2024 roadmap on magnetic microscopy techniques and their applications in materials science
Source abstract
Abstract
Abstract Considering the growing interest in magnetic materials for unconventional computing, data storage, and sensor applications, there is active research not only on material synthesis but also characterisation of their properties. In addition to structural and integral magnetic characterisations, imaging of magnetisation patterns, current distributions and magnetic fields at nano- and microscale is of major importance to understand the material responses and qualify them for specific applications. In this roadmap, we aim to cover a broad portfolio of techniques to perform nano- and microscale magnetic imaging using superconducting quantum interference devices, spin centre and Hall effect magnetometries, scanning probe microscopies, x-ray- and electron-based methods as well as magnetooptics and nanoscale magnetic resonance imaging. The roadmap is aimed as a single access point of information for experts in the field as well as the young generation of students outlining prospects of the development of magnetic imaging technologies for the upcoming decade with a focus on physics, materials science, and chemistry of planar, three-dimensional and geometrically curved objects of different material classes including two-dimensional materials, complex oxides, semi-metals, multiferroics, skyrmions, antiferromagnets, frustrated magnets, magnetic molecules/nanoparticles, ionic conductors, superconductors, spintronic and spinorbitronic materials.
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Research context
OpenAlex topics: Diamond and Carbon-based Materials Research · Electronic and Structural Properties of Oxides · Force Microscopy Techniques and Applications
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (100+)
Show source-provided references
1. Clarke · 2004 · vol I
2. Studying quantum materials with scanning SQUID microscopy10.1146/annurev-conmatphys-031620-104226 ↗
3. NanoSQUIDs: basics & recent advances10.1515/psr-2017-5001 ↗
4. Gradiometric micro-SQUID susceptometer for scanning measurements of mesoscopic samples10.1063/1.2932341 ↗
5. Self-aligned nanoscale SQUID on a tip10.1021/nl100009r ↗
6. A scanning superconducting quantum interference device with single electron spin sensitivity10.1038/nnano.2013.169 ↗
7. Magnetic, thermal, and topographic imaging with a nanometer-scale SQUID-on-lever scanning probe10.1103/PhysRevApplied.17.034002 ↗
8. Fundamental studies of superconductors using scanning magnetic imaging10.1088/0034-4885/73/12/126501 ↗
9. Improving the sensitivity of scanning probe microscopy with mechanical vibrations10.1063/1.5051620 ↗
10. A micro-SQUID with dispersive readout for magnetic scanning microscopy10.1063/1.5030489 ↗
11. Scanning SQUID sampler with 40-ps time resolution10.1063/1.4986525 ↗
12. Nanoscale thermal imaging of dissipation in quantum systems10.1038/nature19843 ↗
13. Superconducting on-chip spectrometer for mesoscopic quantum systems10.1103/PhysRevResearch.3.043078 ↗
14. Josephson junctions and SQUIDs created by focused helium-ion-beam irradiation of YBa2Cu3O710.1103/PhysRevApplied.11.044082 ↗
15. Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface10.1038/nphys2079 ↗
16. Strain-tunable magnetism at oxide domain walls10.1038/s41567-018-0363-x ↗
17. Imaging and control of ferromagnetism in LaMnO3/SrTiO3 heterostructures10.1126/science.aaa5198 ↗
18. Visualization of superparamagnetic dynamics in magnetic topological insulators10.1126/sciadv.1500740 ↗
19. Imaging orbital ferromagnetism in a moiré Chern insulator10.1126/science.abd3190 ↗
20. Colossal magnetoresistance without mixed valence in a layered phosphide crystal10.1002/adma.202005755 ↗
21. Imaging and tuning polarity at SrTiO3 domain walls10.1038/nmat4966 ↗
22. Pairing symmetry in cuprate superconductors10.1103/RevModPhys.72.969 ↗
23. Angle-resolved phase-sensitive determination of the in-plane gap symmetry in YBa2Cu3O7-δ10.1038/nphys215 ↗
24. Imaging of super-fast dynamics and flow instabilities of superconducting vortices10.1038/s41467-017-00089-3 ↗
25. Imaging quantum fluctuations near criticality10.1038/s41567-018-0264-z ↗
26. Spatial control of heavy-fermion superconductivity in CeIrIn510.1126/science.aao6640 ↗
27. Superfluid response of an atomically thin, gate-tuned van der Waals superconductor10.1038/s41467-023-37210-8 ↗
28. Nonsinusoidal current-phase relationship in Josephson junctions from the 3D topological insulator HgTe10.1103/PhysRevLett.114.066801 ↗
29. Current-phase relations of few-mode InAs nanowire Josephson junctions10.1038/nphys4224 ↗
30. Magnetic memory and spontaneous vortices in a van der Waals superconductor10.1038/s41586-022-04855-2 ↗
31. Superconducting vortices carrying a temperature-dependent fraction of the flux quantum10.1126/science.abp9979 ↗
32. Imaging currents in HgTe quantum wells in the quantum spin Hall regime10.1038/nmat3682 ↗
33. Direct visualization of electronic transport in a quantum anomalous Hall insulator10.1038/s41563-023-01622-0 ↗
34. Locally enhanced conductivity due to the tetragonal domain structure in LaAlO3/SrTiO3 heterointerfaces10.1038/nmat3753 ↗
35. Non-universal current flow near the metal-insulator transition in an oxide interface10.1038/s41467-021-23393-5 ↗
36. Direct observation of vortices in an electron fluid10.1038/s41586-022-04794-y ↗
37. Nanoscale imaging of equilibrium quantum Hall edge currents and of the magnetic monopole response in graphene10.1038/s41567-019-0713-3 ↗
38. Mapping the twist-angle disorder and Landau levels in magic-angle graphene10.1038/s41586-020-2255-3 ↗
39. Visualizing current in superconducting networks10.1103/PhysRevApplied.17.024073 ↗
40. Emergent nanoscale superparamagnetism at oxide interfaces10.1038/ncomms12566 ↗
41. Spin microscope based on optically detected magnetic resonance10.1063/1.1829373 ↗
42. High-sensitivity diamond magnetometer with nanoscale resolution10.1038/nphys1075 ↗
43. Scanning magnetic field microscope with a diamond single-spin sensor10.1063/1.2943282 ↗
44. High sensitivity magnetic imaging using an array of spins in diamond10.1063/1.3385689 ↗
45. Sensitivity optimization for NV-diamond magnetometry10.1103/RevModPhys.92.015004 ↗
46. Spin-polarization mechanisms of the nitrogen-vacancy center in diamond10.1021/nl903646p ↗
47. Orders of magnitude improvement in coherence of silicon-vacancy ensembles in isotopically purified 4H-SiC10.1103/PRXQuantum.3.010343 ↗
48. Engineering preferentially-aligned nitrogen-vacancy centre ensembles in CVD grown diamond10.1038/s41598-019-42314-7 ↗
49. Introduction to quantum optimal control for quantum sensing with nitrogen-vacancy centers in diamond10.1116/5.0006785 ↗
50. N-V–diamond magnetic microscopy using a double quantum 4-Ramsey protocol10.1103/PhysRevApplied.15.044020 ↗
51. High-speed wide-field imaging of microcircuitry using nitrogen vacancies in Diamond10.1103/PhysRevApplied.17.064051 ↗
52. Subpicotesla diamond magnetometry10.1103/PhysRevX.5.041001 ↗
53. Magnetometry based on the excited-state lifetimes of a single nitrogen-vacancy center in diamond10.1063/5.0070639 ↗
54. Quantum point defects in 2D materials—the QPOD database10.1038/s41524-022-00730-w ↗
55. Charge stabilization of shallow nitrogen-vacancy centers using graphene/diamond junctions10.1063/5.0143062 ↗
56. Measurement and simulation of the magnetic fields from a 555 timer integrated circuit using a quantum diamond microscope and finite-element analysis10.1103/PhysRevApplied.17.014021 ↗
57. Quantum imaging of current flow in graphene10.1126/sciadv.1602429 ↗
58. Imaging viscous flow of the Dirac fluid in graphene10.1038/s41586-020-2507-2 ↗
59. Spatiotemporal mapping of a photocurrent vortex in monolayer MoS2 using diamond quantum sensors10.1103/PhysRevX.10.011003 ↗
60. Strong correlation between superconductivity and ferromagnetism in an Fe-chalcogenide superconductor10.1021/acs.nanolett.1c02424 ↗
61. Imaging spin-wave damping underneath metals using electron spins in diamond10.1002/qute.202100094 ↗
62. Scanning nitrogen-vacancy magnetometry down to 350 mK10.1063/5.0093548 ↗
63. High spatial and temporal resolution wide-field imaging of neuron activity using quantum NV-diamond10.1038/srep00401 ↗
64. Wide-field magnetometry using nitrogen-vacancy color centers with randomly oriented micro-diamonds10.1038/s41598-022-22610-5 ↗
65. Silicon-vacancy nanodiamonds as high performance near-infrared emitters for live-cell dual-color imaging and thermometry10.1021/acs.nanolett.2c00040 ↗
66. A robust scanning diamond sensor for nanoscale imaging with single nitrogen-vacancy centres10.1038/nnano.2012.50 ↗
67. Magneto-optical imaging of thin magnetic films using spins in diamond10.1038/srep22797 ↗
68. Magnetic measurements on micrometer-sized samples under high pressure using designed NV centers10.1126/science.aaw4329 ↗
69. Coherent quantum control of nitrogen-vacancy center spins near 1000 kelvin10.1038/s41467-019-09327-2 ↗
70. Improved current density and magnetization reconstruction through vector magnetic field measurements10.1103/PhysRevApplied.14.024076 ↗
71. Untrained physically informed neural network for image reconstruction of magnetic field sources10.1103/PhysRevApplied.18.064076 ↗
72. Nanoscale imaging of current density with a single-spin magnetometer10.1021/acs.nanolett.6b05304 ↗
73. Widefield quantum microscopy with nitrogen-vacancy centers in diamond: strengths, limitations, and prospects10.1063/5.0066733 ↗
74. Single crystal diamond pyramids for applications in nanoscale quantum sensing10.1364/OME.380362 ↗
75. Electric noise spectra of a near-surface nitrogen-vacancy center in diamond with a protective layer10.1103/PhysRevApplied.10.064056 ↗
76. Single-nitrogen–vacancy NMR of amine-functionalized diamond surfaces10.1021/acs.nanolett.2c00533 ↗
77. High-fidelity single-shot readout of single electron spin in diamond with spin-to-charge conversion10.1038/s41467-021-21781-5 ↗
78. Robust all-optical single-shot readout of nitrogen-vacancy centers in diamond10.1038/s41467-020-20755-3 ↗
79. Hrubesch · Phys. Rev. Lett. · 2017 · 11810.1103/PhysRevLett.118.037601 ↗
80. Siyushev · Science · 2019 · 363 · 72810.1126/science.aav2789 ↗
81. Real-time charge initialization of diamond nitrogen-vacancy centers for enhanced spin readout10.1103/PhysRevApplied.13.024016 ↗
82. Efficient real-time spin readout of nitrogen-vacancy centers based on Bayesian estimation
83. Resource-efficient adaptive Bayesian tracking of magnetic fields with a quantum sensor10.1088/1361-648X/abe34f ↗
84. Quantitative study of the response of a single NV defect in diamond to magnetic noise10.1103/PhysRevB.103.235418 ↗
85. Diamond surface electric-field noise detection using shallow nitrogen-vacancy centers10.1103/PhysRevB.106.165406 ↗
86. Probing magnetism in 2D materials at the nanoscale with single-spin microscopy10.1126/science.aav6926 ↗
87. Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer10.1038/nature23656 ↗
88. Nanomagnetism of magnetoelectric granular thin-film antiferromagnets10.1021/acs.nanolett.8b04681 ↗
89. Nanoscale mechanics of antiferromagnetic domain walls10.1038/s41567-020-01157-0 ↗
90. Olivier Boulle room-temperature skyrmions at zero field in exchange-biased ultrathin films10.1103/PhysRevApplied.13.044079 ↗
91. The nature of domain walls in ultrathin ferromagnets revealed by scanning nanomagnetometry10.1038/ncomms7733 ↗
92. Quantitative nanoscale vortex imaging using a cryogenic quantum magnetometer10.1038/nnano.2016.63 ↗
93. Imaging topological defects in a noncollinear antiferromagnet10.1103/PhysRevLett.128.187201 ↗
94. Magnetometry with nitrogen-vacancy defects in diamond10.1088/0034-4885/77/5/056503 ↗
95. Control and local measurement of the spin chemical potential in a magnetic insulator10.1126/science.aak9611 ↗
96. Quantum-impurity relaxometry of magnetization dynamics10.1103/PhysRevLett.121.187204 ↗
97. A magnon scattering platform10.1073/pnas.2019473118 ↗
98. Long-range spin wave mediated control of defect qubits in nanodiamonds10.1038/s41534-017-0029-z ↗
99. Magnetic resonance imaging of spin-wave transport and interference in a magnetic insulator10.1126/sciadv.abd3556 ↗
100. Filtering and imaging of frequency-degenerate spin waves using nanopositioning of a single-spin sensor10.1021/acs.nanolett.2c02791 ↗