatomic multicomponent alloys10.1016/j.msea.2003.10.257 ↗
14. Microstructural Study of Cold-Sprayed CoCrFeNiMn High Entropy Alloy10.1007/s11666-023-01646-7 ↗
15. Tuning the Microstructure and Mechanical Properties of Cold Sprayed Equiatomic CoCrFeMnNi High-Entropy Alloy Coating Layer10.1007/s12540-020-00886-4 ↗
16. Solid-state cold spraying of FeCoCrNiMn high-entropy alloy: An insight into microstructure evolution and oxidation behavior at 700–900 °C10.1016/j.jmst.2020.06.041 ↗
17. Microstructural, Mechanical and Wear Behavior of HVOF and Cold-Sprayed High-Entropy Alloys (HEAs) Coatings10.1007/s11666-021-01293-w ↗
18. Cavaliere, P., Perrone, A., Silvello, A., Laska, A., Blasi, G., and Cano, I.G. (2022). Fatigue Bending of V-Notched Cold-Sprayed FeCoCrNiMn Coatings. Metals, 12.10.3390/met12050780 ↗
19. Cold Spray Additive Manufacturing of CoCrFeNiMn High-Entropy Alloy: Process Development, Microstructure, and Mechanical Properties10.1007/s11666-022-01374-4 ↗
20. Process optimisation of cold spray additive manufacturing of FeCoNiCrMn high-entropy alloy10.1080/13621718.2023.2190264 ↗
21. A machine learning-based alloy design system to facilitate the rational design of high entropy alloys with enhanced hardness10.1016/j.actamat.2021.117431 ↗
22. Machine learning-based predictions of fatigue life for multi-principal element alloys10.1016/j.scriptamat.2022.115214 ↗
23. Unlocking the potential of CuAgZr metallic glasses: A comprehensive exploration with combinatorial synthesis, high-throughput characterization, and machine learning10.1002/advs.202302997 ↗
24. Chollet, F. (2021). Deep Learning with Python, Manning Shelter Island.
25. Roy, S., and Ravi, K. (2022, January 4–6). A Machine Learning Based Approach for Cold Spray Deposition Porosity Prediction from Processing Parameters. Proceedings of the Thermal Spray 2022: Proceedings from the International Thermal Spray Conference, Vienna, Austria.10.31399/asm.cp.itsc2022p0961 ↗
26. Prediction and analysis of high velocity oxy fuel (HVOF) sprayed coating using artificial neural network10.1016/j.surfcoat.2019.124988 ↗
27. Effect of connected pores on the corrosion behavior of plasma sprayed alumina coatings10.1016/S0257-8972(89)80033-7 ↗
28. The impact of corrosion on society10.1007/s11661-011-0703-2 ↗
29. The importance of being porous10.1038/s41560-019-0455-6 ↗
30. Historical commentary NIH Image to ImageJ: 25 years of image analysis10.1038/nmeth.2089 ↗
31. Muller, A.C., and Guido, S. (2016). Introduction to Machine Learning with Python: A Guide for Data Scientists, O’Reilly Media.
32. Deep Learning: A Comprehensive Overview on Techniques, Taxonomy, Applications and Research Directions10.1007/s42979-021-00815-1 ↗
33. SHAP and LIME: An Evaluation of Discriminative Power in Credit Risk10.3389/frai.2021.752558 ↗
34. Silvello, A., Cavaliere, P.D., Albaladejo, V., Martos, A., Dosta, S., and Cano, I.G. (2020). Powder properties and processing conditions affecting cold spray deposition. Coatings, 10.10.3390/coatings10020091 ↗
35. Villafuerte, J. (2020). Modern Cold Spray Materials, Process, and Applications, Springer.
36. Effect of processing conditions on porosity formation in cold gas dynamic spraying of copper10.1361/105996306X124437 ↗
37. Particle velocity and deposition efficiency in the cold spray process10.1361/105996399770350278 ↗
38. Machine learning based fatigue life prediction with effects of additive manufacturing process parameters for printed SS 316L10.1016/j.ijfatigue.2020.105941 ↗
39. Effects of traverse scanning speed of spray nozzle on the microstructure and mechanical properties of cold-sprayed Ti6Al4V coatings10.1007/s11666-017-0619-5 ↗